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arXiv:1608.05087 · Physical review. B./Physical review. B

Effects of strong disorder in strongly correlated superconductors

Debmalya Chakraborty, Rajdeep Sensarma, Amit Ghosal

Published Jan 23, 2017• 16 citations
arXivHTMLPDF

Abstract

We investigate the effect of strong disorder on a system with strong electronic repulsion. In the absence of disorder, the system has a d-wave superconducting ground state with strong non-BCS features due to its proximity to a Mott insulator. We find that while strong correlations make superconductivity in this system immune to weak disorder, superconductivity is destroyed efficiently when disorder strength is comparable to the effective bandwidth. The suppression of charge motion in regions of strong potential fluctuation leads to the formation of Mott insulating patches, which anchor a larger nonsuperconducting region around them. The system thus breaks into islands of Mott insulating and superconducting regions, with Anderson insulating regions occurring along the boundary of these regions. Thus, electronic correlation and disorder, when both are strong, aid each other in destroying superconductivity, in contrast to their competition at weak disorder. Our results shed light on why zinc impurities are efficient in destroying superconductivity in cuprates, even though it is robust to weaker impurities.

DOI
10.1103/physrevb.95.014516

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Journal of Physics Conference Series•Sep 1, 2019•0 citations
We investigate the effect of strong disorder on a system with strong electronic repulsion. In the absence of disorder, the system has a d-wave superconducting ground state with strong non-BCS features due to its proximity to a Mott insulator. We find that while strong correlations make superconductivity in this system immune to weak disorder, superconductivity is destroyed efficiently when disorder strength is comparable to the effective bandwidth. The suppression of charge motion in regions of strong potential fluctuation leads to the formation of Mott insulating patches, which anchor a larger nonsuperconducting region around them. The system thus breaks into islands of Mott insulating and superconducting regions, with Anderson insulating regions occurring along the boundary of these regions. Thus, electronic correlation and disorder, when both are strong, aid each other in destroying superconductivity, in contrast to their competition at weak disorder. Our results shed light on why zinc impurities are efficient in destroying superconductivity in cuprates, even though it is robust to weaker impurities.
We address the question of why strongly correlated ddd-wave superconductors, such as the cuprates, prove to be surprisingly robust against the introduction of nonmagnetic impurities. We show that, very generally, both the pair-breaking and the normal state transport scattering rates are significantly suppressed by strong correlations effects arising in the proximity to a Mott insulating state. We also show that the correlation-renormalized scattering amplitude is generically enhanced in the forward direction, an effect which was previously often ascribed to the specific scattering by charged impurities outside the copper-oxide planes.
The effects of disorder are investigated in strongly correlated electronic systems near the Mott metal-insulator transition. Correlation effects are found1 to lead to strong disorder screening, a mechanism restricted to low-lying electronic states, very similar to what is observed in underdoped cuprates. These results suggest, however, that this effect is not specific to disordered d-wave superconductors, but is a generic feature of all disordered Mott systems. In addition, the resulting spatial inhomogeneity rapidly increases2 as the Mott insulator is approached at fixed disorder strength. This behavior, which can be described as an Electronic Griffiths Phase, displays all the features expected for disorder-dominated Infinite-Randomness Fixed Point scenario of quantum criticality.
Many theoretical approaches find ddd-wave superconductivity in the prototypical one-band Hubbard model for high-temperature superconductors. At strong coupling ($U\ensuremath{\ge}W$, where UUU is the on-site repulsion and W=8tW=8tW=8t the bandwidth) pairing is controlled by the exchange energy J=4t2/UJ=4{t}^{2}/UJ=4t2/U. One may then surmise, ignoring retardation effects, that near-neighbor Coulomb repulsion VVV will destroy superconductivity when it becomes larger than JJJ, a condition that is easily satisfied in cuprates, for example. Using cellular dynamical mean-field theory with an exact diagonalization solver for the extended Hubbard model, we show that pairing at strong coupling is preserved, even when $V\ensuremath{\gg}J$, as long as $V\ensuremath{\lesssim}U/2$. While at weak coupling VVV always reduces the spin fluctuations and hence ddd-wave pairing, at strong coupling, in the underdoped regime, the increase of $J=4{t}^{2}/(U\ensuremath{-}V)$ caused by VVV increases binding at low frequency while the pair-breaking effect of VVV is pushed to high frequency. These two effects compensate in the underdoped regime, in the presence of a pseudogap. While the pseudogap competes with superconductivity, the proximity to the Mott transition that leads to the pseudogap, and retardation effects, protect ddd-wave superconductivity from VVV.
Understanding how electrons form pairs in the presence of strong electron correlations demands going beyond the BCS paradigm. We study a correlated superconducting model where the correlation effects are accounted for by a U term local in momentum space. The electron correlation is treated exactly while the electron pairing is treated approximately using the mean-field theory. The self-consistent equation for the pair potential is derived and solved. Somewhat contrary to expectation, a weak attractive U comparable to the pair potential can destroy the superconductivity, whereas for weak to intermediate repulsive U , the pair potential can be enhanced. The fidelity of the mean-field ground state is calculated to describe the strength of the elelectron correlation. We show that the pair potential is not equal to the single-electron superconducting gap for the strongly correlated superconductors, in contrast to the uncorrelated BCS limit.
Using the variational Monte Carlo method, we find that a relatively weak long-range electron-phonon interaction induces a ddd-wave superconducting state in doped Mott-Hubbard insulators and/or strongly correlated metals with a condensation energy significantly larger than can be obtained with Coulomb repulsion only. Moreover, the superconductivity is shown to exist for infinite on-site Coulomb repulsion without the need for additional mechanisms such as spin fluctuations to mediate ddd-wave superconductivity. We argue that our superconducting state is robust with respect to a more intricate choice of the trial-wave function and that a possible origin of high-temperature superconductivity lies in a proper combination of strong electron-electron correlations with poorly screened Fr\"ohlich electron-phonon interaction.
Abstract With cuprate superconductors in mind, we study the effects of point-type impurity potential (V) on a d x 2−y 2 -wave superconducting (d-SC) state in a strongly correlated squarelattice Hubbard model (U/t = 12) with a diagonal transfer (t′), using a variational Monte Carlo method. At half filling, insulator-to-conductor (filling-control-type Mott) transitions occur at <?CDATA V=VU(±)∼±UV={V}_{U}^{(\pm )}\sim \pm UV=VU(±)​∼±U?> V = V U ( ± ) ∼ ± U . The phase realized for <?CDATA V<VU(−)V\lt {V}_{U}^{(-)}V<VU(−)​?> V < V U ( − ) is robust d-SC and the charge carriers are holes, whereas for <?CDATA V>VU(+)V\gt {V}_{U}^{(+)}V>VU(+)​?> V > V U ( + ) a metallic (or weak d-SC) state appears with charge carriers of electrons. For a partially-filled case where the impurity density is equal to the doping rate, a d-SC-to-insulator transition arises at V ≡ V M ∼ 4t. In the weak-|V| phases, the impurity effects in the electron distribution are smeared out by the screening effect, whereas in the strong-|V| phases, the electron distribution directly depend on the impurity configurations.