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arXiv:1606.05149

Resonance interaction of two dipoles in optically active surroundings

Qi-Zhang Yuan, Chun-Hua Yuan, Weiping Zhang

Published Jun 16, 2016• 0 citations
arXivHTMLPDF

Abstract

We study the resonance interaction between two quantum electric dipoles immersed in optically active surroundings. Quantum electrodynamics is employed to deal with dipole-vacuum interaction. Our results show that the optical activity of surroundings will not change the single atom behaviors while it can change the collective behaviors of the two dipoles, as well as greatly affect the dipole-dipole resonance interaction. Especially, if the orientations of two dipoles are orthogonal and respectively perpendicular to the interdipole axis, the interdipole resonance interaction can be established with the help of optically active surroundings while there is no resonance interaction in vacuum.

DOI
10.48550/arxiv.1606.05149

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We study the resonance interaction between two quantum electric dipoles immersed in optically active surroundings. Quantum electrodynamics is employed to deal with dipole-vacuum interaction. Our results show that the optical activity of surroundings will not change the single atom behaviors while it can change the collective behaviors of the two dipoles, as well as greatly affect the dipole-dipole resonance interaction. Especially, if the orientations of two dipoles are orthogonal and respectively perpendicular to the interdipole axis, the interdipole resonance interaction can be established with the help of optically active surroundings while there is no resonance interaction in vacuum.
We investigate the resonance dipole-dipole interaction energy between two identical atoms, one in the ground state and the other in the excited state, interacting with the electromagnetic field in the presence of a perfectly reflecting plane boundary. The atoms are prepared in a correlated (symmetric or antisymmetric) Bell-type state. Following a procedure due to Dalibard et al. [J. Dalibard et al., J. Phys. (Paris) 43, 1617 (1982); J. Phys. (Paris) 45, 637 (1984)], we separate the contributions of vacuum fluctuations and radiation reaction (source) field to the resonance interaction energy between the two atoms and show that only the source field contributes to the interatomic interaction, while vacuum field fluctuations do not. By considering specific geometric configurations of the two-atom system with respect to the mirror and specific choices of dipole orientations, we show that the presence of the mirror significantly affects the resonance interaction energy and that different features appear with respect to the case of atoms in free space, for example, a change in the spatial dependence of the interaction. Our findings also suggest that the presence of a boundary can be exploited to tailor and control the resonance interaction between two atoms, as well as the related energy transfer process. The possibility of observing these phenomena is also discussed.
Within the framework of quantization of the macroscopic electromagnetic field, equations of motion and an effective Hamiltonian for treating both the resonant dipole-dipole interaction between two-level atoms and the resonant atom-field interaction are derived, which can suitably be used for studying the influence of arbitrary dispersing and absorbing material surroundings on these interactions. The theory is applied to the study of the transient behavior of two atoms that initially share a single excitation, with special emphasis on the role of the two competing processes of virtual- and real-photon exchange in the energy transfer between the atoms. In particular, it is shown that for weak atom-field interaction there is a time window, where the energy transfer follows a rate regime of the type obtained by ordinary second-order perturbation theory. Finally, it is shown that the resonant dipole-dipole interaction can change the singlet line of the emitted light to a doublet spectrum for weak atom-field interaction and the doublet spectrum to a triplet spectrum for strong atom-field interaction.
At the most fundamental level of quantum electrodynamics, there is no such thing as two-body interactions between atoms. The potentials that describe these interactions are effective potentials resulting from a series of approximations whose validity depends on the precise situation at hand. Considering a one-dimensional geometry for simplicity, we discuss under which conditions the familiar form of the near-resonant dipole-dipole interaction is valid, paying particular attention to the effects of interatomic propagation of light, and to what extent it can be modified in the tailored electromagnetic environments provided by optical resonators. We find that once the atoms have established that they are inside a resonator, the dipole-dipole potential may or may not remain a useful concept, depending upon the strength of the atom-field interaction. In the weak-coupling regime, one finds a two-body dipole-dipole interaction that can be enhanced or inhibited by varying the atom-field detuning. In the strong-coupling regime, by contrast, the two-body dipole-dipole potential ceases to be meaningful.
The resonance fluorescence emitted by a system of two dipole-dipole interacting nearby four-level atoms in a $J=1/2\ensuremath{\leftrightarrow}J=1/2$ configuration is studied. This setup is the simplest realistic model system which provides a complete description of the (inter-atomic) dipole-dipole interaction for arbitrary orientation of the inter-atomic distance vector, and at the same time allows for intra-atomic spontaneously generated coherences. Our main interest is the interplay of both these different coupling mechanisms. We discuss different methods to analyze the contribution of the various vacuum-induced coupling constants to the total resonance fluorescence spectrum. These allow us to find a dressed state interpretation of the contribution of the different inter-atomic dipole-dipole couplings to the total spectrum. We further study the role of the spontaneously generated coherences, and identify two different contributions to the single-particle vacuum-induced couplings. We show that they have a noticeable impact on the total resonance fluorescence spectrum down to small inter-atomic distances, even though the dipole-dipole coupling constants then are much larger in magnitude than the the single-particle coupling constants. Interestingly, we find that the inter-atomic couplings can induce an effect of the intra-atomic spontaneously generated coherences on the observed spectra which is not present in single-atom systems.
Abstract We study the dispersion interaction between two ground-state two-level atoms near a cylindrical vacuum-clad optical waveguide. We focus on the case where the electric-dipole matrix-element vectors of the atoms are perpendicular to each other and to the interatomic axis. When these atoms are in free space, the dispersion interaction between them vanishes. In the presence of a waveguide aligned parallel to the interatomic axis, the energy of the dispersion interaction between the atoms may become nonzero and comparable to the average energy of the dispersion interaction between two atoms with arbitrarily oriented dipoles in free space. This waveguide-induced dispersion interaction is a consequence of the anisotropy of the medium around the atoms.
This paper researches the nonlinear cooperative transfer of atomic energy in the vacuum field of the cavity. Many scientists are concerned about a more detailed study of the cooperation interactions between different subsystems of quantum processes. Based on the theory of resonant interaction with two photons, between two active dipole atoms and a forbidden dipole in resonance with two photons, the author examines for the first time the resonance effect in two ways of the cavity. In some situations, the so-called quantum inseparability needs a new redefinition in order to describe the process that occurs between the photons belonging to these two modes of the cavity. In such a situation, it is better to study the quantum properties of collective modes arising from nonlinear interactions between traditional modes of the electromagnetic field cavity.