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arXiv:1606.00452 · Physical review. B./Physical review. B

Quantum dynamical field theory for nonequilibrium phase transitions in driven open systems

Jamir Marino, Sebastian Diehl

Published Aug 30, 2016• 59 citations
arXivHTMLPDF

Abstract

Driven-dissipative quantum many-body systems, i.e., many-particle systems where quantum coherent dynamics and dissipative effects occur on the same footing, can constitute a promising platform to initiate a systematic classification of quantum dynamical criticality. In this work, the authors show that both nonequilibrium and quantum features can be simultaneously present and persist in the low-frequency properties of a critical one-dimensional driven open Bose gas, and no effective equilibrium description is applicable for this novel type of nonequilibrium quantum criticality.

DOI
10.1103/physrevb.94.085150

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Driven-dissipative quantum many-body systems, i.e., many-particle systems where quantum coherent dynamics and dissipative effects occur on the same footing, can constitute a promising platform to initiate a systematic classification of quantum dynamical criticality. In this work, the authors show that both nonequilibrium and quantum features can be simultaneously present and persist in the low-frequency properties of a critical one-dimensional driven open Bose gas, and no effective equilibrium description is applicable for this novel type of nonequilibrium quantum criticality.
We present a comprehensive analysis of critical behavior in the driven-dissipative Bose condensation transition in three spatial dimensions. The starting point is a microscopic description of the system in terms of a many-body quantum master equation, where coherent and driven-dissipative dynamics occur on an equal footing. An equivalent Keldysh real-time functional integral reformulation opens up the problem to a practical evaluation using the tools of quantum field theory. In particular, we develop a functional renormalization group approach to quantitatively explore the universality class of this stationary nonequilibrium system. Key results comprise the emergence of an asymptotic thermalization of the distribution function, while manifest nonequilibrium properties are witnessed in the response properties in terms of a new, independent critical exponent. Thus, the driven-dissipative microscopic nature is seen to bear observable consequences on the largest length scales. The absence of two symmetries present in closed equilibrium systems---underlying particle number conservation and detailed balance, respectively---is identified as the root of this new nonequilibrium critical behavior. Our results are relevant for broad ranges of open quantum systems on the interface of quantum optics and many-body physics, from exciton-polariton condensates to cold atomic gases.
We explore the nature of the Bose condensation transition in driven open quantum systems, such as exciton-polariton condensates. Using a functional renormalization group approach formulated in the Keldysh framework, we characterize the dynamical critical behavior that governs decoherence and an effective thermalization of the low frequency dynamics. We identify a critical exponent special to the driven system, showing that it defines a new dynamical universality class. Hence critical points in driven systems lie beyond the standard classification of equilibrium dynamical phase transitions. We show how the new critical exponent can be probed in experiments with driven cold atomic systems and exciton-polariton condensates.
We identify a new universality class in one-dimensional driven open quantum systems with a dark state. Salient features are the persistence of both the microscopic nonequilibrium conditions as well as the quantum coherence of dynamics close to criticality. This provides a nonequilibrium analogue of quantum criticality, and is sharply distinct from more generic driven systems, where both effective thermalization as well as asymptotic decoherence ensue, paralleling classical dynamical criticality. We quantify universality by computing the full set of independent critical exponents within a functional renormalization group approach.
Due to the variety of tools available to control atomic, molecular, and optical (AMO) systems, they provide a versatile platform for studying many-body physics, quantum simulation, and quantum computation. Although extensive efforts are employed to reduce coupling between the system and the environment, the effects of the environment can never fully be avoided, so it is important to develop a comprehensive understanding of open quantum systems. The system-environment coupling often leads to loss via dissipation, which can be countered by a coherent drive. Open quantum systems subject to dissipation and drive are known as driven-dissipative systems, and they provide an excellent platform for studying many-body nonequilibrium physics. The first part of this dissertation will focus on driven-dissipative phase transitions. Despite the nonequilibrium nature of these systems, the corresponding phase transitions tend to exhibit emergent equilibrium behavior. However, we will show that in the vicinity of a multicritical point where multiple phase transitions intersect, genuinely nonequilibrium criticality can emerge, even though the individual phase transitions on their own exhibit equilibrium criticality. These nonequilibrium multicritical points can exhibit a variety of exotic phenomena not possible for their equilibrium counterparts, including the emergence of complex critical exponents, which lead to discrete scale invariance and spiraling phase boundaries. Furthermore, the Liouvillian gap can take on complex values, and the fluctuation-dissipation theorem is violated, corresponding to an effective temperature which gets "hotter" and "hotter" at longer and longer wavelengths. The second part of this dissertation will focus on Rydberg atoms. In particular, we study how the spontaneous generation of contaminant Rydberg states drastically modifies the behavior of a driven-dissipative Rydberg system due to the resultant dipole-dipole interactions. These interactions lead to a complicated competition of both blockade and anti-blockade effects, leading to strongly enhanced Rydberg populations for far-detuned drive and reduced Rydberg populations for resonant drive.
A deeper theoretical understanding of driven-dissipative interacting systems and their nonequilibrium phase transitions is essential both to advance our fundamental physics understanding and to harness technological opportunities arising from optically controlled quantum many-body states. This paper provides a numerical study of dynamical phases and the transitions between them in the nonequilibrium steady state of the prototypical two-dimensional Heisenberg antiferromagnet with drive and dissipation. We demonstrate a nonthermal transition that is characterized by a qualitative change in the magnon distribution from subthermal at low drive to a generalized Bose-Einstein form including a nonvanishing condensate fraction at high drive. A finite-size analysis reveals static and dynamical critical scaling at the transition, with a discontinuous slope of the magnon number versus driving field strength and critical slowing down at the transition point. Implications for experiments on quantum materials and polariton condensates are discussed.