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arXiv:1606.02397 · Physical Review A

Nonequilibrium transient dynamics of photon statistics

Md. Manirul Ali, Wei-Min Zhang

Published Mar 23, 2017• 17 citations
arXivHTMLPDF

Abstract

We investigate the transient dynamics of photon statistics through two-time correlation functions for optical field coupled to a non-Markovian environment, described by the Fano-type Hamiltonian. We exactly solve the time-evolution of an initially nonclassical state which exhibits photon antibunching. We find that the transient correlations at different times $t$ yield a smooth transition from antibunching to bunching photon statistics in the weak system-environment coupling regime. In the strong-coupling regime, the two-time correlations exhibit oscillations that persists both in the transient process and in the steady-state limit. The oscillatory behavior of photon statistics is a manifestation of strong non-Markovian memory dynamics where the system remains in nonequilibrium from its environment. We also find that the antibunching-to-bunching transition in the weak-coupling regime and the photon statistical oscillations in the strong-coupling regime are strongly influenced by the environment temperature.

DOI
10.1103/physreva.95.033830

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We investigate the transient dynamics of photon statistics through two-time correlation functions for optical field coupled to a non-Markovian environment, described by the Fano-type Hamiltonian. We exactly solve the time-evolution of an initially nonclassical state which exhibits photon antibunching. We find that the transient correlations at different times ttt yield a smooth transition from antibunching to bunching photon statistics in the weak system-environment coupling regime. In the strong-coupling regime, the two-time correlations exhibit oscillations that persists both in the transient process and in the steady-state limit. The oscillatory behavior of photon statistics is a manifestation of strong non-Markovian memory dynamics where the system remains in nonequilibrium from its environment. We also find that the antibunching-to-bunching transition in the weak-coupling regime and the photon statistical oscillations in the strong-coupling regime are strongly influenced by the environment temperature.
By considering single chromophore systems whose radiative decay can be written in terms of a nonlocal Lindblad-type evolution, the authors extend the formalism of generalized optical Bloch equations [Y. Zheng and F. L. H. Brown, Phys. Rev. Lett. 90, 238305 (2003)] to non-Markovian dynamics. They demonstrate that photon statistical properties such as bunching and antibunching, as well as sub- and super-Poissonian photon statistics can be fitted in the context of non-Markovian dynamics. The nonlocal effects may arise due to the interaction with a complex structured environment. In this case, the photon statistics can be related with the parameters that define the microscopic system-environment interaction. Alternatively, the authors demonstrate that effective dynamics such as triplet blinking, where the system is coupled via incoherent transitions to an extra dark state, can also be worked out in terms of generalized non-Markovian optical Bloch equations. The corresponding memory contributions are mapped with those that arise from the microscopic approach.
The transient dynamics of quantum coherence of Gaussian states are investigated. The state is coupled to an external environment which can be described by a Fano-Anderson type Hamiltonian. Solving the quantum Langevin equation, we obtain the Greens functions which are used to compute the time evolved first and second moments of the quadrature operators. From the quadrature operator moments, we construct the covariance matrix which is used to measure the coherence in the system. The coherence is measured using the relative entropy of coherence measure. We consider three different classes of spectral densities in our analysis viz, the Ohmic, the sub-Ohmic, and the super-Ohmic densities. In our work, we study the dynamics of the coherent state, squeezed state, and displaced squeezed state. For all these states we observe that when the coupling with the system and the environment is weak, the coherence monotonically decreases and eventually vanishes in a long time. Thus all the states exhibit Markovian evolution in the weak coupling limit. In the strong coupling limit, the dynamics for the initial period is Markovian and after a certain period, it becomes non-Markovian where we observe an environmental backaction on the system. Thus in the strong coupling limit, we observe a dynamical crossover from Markovian nature to non-Markovian behavior. This crossover is very abrupt under some environmental conditions and for some parameters of the quantum state. Using a quantum master equation approach we verify the crossover from the dynamics of the dissipation and fluctuation parameters and the results endorse those obtained from coherence dynamics.
Nonequilibrium transport properties of quantum systems have recently become experimentally accessible in a number of platforms in so-called full-counting experiments that measure transient and steady-state nonequilibrium transport dynamics. We show that the effect of the measurement back-action can be exploited to establish general relationships between transport coefficients in the transient regime which take the form of fluctuation-dissipation theorems in the steady state. This result becomes most conspicuous in the transient dynamics of open quantum systems under strong-coupling to non-Markovian environments in nonequilibrium settings. In order to explore this regime, a new simulation method based in a hierarchy of equations of motion has been developed. We instantiate our proposal with the study of energetic conductance between two baths connected via a few level system.
Abstract Nonclassical two-photon statistics and photon squeezing are considered as representative features of the nonclassicality of light. In this work we investigate two-photon correlation function and quadrature photon squeezing in the dissipative mixed quantum Rabi model (QRM), which includes both the one-photon and two-photon qubit–resonator interactions. The quantum dressed master equation combined with squeezed-coherent states is applied to obtain the steady state. Based on the zero-time delay two-photon correlation function, it is found that with the increase of the two-photon qubit–resonator interaction strength the photon antibunching behavior is monotonically suppressed, whereas the photon bunching signature persists. One additional giant photon bunching feature is unraveled at deep-strong two-photon coupling, which mainly stems from efficient successive transition trajectories. The finite-time delay two-photon correlation function asymptotically approaches the unit by raising the delayed time. Moreover, the steady-state quadrature photon squeezing becomes significant at strong two-photon coupling, which may become perfect in the zero temperature limit.
Abstract The nonclassical feature of photons in the open finite-size Dicke model is investigated via the two-photon correlation function. The quantum dressed master equation combined with the extended coherent photonic states is applied to analyze the dissipative dynamics of both the photons and qubits. The antibunching to bunching transition of photons is clearly observed by tuning the qubit–photon coupling strength. The optimal qubit number is unraveled to enhance the two-photon correlation function. Moreover, the temperature bias of thermal baths induces significant two-photon bunching signature with deep strong qubit–photon interaction.