Cat codes are one of the promising encoding schemes for quantum information that enables hardware-efficient error correction. So far, only photonic cat states produced by superconducting circuits have been under consideration. Their realization within coherent spin states (CSS) can pave the way toward nuclear magnetic resonance-based implementations of this new class of codes. Here, we show how the crucial superpositions of CSS can be generated for the nuclear spins. This is through the intrinsic electric quadrupole interaction involving a critical role by the biaxiality term that is readily available, as in strained heterostructures of semiconductors, or defect centers having nearby quadrupolar spins. The persistence of the cat states is achieved using a rotation pulse so as to harness the underlying fixed points of the classical Hamiltonian. We classify the two distinct types as polar- and equator-bound over the Bloch sphere with respect to principal axes, both of which are, so-called mod~2 cat states. Their optimal performance as well as sensitivity under numerous parameter deviations are analyzed. Finally, we show that a higher level, mod 4 cat state, with one of the legs rotating can also be produced along the same spirit using three pulses.
Control over nuclear-spin fluctuations is essential for processes that rely on preserving the quantum state of an embedded system. For this purpose, squeezing is a viable alternative, so far that has not been properly exploited for the nuclear spins. Of particular relevance in solids is the electric quadrupole interaction (QI), which operates on nuclei having spin higher than 1/2. In its general form, QI involves an electric-field gradient (EFG) biaxiality term. Here, we show that as this EFG biaxiality increases, it enables continuous tuning of single-particle squeezing from the one-axis twisting to the two-axis countertwisting limits. A detailed analysis of QI squeezing is provided, exhibiting the intricate consequences of EFG biaxiality. The initial states over the Bloch sphere are mapped out to identify those favorable for fast initial squeezing, or for prolonged squeezings. Furthermore, the evolution of squeezing in the presence of a phase-damping channel and an external magnetic field are investigated. We observe that dephasing drives toward an antisqueezed terminal state, the degree of which increases with the spin angular momentum. Finally, QI squeezing in the limiting case of a two-dimensional EFG with a perpendicular magnetic field is discussed, which is of importance for two-dimensional materials, and the associated beat patterns in squeezing are revealed.
The use of noise-robust qubit encodings provides a way of extending the lifetime of quantum information at the hardware level. In this work, we introduce the spin Kerr-cat encoding, which leverages a sweet spot near a clock transition in the spectrum of quadrupolar nuclei (having spin
I≥1) to achieve a suppression of charge and magnetic noise leading to qubit dephasing. The basis states of the spin Kerr-cat qubit are given by the two lowest levels of a
Z2-symmetric nuclear-spin Hamiltonian and are well approximated by spin cat states for sufficiently high asymmetry parameters. For nuclei in highly asymmetric electric-field gradients, the nuclear spin could therefore be initialized in the spin-Kerr-cat subspace using SU(2) rotations and measurement rather than full SU(
2I+1) control. We calculate the dephasing time of the spin Kerr-cat qubit under a model of
1/f noise, as well as relaxation of the qubit due to breaking of the
Z2 symmetry by charge-noise-induced fluctuations of the quadrupolar tensor. Using measured parameters for antimony (
123Sb) donors in silicon, we estimate that second-scale
T2∗ times could be achieved with this encoding, with bitflips and leakage occurring on significantly longer timescales. We propose a two-qubit gate acting on spin Kerr-cat qubits and electron-spin qubits, enabled by adiabatically moving an electron on and off the donor potential. Based on numerical simulations, we estimate that with an enhancement of measured quadrupolar couplings by a factor of
≈2, a gate fidelity exceeding
99% could be achieved for spin Kerr cats encoded in
123Sb, with a gate time under
100 ns. By entangling the nuclear spin with an electron spin in this way, the spin Kerr-cat qubit could then be measured using a Pauli spin blockade readout of the electron.
We propose a scheme to generate spin cat states, i.e., superpositions of maximally separated quasiclassical states on a single high-dimensional nuclear spin in a solid-state device. We exploit a strong quadrupolar nonlinearity to drive the nucleus significantly faster than usual gate sequences, achieving collapses and revivals two orders of magnitude faster than the dephasing timescale. Furthermore, these states are engineered without entanglement with an ancilla, hence, are robust against error propagation. With our multitone control, we can realize arbitrary high-spin rotations within an experimentally feasible regime, as well as transform a spin coherent state to a spin cat state using only phase modulation, opening the possibility of storing and manipulating high-fidelity cat states. Published by the American Physical Society 2024
We have produced and characterized spin-squeezed states at a temperature of 26 °C in a nuclear magnetic resonance quadrupolar system. The experiment was carried out on 133Cs nuclei of spin I=7/2 in a sample of lyotropic liquid crystal. The source of spin squeezing was identified as the interaction between the quadrupole moment of the nuclei and the electric field gradients present within the molecules. We use the spin angular momentum representation to describe formally the nonlinear operators that produce the spin squeezing on a Hilbert space of dimension 2I+1=8. The quantitative and qualitative characterization of this spin-squeezing phenomenon is expressed by a squeezing parameter and squeezing angle developed for the two-mode Bose-Einstein condensate system, as well as by the Wigner quasiprobability distribution function. The generality of the present experimental scheme points to potential applications in solid-state physics.
We study theoretically the interaction-induced generation of mesoscopic coherent spin state superpositions (small-particle-number cat states) from an initial coherent spin state in bimodal Bose-Einstein condensates and the subsequent phase revival, including decoherence due to particle losses and fluctuations of the total particle number. In a full multimode description, we propose a preparation procedure of the initial coherent spin state and we study the effect of preexisting thermal fluctuations on the phase revival, and on the spin and orbito-spinorial cat-state fidelities.