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arXiv:1611.04873 · Physical review. B./Physical review. B

Numerical study of magnetization plateaus in the spin- 1 2 Heisenberg antiferromagnet on the checkerboard lattice

Sylvain Capponi

Published Jan 18, 2017• 16 citations
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Abstract

We present numerical evidence that the spin-1/2 Heisenberg model on the two-dimensional checkerboard lattice exhibits several magnetization plateaus for $m=0, 1/4, 1/2$, and $3/4$, where $m$ is the magnetization normalized by its saturation value. These incompressible states correspond to somewhat similar valence-bond crystal phases that break lattice symmetries, though they are different from the already established plaquette phase for $m=0$. Our results are based on exact diagonalization as well as density-matrix renormalization-group large-scale simulations and interpreted in terms of simple parameter-free trial wave functions.

DOI
10.1103/physrevb.95.014420

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We present numerical evidence that the spin-1/2 Heisenberg model on the two-dimensional checkerboard lattice exhibits several magnetization plateaus for m=0,1/4,1/2m=0, 1/4, 1/2m=0,1/4,1/2, and 3/43/43/4, where mmm is the magnetization normalized by its saturation value. These incompressible states correspond to somewhat similar valence-bond crystal phases that break lattice symmetries, though they are different from the already established plaquette phase for m=0m=0m=0. Our results are based on exact diagonalization as well as density-matrix renormalization-group large-scale simulations and interpreted in terms of simple parameter-free trial wave functions.
We study the ground state of the S=12S=\frac{1}{2}S=21​ Heisenberg model on the checkerboard lattice in a magnetic field by the density matrix renormalization group method with the sine-square deformation. We obtain magnetization plateaus at M/Msat=0,14,38,12M/{M}_{\mathrm{sat}}=0,\frac{1}{4},\frac{3}{8},\frac{1}{2}M/Msat​=0,41​,83​,21​, and 34\frac{3}{4}43​, where Msat{M}_{\mathrm{sat}}Msat​ is the saturated magnetization. The obtained 34\frac{3}{4}43​ plateau state is consistent with the exact result, and the 12\frac{1}{2}21​ plateau is found to have a four-spin resonating loop structure similar to the six-spin loop structure of the 13\frac{1}{3}31​ plateau of the kagome lattice. Different four-spin loop structures are obtained in the 14\frac{1}{4}41​ and 38\frac{3}{8}83​ plateaus but no corresponding states exist in the kagome lattice. The 38\frac{3}{8}83​ plateau has a unique magnetic structure of three types of four-spin local quantum states in a $4\sqrt{2}\ifmmode\times\else\texttimes\fi{}2\sqrt{2}$ magnetic unit cell with a 16-fold degeneracy.
We clarify the existence of several magnetization plateaus for the kagome S=12S=\frac{1}{2}S=21​ antiferromagnetic Heisenberg model in a magnetic field. Using approximate or exact localized magnon eigenstates, we are able to describe in a similar manner the plateau states that occur for magnetization per site m=13m=\frac{1}{3}m=31​, 59\frac{5}{9}95​, and 79\frac{7}{9}97​ of the saturation value. These results are confirmed using large-scale exact diagonalization on lattices up to 63 sites.
I use an improved version of the two-step density-matrix renormalization group method to study ground-state properties of the two-dimensional (2D) Heisenberg model on the checkerboard lattice. In this version, the Hamiltonian is projected on a tensor product of two-leg ladders instead of chains. This allows investigations of 2D isotropic models. I show that this method can describe both the magnetically disordered and ordered phases. The ground-state phases of the checkerboard model as J2{J}_{2}J2​ increases are (i) N\'eel with $Q=(\ensuremath{\pi},\ensuremath{\pi})$, (ii) a valence-bond crystal (VBC) of plaquettes, (iii) N\'eel with $Q=(\ensuremath{\pi}∕2,\ensuremath{\pi})$, and (iv) a VBC of crossed dimers. In agreement with previous results, I find that at the isotropic point J2=J1{J}_{2}={J}_{1}J2​=J1​, the ground state is made of weakly interacting plaquettes with a large gap $\ensuremath{\Delta}\ensuremath{\approx}0.67{J}_{1}$ to triplet excitations. The same approach is also applied to the ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ model. There is no evidence of a columnar dimer phase in the highly frustrated regime.
I use an improved version of the two-step density matrix renormalization group method to study ground-state properties of the 2D Heisenberg model on the checkerboard lattice. In this version the Hamiltonian is projected on a tensor product of two-leg ladders instead of chains. This allows investigations of 2D isotropic models. I show that this method can describe both the magnetically disordered and ordered phases. The ground-state phases of the checkerboard model as J2J_2J2​ increases are: (i) Néel with Q=(π,π)Q=(π,π)Q=(π,π), (ii) a valence bond crystal (VBC) of plaquettes, (iii) Néel with Q=(π/2,π)Q=(π/2,π)Q=(π/2,π), and (iv) a VBC of crossed dimers. In agreement with previous results, I find that at the isotropic point J2=J1J_2=J_1J2​=J1​, the ground state is made of weakly interacting plaquettes with a large gap Δ≈0.67J1Δ\approx 0.67 J_1Δ≈0.67J1​ to triplet excitations.
We analyze the magnetization curve of the spin-1/2 kagome Heisenberg model in a magnetic field. Using state-of-the-art variational wave functions based on neural networks, we confirm the presence of robust magnetization plateaus at m=1/3m=1/3m=1/3, 5/95/95/9 and 7/97/97/9 of the saturation value, stabilized by a spontaneous symmetry breaking of lattice translations with a 3×3\sqrt{3}\times \sqrt{3}3​×3​ unit cell. Regarding the more challenging m=1/9m=1/9m=1/9 plateau, we find two competing valence bond crystals depending on the system size, both breaking translation as well as point group symmetries and with a larger 3×33\times 33×3 unit cell. Such quantum states with local modulations of the magnetization average values could be observed experimentally in the near future.
The spin-12\frac{1}{2}21​ Heisenberg model on a kagome lattice is a typical frustrated quantum spin system. The basic structure of a kagome lattice is also present in the kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus study the magnetization plateaus of the spin-12\frac{1}{2}21​ Heisenberg model on a kagome-strip chain with three-independent antiferromagnetic exchange interactions using the density-matrix renormalization-group method. In a certain range of exchange parameters, we find twelve kinds of magnetization plateaus, nine of which have magnetic structures breaking translational and/or reflection symmetry spontaneously. The structures are classified by an array of five-site unit cells with specific bond-spin correlations. In a case with a nontrivial plateau, namely a 3/10 plateau, we find long-period magnetic structure with a period of four unit cells.