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arXiv:1607.03228 · Reviews of Modern Physics

Quantum spin liquid states

Yi Zhou, Kazushi Kanoda, Tai Kai Ng

Published Apr 18, 2017• 1,464 citations
arXivHTMLPDF

Abstract

The concept of a quantum spin liquid is important for problems ranging from quantum spin chains to high-temperature superconductivity. This review gives a pedagogical introduction to the theoretical concepts behind this fascinating topic, and also discusses the current experimental situation.
DOI
10.1103/revmodphys.89.025003

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Abstract In condensed matter physics there is a novel phase termed ‘quantum spin liquid’, in which strong quantum fluctuations prevent long-range magnetic order from being estab lished, and so electron spins do not form an ordered pattern but remain liquid-like even at absolute zero temperature. Such a phase is not involved in any spontaneous symmetry breaking and local order parameter, and to understand it is beyond conventional phase transition theory. Due to the rich physics and exotic properties of quantum spin liquids, such as long-range entanglement and fractional quantum excitations, which are believed to hold great potential for quantum communication and computation, they have been intensively studied since the concept was proposed in 1973 by P.W. Anderson. Currently, experimental identification of a quantum spin liquid remains a great challenge. Here, we highlight some interesting experimental progress that has been made recently. We also discuss outstanding issues and raise questions that we consider to be important for future research.
Quantum spin liquids may be considered 'quantum disordered' ground states of spin systems, in which zero-point fluctuations are so strong that they prevent conventional magnetic long-range order. More interestingly, quantum spin liquids are prototypical examples of ground states with massive many-body entanglement, which is of a degree sufficient to render these states distinct phases of matter. Their highly entangled nature imbues quantum spin liquids with unique physical aspects, such as non-local excitations, topological properties, and more. In this review, we discuss the nature of such phases and their properties based on paradigmatic models and general arguments, and introduce theoretical technology such as gauge theory and partons, which are conveniently used in the study of quantum spin liquids. An overview is given of the different types of quantum spin liquids and the models and theories used to describe them. We also provide a guide to the current status of experiments in relation to study quantum spin liquids, and to the diverse probes used therein.
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Frustration in spin systems can prevent ordering even at T=0T=0T=0, creating quantum spin liquids that have been sought since Anderson's pioneering work in 1973 and his influential 1987 paper connecting them to high-temperature superconductivity. Kitaev's solvable spin-1/2 models on a honeycomb lattice brought renewed attention to this field, with Jackeli and Khaliullin later revealing how to engineer Kitaev interactions in real materials. This review highlights theoretical and experimental developments in Kitaev spin liquids, emphasizing leading candidate materials and their broad topological properties such as chiral edge modes. Consequently, it provides essential insights for both experimentalists and theorists working on quantum spin liquid problems.
This paper presents an overview of the properties of magnetic insulators, with emphasis on quantum effects. In particular, the consequences of strong quantum fluctuations on the low-energy properties of a number of systems are reviewed: the occurrence of a spin gap in spin-1 chains and other low-dimensional magnets; the presence of low-lying singlet excitations in several frustrated magnets; the interplay of orbital and spin fluctuations in orbitally degenerate Mott insulators. This review is intended as a pedagogical introduction to the field, and the formalism has been kept at a minimal level.
In this brief overview, I address some of the fundamental topics related to the physics of strongly correlated fermions, which have been also the subject of my research. After addressing the question why the field has a fundamental meaning, we next turn to the specific problems with their simple theoretical description. Those topics are: (i) the concept of spindependent masses of heavy particles and its subsequent experimental verification; (ii) the correlated metal–insulator transitions of the Mott–Hubbardtype; (iii) real space pairing and its subsequent experimental verification for high-temperature superconducting cuprates. I mention also the persistence of quantum spin and charge excitations in the superconducting phase. All those phenomena confirm the view that the strongly correlated fermionic \nsystems represent a new class of quantum liquids, with some properties quantitatively different than those of the Landau Fermi liquids. Namely, they can be classified as those that fall in between those of the anomalous Landau Fermi liquid and localized-magnetic-moment system.