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arXiv:1611.08471 · npj Quantum Materials

Controlling heat and particle currents in nanodevices by quantum observation

Robert Biele, César A. Rodríguez-Rosario, Thomas Frauenheim, Ángel Rubio

Published Jun 29, 2017• 18 citations
arXivHTMLPDF

Abstract

Abstract We demonstrate that in a standard thermo-electric nanodevice the current and heat flows are not only dictated by the temperature and potential gradient, but also by the external action of a local quantum observer that controls the coherence of the device. Depending on how and where the observation takes place, the direction of heat and particle currents can be independently controlled. In fact, we show that the current and heat flow in a quantum material can go against the natural temperature and voltage gradients. Dynamical quantum observation offers new possibilities for the control of quantum transport far beyond classical thermal reservoirs. Through the concept of local projections, we illustrate how we can create and directionality control the injection of currents (electronic and heat) in nanodevices. This scheme provides novel strategies to construct quantum devices with application in thermoelectrics, spintronic injection, phononics, and sensing among others. In particular, highly efficient and selective spin injection might be achieved by local spin projection techniques.

DOI
10.1038/s41535-017-0043-6

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Abstract We demonstrate that in a standard thermo-electric nanodevice the current and heat flows are not only dictated by the temperature and potential gradient, but also by the external action of a local quantum observer that controls the coherence of the device. Depending on how and where the observation takes place, the direction of heat and particle currents can be independently controlled. In fact, we show that the current and heat flow in a quantum material can go against the natural temperature and voltage gradients. Dynamical quantum observation offers new possibilities for the control of quantum transport far beyond classical thermal reservoirs. Through the concept of local projections, we illustrate how we can create and directionality control the injection of currents (electronic and heat) in nanodevices. This scheme provides novel strategies to construct quantum devices with application in thermoelectrics, spintronic injection, phononics, and sensing among others. In particular, highly efficient and selective spin injection might be achieved by local spin projection techniques.
Thermoelectric effects, such as the generation of a particle current by a temperature gradient, have their origin in a reversible coupling between heat and particle flows. These effects are fundamental probes for materials and have applications to cooling and power generation. Here, we demonstrate thermoelectricity in a fermionic cold atoms channel in the ballistic and diffusive regimes, connected to two reservoirs. We show that the magnitude of the effect and the efficiency of energy conversion can be optimized by controlling the geometry or disorder strength. Our observations are in quantitative agreement with a theoretical model based on the Landauer-Büttiker formalism. Our device provides a controllable model system to explore mechanisms of energy conversion and realizes a cold atom-based heat engine.
Quantum heat transport governs energy exchange processes and statistical laws in non-equilibrium quantum systems, and plays a pivotal role in quantum thermodynamics. We investigate the steady-state thermal transport of a noncommuting coupled spin system. We employ the quantum dressed master equation approach within the framework of open quantum system theory to accurately analyze the non-equilibrium dynamics, ensuring the validity of transport results in the strong coupling regime. Our results demonstrate that noncommuting spin coupling serves as a significant resource for modulating the nonlinearity of the heat current. Specifically, in the weak spin-coupling regime, the system exhibits robust negative differential thermal conductance (NDTC) across various spin numbers. By deriving analytical expressions for the heat current in both the single-spin and large-spin limits, we reveal that this NDTC behavior is governed by microscopic cycle fluxes. Physically, this arises because spin excitation channels induced by the cold reservoir are suppressed under a large temperature bias, thereby blocking energy exchange cycles. Conversely, in the strong spin-coupling and large temperature bias regime, the quantum system demonstrates pronounced thermal rectification. This high rectification efficiency originates from the unidirectional saturation of the heat current, rendering the system a promising candidate for high-performance thermal diodes. Furthermore, we extend the model to a three-terminal configuration to construct a quantum thermal transistor. By manipulating the temperature of the gate reservoir, we achieve efficient modulation and amplification of heat flow between the source and drain. The heat amplification factor is shown to far exceed unity in specific operating regions, confirming significant thermal amplification.
The unavoidable dissipation of heat in electronic nanostructures is a crucial problem, specially when their operation requires low temperatures. It demands finding devices able to control and redirect the excess heat, ideally without perturbing the electrostatic environment. We propose three-terminal junctions working either as thermal routers or as thermal single-pole double-throw switches controlled by a single external knob. Two models are discussed based on resonant tunneling energy filters and different couplings to the heat source: (i) Phase-coherent contact via a scanning tip modulates the relative amount of the two output currents via position-dependent quantum interference; (ii) Coupling via a gate voltage tunable filter selectively switches one of the currents in the presence of dephasing. In the later case, we find that the heat flow using ideal filtering is bounded by fourth the open conductor current.
In realistic nanoscale transport set-ups, electron-phonon coupling leads to the exchange of heat between phonon baths and electronic reservoirs with finite heat capacities. Such exchange affects the finite reservoir's temperature. However, this sensitivity of the finite reservoir temperature to the exchange of heat with the finite reservoir has remained unexplored for thermometry. Here, we fill this gap by combining current metrology techniques with a thermodynamic framework encompassing finite reservoirs. We focus on an experimentally realizable set-up with a quantum dot coupled to a finite reservoir and consider two distinct current-based strategies in the long time limit, namely monitoring quanta exchanged between the quantum dot and finite reservoir and the measurement of the total current flowing from the quantum dot into an infinite reservoir. A third strategy involves measurements of the quantum dot occupation. For a large but finite reservoir, we show that the Fisher information for all three strategies captures the finite reservoir's contribution to sensitivity through common factors. We also demonstrate that monitoring quanta exchanged between the system and finite reservoir in the long time limit achieves optimal precision. Finally, we provide an optimization analysis that explores how maximal precision can be achieved within each of the current-based strategies by tuning the gate voltage.
Continuous particle exchange thermal machines require no time-dependent driving, can be realised in solid-state electronic devices, and miniaturised to nanometre scale. Quantum dots, providing a narrow energy filter and allowing to manipulate particle flow between the hot and cold reservoirs are at the heart of such devices. It has been theoretically shown that by mitigating passive heat flow, Carnot efficiency can be approached arbitrarily closely in a quantum dot heat engine, and experimentally, values of 0.7ηC have been reached. However, for practical applications, other parameters of a thermal machine, such as maximum power, efficiency at maximum power, and noise - stability of the power output or heat extraction - take precedence over maximising efficiency. We explore the effect of internal microscopic dynamics of a quantum dot on these quantities and demonstrate that its performance as a thermal machine depends on few parameters - the overall conductance and three inherent asymmetries of the dynamics. These parameters will act as a guide to engineering the quantum states of the quantum dot, allowing to optimise its performance beyond that of the simplest case of a two-fold spin-degenerate transmission level.
We propose to generate heat pulses in mesoscopic conductors using light fields. In contrast to single-electron excitations such as levitons, which are created by accurate voltage drives, our approach relies on modulating the temperature of an electronic reservoir. To this end, we show that the interactions with a light field can induce a controllable time-dependent temperature in an electrode. The temperature modulations generate charge-neutral heat pulses that can be emitted into a mesoscopic conductor and detected in the outputs. We illustrate our approach by evaluating the time-dependent currents and their fluctuations using a tight-binding model of two electronic reservoirs connected by a quantum point contact. Our work establishes a route towards on-demand caloritronics, where energy rather than charge carries quantum information, and it paves the way for probing time-resolved heat transport and quantum coherence in thermally driven conductors.