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arXiv:1607.00922 · Proceedings of the National Academy of Sciences

Quantum entanglement of angular momentum states with quantum numbers up to 10,010

Robert Fickler, Geoff Campbell, B. C. Buchler, Ping Koy Lam, Anton Zeilinger

Published Nov 15, 2016• 276 citations
arXivHTMLPDF

Abstract

Photons with a twisted phase front carry a quantized amount of orbital angular momentum (OAM) and have become important in various fields of optics, such as quantum and classical information science or optical tweezers. Because no upper limit on the OAM content per photon is known, they are also interesting systems to experimentally challenge quantum mechanical prediction for high quantum numbers. Here, we take advantage of a recently developed technique to imprint unprecedented high values of OAM, namely spiral phase mirrors, to generate photons with more than 10,000 quanta of OAM. Moreover, we demonstrate quantum entanglement between these large OAM quanta of one photon and the polarization of its partner photon. To our knowledge, this corresponds to entanglement with the largest quantum number that has been demonstrated in an experiment. The results may also open novel ways to couple single photons to massive objects, enhance angular resolution, and highlight OAM as a promising way to increase the information capacity of a single photon.

DOI
10.1073/pnas.1616889113

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Orbital angular momentum (OAM) of single photons represents a new optical degree of freedom for the entanglement of photons [1,2]. One physical realization of OAM carrying light beams are the so called Laguerre-Gaussian modes of light with the required helical phase structure. One big advantage over the well known polarization degree of freedom is the possibility of realizing entanglement between two photons with very high quantum numbers. However, the creation of photonic OAM entanglement using the widely used spontaneous parametric downconversion process is limited by the strongly reduced efficiency for higher momenta [3]. We have realized a novel method to create entanglement between two photons with a very high difference in their OAM quantum number and momentum respectively. Furthermore we have explored hybrid entanglement of photons in the OAM and polarization degree of freedom.

