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arXiv:1608.00137 · Physical Review A

Phase control of the quantum statistics of collective emission

Marc-Oliver Pleinert, Joachim von Zanthier, G. S. Agarwal

Published Feb 21, 2018• 22 citations
arXivHTMLPDF

Abstract

We report nonclassical aspects of the collective behavior of two atoms in a cavity by investigating the photon statistics and photon distribution over a very broad domain of parameters. Starting with the dynamics of two atoms radiating in phase into the cavity, we study the photon statistics for arbitrary interatomic phases as revealed by the second-order intensity correlation function at zero time, ${g}^{(2)}(0)$, and the Mandel $Q$ parameter. We find that the light field can be tuned from antibunched to (super-)bunched as well as nonclassical to classical behavior by merely modifying the atomic position. The highest nonclassicality in the sense of the smallest $Q$ parameter is found when spontaneous emission, cavity decay, coherent pumping, and atom-cavity coupling are of comparable magnitude. We introduce a quantum version of the negative binomial distribution with its parameters directly related to $Q$ and ${g}^{(2)}(0)$ and discuss its range of applicability. We also examine the Klyshko parameter, which highlights the nonclassicality of the photon distribution.

DOI
10.1103/physreva.97.023831

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We report nonclassical aspects of the collective behavior of two atoms in a cavity by investigating the photon statistics and photon distribution over a very broad domain of parameters. Starting with the dynamics of two atoms radiating in phase into the cavity, we study the photon statistics for arbitrary interatomic phases as revealed by the second-order intensity correlation function at zero time, g(2)(0){g}^{(2)}(0)g(2)(0), and the Mandel QQQ parameter. We find that the light field can be tuned from antibunched to (super-)bunched as well as nonclassical to classical behavior by merely modifying the atomic position. The highest nonclassicality in the sense of the smallest QQQ parameter is found when spontaneous emission, cavity decay, coherent pumping, and atom-cavity coupling are of comparable magnitude. We introduce a quantum version of the negative binomial distribution with its parameters directly related to QQQ and g(2)(0){g}^{(2)}(0)g(2)(0) and discuss its range of applicability. We also examine the Klyshko parameter, which highlights the nonclassicality of the photon distribution.
We present a study of the quantum statistical properties of light emitted by two coherently driven atoms coupled to a single-mode cavity, an ideal setup to precisely investigate various aspects of collective behavior over a wide range of couplings to cavity and external drive. At high pumping and coupling, we predict the possibility of steady-state hyperradiance accompanied by (super-)bunching for an out of phase radiation. The mean photon number can be up to 222 orders of magnitude higher than in the single atom case. The highest nonclassicality in the sense of the smallest Mandel QQQ parameter is found when spontaneous emission, cavity decay, coherent pumping, and atom-cavity coupling are comparable. A quantum version of the negative binomial distribution with parameters directly related to QQQ characterizes the photon distribution in the cavity and its quantum features.
We consider an optical cavity containing a single two-level atom driven on resonance by an external laser source.1 We focus on the limit of weak excitation where the dynamic response of this system is governed by just three parameters: the atom-field coupling constant g, spontaneous emission rate γ for the atom, and cavity decay rate κ. The statistics of the transmitted light are analyzed as a function of g, γ, and κ, in terms of the second-order correlation function g(2)(τ), and the quadrature variances measured in a homodyne detection scheme. Squeezing and photon antibunching exist over a wide range of parameters. For γ ~ κ, the system can exhibit an oscillatory response, even when the mean intracavity photon number is much less than unity.2 The oscillations can be understood in terms of the coupling between the free atom-field eigenstates |0,−>, |0,+>, and |1,−>. The oscillation frequency is determined by the energy level splitting produced between the degenerate one-quantum states |0,+> and |1,−> by the atom-field interaction. The second-order correlation function can exhibit a novel nonclassical effect, where, for g(2)(0) ≠ 0, at some finite delay τ0, the correlation function dips exactly to zero—g(2)(τ0) = 0.
We investigate the photon statistics of an ensemble of coherently driven non-interacting two-level atoms in the weak driving regime. As it turns out, the system displays unique emission characteristics that are strongly in contrast to the emission of classical oscillating dipoles. By deriving the second-order autocorrelation function, we show that extraordinary two-photon correlations are obtained, ranging from strong antibunching to superbunching. These features are enhanced by disorder in the emitter positions, and the control parameter is the number of excitations in the system. We observe the appearance of bunching and antibunching when the light is scattered by the atoms predominantly coherently, i.e., mimicking classical Rayleigh scattering, whereas thermal photon statistics is obtained when the light is scattered via spontaneous decay, a well-known quantum effect. The underlying mechanism is the interplay between coherent scattering, which exhibits spatial fluctuations due to interference, and dissipation in the form of isotropic spontaneous decay.
