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arXiv:1611.09622 · Physical Review A

Modal decomposition of a propagating matter wave via electron ptychography

Shaohong Cao, Pieter Kok, Peng Li, Andrew Maiden, John Marius Rodenburg

Published Dec 19, 2016• 33 citations
arXivHTMLPDF

Abstract

We employ ptychography, a phase-retrieval imaging technique, to show experimentally that a partially coherent high-energy matter (electron) wave emanating from an extended source can be decomposed into a set of mutually independent modes of minimal rank. Partial coherence significantly determines the optical transfer properties of an electron microscope and so there has been much work on this subject. However, previous studies have employed forms of interferometry to determine spatial coherence between discrete points in the wave field. Here we use the density matrix to derive a formal quantum mechanical description of electron ptychography and use it to measure a full description of the spatial coherence of a propagating matter wave field, at least within the fundamental uncertainties of the measurements we can obtain.

DOI
10.1103/physreva.94.063621

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We employ ptychography, a phase-retrieval imaging technique, to show experimentally that a partially coherent high-energy matter (electron) wave emanating from an extended source can be decomposed into a set of mutually independent modes of minimal rank. Partial coherence significantly determines the optical transfer properties of an electron microscope and so there has been much work on this subject. However, previous studies have employed forms of interferometry to determine spatial coherence between discrete points in the wave field. Here we use the density matrix to derive a formal quantum mechanical description of electron ptychography and use it to measure a full description of the spatial coherence of a propagating matter wave field, at least within the fundamental uncertainties of the measurements we can obtain.
The quantum analogue of ptychography, a powerful coherent diffractive imaging technique, is a simple method for reconstructing d -dimensional pure states. It relies on measuring partially overlapping parts of the input state in a single orthonormal basis and feeding the outcomes to an iterative phase retrieval algorithm for postprocessing. We provide a proof of concept demonstration of this method by determining pure states given by superpositions of d transverse spatial modes of an optical field. A set of n rank- r projectors, diagonal in the spatial mode basis, is used to generate n partially overlapping parts of the input, and each part is projectively measured in the Fourier transformed basis. For d up to 32, we successfully reconstructed hundreds of random states using n = 5 and n = d rank- ⌈ d / 2 ⌉ projectors. The extension of quantum ptychography for other types of photonic spatial modes is outlined.
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A new class of phase-retrieval methods for 2-D fields is introduced. Phase-space tomography can be used for the experimental determination of the amplitude and phase structure of a quasi-monochromatic wave field in a plane normal to its propagation direction. The wave field ψ(r) may represent either a scalar electromagnetic (EM) field or the quantum-mechanical (QM) wave function of a matter wave. The complex wave field may be coherent or partially coherent, in which case the method reconstructs the two-point spatial correlation function, Γ(r, r′) = ⟨ψ(r)ψ*(r′)⟩. (In the QM case, the analogous quantity is the density matrix.) The experiment uses only intensity measurements and refractive optics (lenses), and the data-analysis algorithm is noniterative and requires no deconvolution.
Programmable electron optics -- electronically controlled phase plates -- underpin proposals from dose-efficient phase imaging to shaped-electron X-ray sources, nearly all assuming a pure, fully coherent delivered wave whose purity has never been measured. Here we reconstruct the transverse density matrix of a microelectromechanical electrostatic spiral phase plate by mixed-state ptychography, from one four-dimensional STEM scan per state and without added hardware. The delivered beam is substantially mixed: its purity falls from approximately 0.47 to approximately 0.24 as the applied bias grows, inconsistent with a fixed lateral source-blur model, while the real-space coherence width stays near 1 nm. The same scans calibrate the device in situ, allow virtual orbital-angular-momentum sorting and, through a partial-coherence-aware transfer theory, indicate that purifying the output could improve dose efficiency roughly threefold. One acquisition thus becomes a quantum-state acceptance test for programmable electron optics, supplying the purity and coherence that emerging phase-plate and diffractive-imaging schemes assume but leave unquantified.
A method is proposed for the experimental determination of the amplitude and phase structure of a quasimonochromatic wave field in a plane normal to its propagation direction. The wave field may represent either a scalar electromagnetic (EM) field or the quantum mechanical (QM) wave function of a matter wave. For coherent EM fields or pure QM states, the method uniquely reconstructs the complex wave fields. For partially coherent EM fields or mixed QM states, it reconstructs the two-point correlation function or density matrix. The experiment uses only intensity measurements and refractive optics (lenses), and the data analysis algorithm is noniterative and requires no deconvolution.
Recent advances in optical imaging and communication increasingly involve high-dimensional, partially coherent light, creating a growing need for scalable tools to measure and manipulate coherence. Here, we demonstrate the automatic separation of spatially partially coherent light into "coherence modes" -- its orthogonal and mutually incoherent components. To make this separation possible, we exploit variational processing in layered self-configuring interferometer architectures in a silicon photonic circuit. This process formally finds and measures the eigenvectors and eigenvalues of the coherency matrix, hence measuring the partially coherent state, while leaving it intact and separated after optimization. Furthermore, we show that mutually incoherent beams, if spatially orthogonal, can be automatically separated even if they are completely overlapped, hence separating unknown laser beams based only on their mutual incoherence. Our experiment finds and separates the two strongest coherence modes starting from a nine-mode sampling of the partially or fully overlapping fields from two independent lasers. The method requires a number of physical components that scales linearly with the rank rrr of the coherency matrix and operates through a sequence of rrr in situ gradient-based optimizations enabled by electronic drive frequency multiplexing of interferometer phase shifters. We benchmark its performance against a mixture-based tomographic method, also implemented on chip. These results establish a scalable framework for programmable coherence analysis and control in imaging, communication, and photonic information processing.