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arXiv:1605.09014 · Physical review. B./Physical review. B

Heisenberg necklace model in a magnetic field

Alexei M. Tsvelik, Igor A. Zaliznyak

Published Aug 26, 2016• 8 citations
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Abstract

We study the low-energy sector of the Heisenberg necklace model. Using the field-theory methods, we estimate how the coupling of the electronic spins with the paramagnetic Kondo spins affects the overall spin dynamics and evaluate its dependence on a magnetic field. We are motivated by the experimental realizations of the spin-1/2 Heisenberg chains in ${\mathrm{SrCuO}}_{2}$ and ${\mathrm{Sr}}_{2}{\mathrm{CuO}}_{3}$ cuprates, which remain one-dimensional Luttinger liquids down to temperatures much lower than the in-chain exchange coupling $J$. We consider the perturbation of the energy spectrum caused by the interaction $\ensuremath{\gamma}$ with nuclear spins ($I=3/2$) present on the same sites. We find that the resulting necklace model has a characteristic energy scale, $\mathrm{\ensuremath{\Lambda}}\ensuremath{\sim}{J}^{1/3}{(\ensuremath{\gamma}I)}^{2/3}$, at which the coupling between (nuclear) spins of the necklace and the spins of the Heisenberg chain becomes strong. This energy scale is insensitive to a magnetic field $B$. For ${\ensuremath{\mu}}_{B}B>\mathrm{\ensuremath{\Lambda}}$ we find two gapless bosonic modes that have different velocities, whose ratio at strong fields approaches a universal number, $\sqrt{2}+1$.

DOI
10.1103/physrevb.94.075152

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We study a lattice realization of a Luttinger liquid interacting with quantum spins in terms of an antiferromagnetic S=1∕2S=1∕2S=1∕2 Heisenberg chain, where each spin is also coupled to a $\ensuremath{\sigma}=1∕2$ Kondo spin degree of freedom. This model describes the low-energy spin dynamics in quasi-one-dimensional materials, where the electronic spins of the magnetic ions interact with those of impurities, nuclei, and possibly other spin species present in their environment. For large ferromagnetic and antiferromagnetic Kondo interaction ${J}^{\ensuremath{'}}$, there are two phases corresponding to an effective spin-1 Heisenberg chain and a dimerized spin-1∕21∕21∕2 ladder, respectively. For weak Kondo interaction, we establish that the Kondo interaction drives the system to a strong coupling regime. This suggests that ${J}^{\ensuremath{'}}=0$ is the only critical point in the system.
A comprehensive comparison between the magnetic field- and temperature-dependent low-frequency spin dynamics in the antiferromagnetic spin-1/2 Heisenberg chain system copper pyrazine dinitrate, probed via the 13C^{13}\mathrm{C}13C nuclear magnetic resonance relaxation rate ${T}_{1}^{\ensuremath{-}1}$, and the field theoretical approach in the Luttinger liquid regime was performed. We found very good agreement between experiment and theory in the investigated temperature and field range. Our results demonstrate how spin-spin interactions strongly affect the spin dynamics of Heisenberg spin chain compounds in the vicinity of the quantum critical point.
We discuss the thermal and magnetic entanglement in the one-dimensional Kondo necklace model. First, we show how the entanglement naturally present at zero temperature is distributed among pairs of spins according to the strength of the two couplings of the chain, namely, the Kondo exchange interaction and the hopping energy. The effect of temperature and the presence of an external magnetic field are then investigated. We also discuss the adjustment of these variables in order to control the entanglement available in the system. In particular, it is indicated that there exists a critical magnetic field above which the entanglement undergoes a sharp variation, leading the ground state to a completely unentangled phase.
The projector Monte Carlo method and finite-size scaling are applied to the solution of the ground-state properties of the ``Kondo necklace'' Hamiltonian. The energy and various spin-spin correlation functions are calculated for chains up to 16 sites in length. Correlations between the spins on different sites are evaluated, and the nature of the ground-state phase as a function of the ratio of the exchange coupling J to the bandwidth W is examined. Evaluation of the correlation function 〈S\ensuremath{\rightarrow}(i)\ensuremath{\cdot}\ensuremath{\tau}\ensuremath{\rightarrow}(i)〉 shows that as the coupling between the localized S spins and the \ensuremath{\tau} spin chain increases, the system becomes composed of independent singlets on each site. Contrary to both mean-field and various approximate renormalization-group calculations, we find that our results are consistent with an absence of magnetic order as soon as J is different from 0.
We have studied the quantum phase transition between the antiferromagnetic and spin liquid phases for the two-dimensional anisotropic Kondo necklace model. The bond operator formalism has been implemented to transform the spin Hamiltonian to a bosonic one. We have used the Green's function approach including a hard core repulsion to find the low energy excitation spectrum of the model. The bosonic excitations become gapless at the quantum critical point where the phase transition from the Kondo singlet state to long range antiferromagnetic order takes place. We have studied the effect of both intersite $(\ensuremath{\delta})$ and local $(\ensuremath{\Delta})$ anisotropies on the critical point and on the critical exponent of the excitation gap in the paramagnetic phase. We have also compared our results with previous bond operator mean field calculations.
The Kondo-necklace model can describe magnetic low-energy limit of strongly correlated heavy fermion materials. There exist multiple energy scales in this model corresponding to each phase of the system. Here, we study quantum phase transition between the Kondo-singlet phase and the antiferromagnetic long-range ordered phase, and show the effect of anisotropies in terms of quantum information properties and vanishing energy gap. We employ the perturbative continuous unitary transformations approach to calculate the energy gap and spin-spin correlations for the model in the thermodynamic limit of one, two, and three spatial dimensions as well as for spin ladders. In particular, we show that the method, although being perturbative, can predict the expected quantum critical point, where the gap of low-energy spectrum vanishes, which is in good agreement with results of other numerical and Green's function analyses. In addition, we employ concurrence, a bipartite entanglement measure, to study the criticality of the model. Absence of singularities in the derivative of concurrence in two and three dimensions in the Kondo-necklace model shows that this model features multipartite entanglement. We also discuss crossover from the one-dimensional to the two-dimensional model via the ladder structure.