We consider a single two-level atom in an optical cavity, in which the system is driven by a coherent driving field. In the bad-cavity limit, when the cavity loss rate is taken to be large compared to the atomic decay rate and atom-field coupling, the cavity field can be adiabatically eliminated from the equations of motion for the atomic operators. The main effect of the cavity in this limit is the enhancement of spontaneous emission into the cavity mode. For this model, the second-order intensity correlation function g(2)() has been shown to exhibit photon antibunching, sub-Poissonian photon number distributions, and other nonclassical effects.1 In this paper, analytic results are presented for g(2)() for both the transmitted and fluorescent light fields when broadband squeezed light is injected into the cavity. Effects of the squeezing on nonclassical behavior is examined.
Superradiance, i.e., spontaneous emission of coherent radiation by an ensemble of two-level atoms in collective states introduced by Dicke in 1954, is one of the enigmatic problems of quantum optics. The startling gist is that even though the atoms have no dipole moment they radiate with increased intensity in particular directions. Following the advances in our understanding of superradiant emission by atoms in entangled W-states we examine the quantum statistical properties of superradiance. Such investigations require the system to have at least two excitations in order to explore the photon-photon correlations of the radiation emitted by such states. We present specifically results for the spatially resolved photon-photon correlations of systems prepared in doubly excited W-states and give conditions when the atomic system emits nonclassial light. Equally, we derive the conditions for the occurrence of bunching and even of superbunching, a rare phenomenon otherwise known only from nonclassical states of light like the squeezed vacuum. We finally investigate the photon-photon cross correlations of the spontaneously scattered light and highlight the nonclassicalty of such correlations. The theoretical findings can be implemented with current technology, e.g., using ions in a linear rf-trap, atoms in an optical lattice or quantum dots in a cavity.
In this thesis three different approaches to control the quantum statistics in nanoscopic devices are investigated. In the first part of the thesis, mechanical oscillations in solid state devices are manipulated by an external laser to show bistabilities, coherent amplification, and enhanced damping. The dynamics is controlled by the frequency of the external laser. This study is performed in a semiclassical approximation, where expectation values of operators are factorized. These effects are used to show the similarities and differences between optomechanical systems and phonon cavities. In the regime of coherent amplification of phonons the theoretical description is extended to a fully quantum mechanical model. This reveals additional resonances due to collective processes that can be addressed via the frequency of the external laser. In the second part, a quantum light source is considered for manipulation of the emission statistics of a second quantum optical system serving as target. A Jaynes-Cummings system is used as a source that may be tuned from nonclassical to thermal emission via the pump strength. The target consists of a cavity with two emitters. The nature of the imprinted statistics is studied by higher order correlation functions. The resulting statistics deviates strongly from thermal, coherent or antibunched statistics. The third part considers coherent self feedback with time-delay, which is motivated by classical Pyragas control. The finite time delay is used as control parameter. The matrix product state evolution in the picture of the quantum stochastic Schrödinger equation is employed as a systematic way of dealing with quantum self-feedback. In this thesis, the approach is extended to include higher order terms in the time evolution operator. This is done systematically so that arbitrary order can be included enabling faster numerical evaluation. This extension of the matrix product state evolution method allows to investigate efficiently the emission statistics of a single mode cavity containing two emitters. It is shown that feedback can enhance antibunching in the light field while also counter-intuitively increasing the number of emitted photons at the same time. Expressing the time evolution operator as a sum of sparse matrices allows to include time dependent Hamiltonians in an efficient manner. Considering the pulsed excitation of a two level emitter, it is demonstrated that emission statistics may be tuned via feedback. This allows to switch between single photon emission and enhanced two photon emission.