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arXiv:1606.08580 · Scientific Reports

Many-body Tunneling and Nonequilibrium Dynamics of Doublons in Strongly Correlated Quantum Dots

Wenjie Hou, Yuandong Wang, Jianhua Wei, Zhen‐Gang Zhu, YiJing Yan

Published May 23, 2017• 12 citations
arXivHTMLPDF

Abstract

Abstract Quantum tunneling dominates coherent transport at low temperatures in many systems of great interest. In this work we report a many–body tunneling (MBT), by nonperturbatively solving the Anderson multi-impurity model, and identify it a fundamental tunneling process on top of the well–acknowledged sequential tunneling and cotunneling. We show that the MBT involves the dynamics of doublons in strongly correlated systems. Proportional to the numbers of dynamical doublons, the MBT can dominate the off–resonant transport in the strongly correlated regime. A T3/2–dependence of the MBT current on temperature is uncovered and can be identified as a fingerprint of the MBT in experiments. We also prove that the MBT can support the coherent long–range tunneling of doublons, which is well consistent with recent experiments on ultracold atoms. As a fundamental physical process, the MBT is expected to play important roles in general quantum systems.

DOI
10.1038/s41598-017-02728-7

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Abstract Quantum tunneling dominates coherent transport at low temperatures in many systems of great interest. In this work we report a many–body tunneling (MBT), by nonperturbatively solving the Anderson multi-impurity model, and identify it a fundamental tunneling process on top of the well–acknowledged sequential tunneling and cotunneling. We show that the MBT involves the dynamics of doublons in strongly correlated systems. Proportional to the numbers of dynamical doublons, the MBT can dominate the off–resonant transport in the strongly correlated regime. A T3/2–dependence of the MBT current on temperature is uncovered and can be identified as a fingerprint of the MBT in experiments. We also prove that the MBT can support the coherent long–range tunneling of doublons, which is well consistent with recent experiments on ultracold atoms. As a fundamental physical process, the MBT is expected to play important roles in general quantum systems.
Quantum tunneling is fundamental to diverse phenomena and underpins a wide range of modern technologies. In the study of superconducting quantum computation and high-temperature superconducting materials, tunneling on multi-particle scale is central. Recently, several cold atom experiments successfully simulated the tunneling process in a many-particle ensemble. However, the many-body nature remains largely unexplored. Here, we observe the universal scaling of many-body effects in quantum tunneling process, using a hexagonal-triangular quantum simulator with independent control of barrier, temperature and interaction. In the weak-interaction regime, the critical tunneling coefficient scales parabolically with temperature under various conditions, in contrast to the linear scaling of single-particle tunneling. By further increasing the interactions beyond the mean-field regime, the scaling exponent decreases, consistent with quantum field theory predictions. Our results address the fundamental question of how many-body effects renormalize quantum tunneling, with direct implications for correlated quantum matter and devices.
Quantum tunneling is at the heart of many low-temperature phenomena. In strongly correlated lattice systems, tunneling is responsible for inducing effective interactions, and long-range tunneling substantially alters many-body properties in and out of equilibrium. We observe resonantly enhanced long-range quantum tunneling in one-dimensional Mott-insulating Hubbard chains that are suddenly quenched into a tilted configuration. Higher-order tunneling processes over up to five lattice sites are observed as resonances in the number of doubly occupied sites when the tilt per site is tuned to integer fractions of the Mott gap. This forms a basis for a controlled study of many-body dynamics driven by higher-order tunneling and demonstrates that when some degrees of freedom are frozen out, phenomena that are driven by small-amplitude tunneling terms can still be observed.
This thesis contributes to the field of transport through quantum dots. These devices allow for a controlled study of quantum transport and fundamental physical effects, like the Kondo effect. In this thesis we will focus on dots that are well described by generalized Anderson impurity models, where the discrete levels of the quantum dot are tunnel-coupled to fermionic reservoirs. The model parameters, like level energy and width, can be tuned in experiments. Therefore these systems constitute a valuable arena for testing experiment against theory and vice versa. In order to describe these strongly correlated systems, we employ the numerical renormalization group method. This allows us to address both longstanding questions concerning experimental results and new physical phenomena in these fundamental models. This thesis consists of three major projects. The first and most extensive one is concerned with the phase of the transmission amplitude through a quantum dot. Measurements of many-electron quantum dots with small level spacing reveal universal phase behaviour, a result not fully understood for almost 10 years. Recent experiments have seen that, contrarily, for dots with only a few electrons, i.e. large level spacing, the phase depends on the mesoscopic dot parameters. Analyzing a multi-level Anderson model, we show that the generic feature of the two regimes can be reproduced in the regime of overlapping levels or well separated levels, respectively. Thereby the universal character follows from Fano-type antiresonances of the renormalized single-particle levels. Moderate temperature supports the universal character. In the mesoscopic regime, we also investigate the effect of Kondo correlations on the transmission phase. In a second project we analyze a quantum dot coupled to a superconducting reservoir. In contrast to previous belief, the energy resolution of our method is not restricted by the energy scale of the superconducting gap, leading to new insights into the method. The high resolution allows us to resolve sharp peaks in the spectral function that emerge for a certain regime of parameters. A third project deals with a quantum dot coupled to two independent channels, a system known to exhibit non-Fermi liquid behaviour. We investigate the existence of the non-Fermi liquid regime when driving the system out of the Kondo regime by emptying the dot. We find that the extent of the non-Fermi liquid regime strongly depends on the mechanisms that couple impurity and reservoirs but prevent mixing of the latter.
The out-of-equilibrium transport properties of a double quantum dot system in the Kondo regime are studied theoretically by means of a two-impurity Anderson Hamiltonian with interimpurity hopping. The Hamiltonian is solved by means of a nonequilibrium generalization of the slave-boson mean-field theory. It is demonstrated that measurements of the differential conductance dI/dV, for appropriate values of voltages and tunneling couplings, can give a direct observation of the coherent superposition between the many-body Kondo states of each dot. For large voltages and arbitrarily large interdot tunneling, there is a critical voltage above which the physical behavior of the system again resembles that of two decoupled quantum dots.
The creation of tunable open quantum systems is becoming feasible in current experiments with ultracold atoms in low-dimensional traps. In particular, the high degree of experimental control over these systems allows detailed studies of tunneling dynamics, e.g., as a function of the trapping geometry and the interparticle interaction strength. In order to address this exciting opportunity we present a theoretical framework for two-body tunneling based on the rigged Hilbert space formulation. In this approach, bound, resonant, and scattering states are included on an equal footing and we argue that the coupling of all these components is vital for a correct description of the relevant threshold phenomena. In particular, we study the tunneling mechanism for two-body systems in one-dimensional traps and different interaction regimes. We find a strong dominance of sequential tunneling of single particles for repulsive and weakly attractive systems, while there is a signature of correlated pair tunneling in the calculated many-particle flux for strongly attractive interparticle interaction.