Frontiers in Optics•Jan 1, 2011•1 citation
Photons with a twisted phase front carry a quantized amount of orbital angular momentum (OAM) and have become important in various fields of optics, such as quantum and classical information science or optical tweezers. Because no upper limit on the OAM content per photon is known, they are also interesting systems to experimentally challenge quantum mechanical prediction for high quantum numbers. Here, we take advantage of a recently developed technique to imprint unprecedented high values of OAM, namely spiral phase mirrors, to generate photons with more than 10,000 quanta of OAM. Moreover, we demonstrate quantum entanglement between these large OAM quanta of one photon and the polarization of its partner photon. To our knowledge, this corresponds to entanglement with the largest quantum number that has been demonstrated in an experiment. The results may also open novel ways to couple single photons to massive objects, enhance angular resolution, and highlight OAM as a promising way to increase the information capacity of a single photon.
Single photons with helical phase structures may carry a quantized amount of orbital angular momentum (OAM), and their entanglement is important for quantum information science and fundamental tests of quantum theory. Because there is no theoretical upper limit on how many quanta of OAM a single photon can carry, it is possible to create entanglement between two particles with an arbitrarily high difference in quantum number. By transferring polarization entanglement to OAM with an interferometric scheme, we generate and verify entanglement between two photons differing by 600 in quantum number. The only restrictive factors toward higher numbers are current technical limitations. We also experimentally demonstrate that the entanglement of very high OAM can improve the sensitivity of angular resolution in remote sensing.
Photons are an ideal candidate for encoding both classical and quantum information. Besides spin angular momentum associated with circular polarization, single photon can also carry other fundamentally new degree of freedom of orbital angular momentum related to the spiral phase structure of light. The key significance of orbital angular momentum lies in its potential in realizing a high-dimensional Hilbert space and in encoding a high-dimensional quantum information. Since Allen et al. [Allen L, Beijersbergen M W, Spreeuw R J C, Woerdman J P 1992 Phys. Rev. A 45 8185] recognized the physical reality of photon orbital angular momentum in 1992, rapidly growing interest has been aroused in orbital angular momentum (OAM) from both classical and quantum points of view. Here we present an overall review on the high-order orbital angular momentum of photon, including its preparation and manipulation based on some specific techniques and also its applications. The spatial light modulator is a commercial device that has been widely employed to generate the OAM beams. We make and identify the optical OAM superposition with very high quantum numbers up to l=360. Recently, the metallic spiral phase mirrors were also developed to produce high-order OAM beams up to l=5050. In addition, the Q-plates made of anisotropic and inhomogeneous liquid crystals were invented to generate high-order OAM beams in a polarization-controllable manner, and the OAM superposition of l=± 50 were achieved. Owing to high rotational symmetry, these high OAM beams have been found to have more and more important applications in the fields of high-sensitivity sensing and high-precision measurements. Two fascinating examples are discussed in detail. The first example is that the research group led by Prof. Zeilinger has prepared and observed the quantum entanglement of high orbital angular momenta up to l=±300 by the technique of polarization-OAM entanglement swapping, and they demonstrated that the angular resolution could be significantly improved by a factor of l. Their result was the first step for entangling and twisting even macroscopic, spatially separated objects in two different directions. The second example is that the research group led by Prof. Padgett has demonstrated an elegant experiment of rotational Doppler effects for visible light with l=±20 OAM superposition. They showed that a spinning object with an optically rough surface might induce a Doppler effect in light reflected from the direction parallel to the rotation axis, and the frequency shift was proportional to both the disk's angular speed and the optical OAM. The potential applications in noncontact measurement of angular speed and in significant improvement of angular resolution for remote sensing will be particularly fascinating.
Introduction In this chapter, we will be concerned with entangled states of light. Historically, quantum states of light, i.e., photons, have played a dominant role in the experimental study of quantum entanglement. For instance, the first Bell tests and the first realizations of quantum teleportation were performed using two-dimensional polarization-entangled twophoton states [3]. From an experimental point of view these states are readily prepared and manipulated using conventional polarization optics. Recently, however, both theoretical and experimental efforts have shifted towards entanglement in more than two modes , which is often referred to as high-dimensional entanglement. This is much richer than two-dimensional entanglement, as is, for instance, reflected in stronger violations of various measures of nonlocality which reveal the complexity of high-dimensional Hilbert spaces [4–7]. Also, from an applications perspective, it promises a larger channel capacity [8, 9] and improved security for quantum communication [10, 11]. There are several ways to implement high-dimensional two-photon entanglement. One can exploit the temporal [12], frequency [13], or spatial [14–18] degrees of freedom of the optical field. A promising way to implement high-dimensional two-photon entanglement is to use the orbital-angular-momentum (OAM) degree of freedom of light. Light beams that carry OAM have a helical wavefront that spirals around the optical axis during propagation [19]. The winding number m , which characterizes the OAM eigenmodes, can adopt any integer value between −∞ and ∞; since all coaxial OAM modes are orthogonal they can thus span a very high-dimensional Hilbert space.
Introduction Although the orbital angular momentum (OAM) of light is often quantified in terms of ℓℏ per photon, one should recognise that this result can be derived directly from Maxwell's equations and is most certainly not an exclusively quantum property. Following the recognition of optical OAM in 1992 [1], the immediate thrust of experimental work was to observe OAM transfer to microscopic objects. These exciting experiments by Rubinsztein- Dunlop [2, 3] and others established that the predicted angular momentum was truly mechanical, but did not provide insight on OAM at the level of single photons. Laguerre- Gaussian modes were identified as being a natural basis set for describing beams with OAM, where their phase terms describe the helical phasefronts corresponding to an OAM of ℓℏ per photon. The polarisation of light has played an important historical role in the experimental investigation of quantum entanglement, quantum gate operations and quantum cryptography. A potential advantage of OAM is that it resides in a higher-dimensional state space which, as follows from the theory, is infinite-dimensional. One of the experimental challenges is to access a large number of these dimensions. In quantum communication, the most obvious advantage of high n -dimensional systems is the increased bandwidth [4], but qunits also lead to stronger security [5, 6]. An increase in the number of entangled quantum modes has also been shown to improve measures of nonlocality [7], to allow quantum computation with better fault tolerance [8] and to simplify quantum logic structures [9].
Abstract The complex interactions between orbital angular momentum (OAM) of light and atoms are particularly intriguing in the areas of quantum optics and quantum information. Building a versatile high-dimensional quantum network needs broad spiral-bandwidth for preparing higher-quanta OAM mode and resolving the bandwidth mismatch in spatial space. Here, we demonstrate a broad spiral-bandwidth quantum-interface between photon and memory. Through twisted fields of the writing and reading, the correlated OAM distribution between photon and memory is significantly broadened. This broad spiral-bandwidth quantum-interface could be spanned in multiplexing regime and could work in high-quanta scenario with capability of ∣l∣=\vert l\vert =∣l∣= ∣ l ∣ = 30, and we demonstrate the entanglement within 2-D subspace with a fidelity of 80.5 ± 4.8% for high lll l . Such state-of-the-art technology to freely control the spatial distribution of OAM memory is very helpful to construct high-dimensional quantum networks and provides a benchmark in the field of actively developing methods to engineer OAM single photon from matters.
Orbital angular momentum (OAM) of single photons represents a new optical degree of freedom for the entanglement of photons [1,2]. One physical realization of OAM carrying light beams are the so called Laguerre-Gaussian modes of light with the required helical phase structure. One big advantage over the well known polarization degree of freedom is the possibility of realizing entanglement between two photons with very high quantum numbers. However, the creation of photonic OAM entanglement using the widely used spontaneous parametric downconversion process is limited by the strongly reduced efficiency for higher momenta [3]. We have realized a novel method to create entanglement between two photons with a very high difference in their OAM quantum number and momentum respectively. Furthermore we have explored hybrid entanglement of photons in the OAM and polarization degree of freedom.