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arXiv:1605.07257

Characterizing micro-macro transitions with an atomic-vapor-based linear optical amplifier

Zhifan Zhou, Ulrich Vogl, Ryan T. Glasser, Zhongzhong Qin, Yami Fang, Jietai Jing, Weiping Zhang

Published May 24, 2016• 3 citations
arXivHTMLPDF

Abstract

Fundamentally, the dynamics of micro-macro transitions is instrumental to understanding the process of quantum-to-classical transitions; technologically, it can also facilitate the detection of the microscopic signals in quantum experiments via convenient detectors. Here, we demonstrate a scheme to characterize micro-macro transitions based on a four-wave mixing linear optical amplification process in a hot rubidium vapor. The linear optical amplifier provides a large optical gain of $10^7$ for injected single-photon-level pulses, enabling photon-number-resolving detection by average via non-single-photon counting detectors with a large dynamic range. The scheme exhibits strong dispersion which is sensitive to the input's change at the single-photon level, resulting in the group-velocity delay time scaling with $1/\sqrt{N}$, where $N$ is the average input photon number. The output probe and conjugate modes have different coefficients of this $1/\sqrt{N}$ scaling, indicating the coefficient can serve as an efficient parameter to characterize the specified micro-macro transitions. The demonstrated results are generally applicable for quantum detection and optical signal processing in light-atom interfaces. Furthermore, the present system is suitable for the study of relevant time-resolved dynamics of the quantum-to-classical transitions.

DOI
10.48550/arxiv.1605.07257

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Fundamentally, the dynamics of micro-macro transitions is instrumental to understanding the process of quantum-to-classical transitions; technologically, it can also facilitate the detection of the microscopic signals in quantum experiments via convenient detectors. Here, we demonstrate a scheme to characterize micro-macro transitions based on a four-wave mixing linear optical amplification process in a hot rubidium vapor. The linear optical amplifier provides a large optical gain of 10710^7107 for injected single-photon-level pulses, enabling photon-number-resolving detection by average via non-single-photon counting detectors with a large dynamic range. The scheme exhibits strong dispersion which is sensitive to the input's change at the single-photon level, resulting in the group-velocity delay time scaling with 1/N1/\sqrt{N}1/N​, where NNN is the average input photon number. The output probe and conjugate modes have different coefficients of this 1/N1/\sqrt{N}1/N​ scaling, indicating the coefficient can serve as an efficient parameter to characterize the specified micro-macro transitions. The demonstrated results are generally applicable for quantum detection and optical signal processing in light-atom interfaces. Furthermore, the present system is suitable for the study of relevant time-resolved dynamics of the quantum-to-classical transitions.
The transition between the microscopic to the macroscopic world is of broad fundamental and technological significance. Optical parametric amplifiers allow for amplifying single photons to the macroscopic level, but the underlying temporal dynamics are still not well understood. Slow light, in which the group velocity is delayed via quantum interference, is an effective tool to interrogate the temporal dynamics of light-matter interactions. Here, we demonstrate a scheme to characterize micro-macro transitions with slow light based on a four-wave mixing linear amplification process in a hot rubidium vapour. The scheme exhibits strong dispersion which is sensitive to the input's change at the single-photon level, resulting in a nonlinear decay of the micro-macro transition time with the increased microscopic input. The present system is suitable for the study of the relevant time scale of quantum-to-classical transitions and the potential impact from fundamental effects such as gravity, as indicated by recent proposals.
We recently demonstrated optical pulses with large negative group velocities using a scheme based on four-wave-mixing in rubidium vapor. Both the probe and the generated conjugate pulses can experience anomalous dispersion, and we have demonstrated a maximum group advancement of 64% relative to the input pulse width. The four-wave-mixing scheme allows us to send whole images through a fast light medium, and we have analyzed the arrival of spatially-encoded information in the system. We are currently investigating the transport of quantum correlations that are shared by the probe and conjugate modes when sent through fast light media.
Wavepackets are excited in rubidium vapor by intense ultrashort (∼100 fs) pulses centered at a wavelength of 620 nm or 770 nm. The generated atomic wavepackets are optically detected via a pump-probe experiment based on axially phase-matched parametric four-wave mixing (FWM). This nonlinear process results in coherent ultraviolet (UV) or violet emission that carries information about the relative number densities of the excited states. The frequency spectrum of the UV/violet signal intensity, recorded while varying the pump-probe time delay, shows the presence of quantum beats between energy levels involved in the FWM process. The time-frequency analysis of that temporal UV/violet data is done by means of the short-time Fourier transform that leads to retrieval of the temporal evolution of amplitude and phase of the quantum beats. The observed dynamics suggest that not only atomic but also molecular ( Rb*2 ) wavepackets are generated, and that the temporal history of the amplitude of the quantum beats reflects the production of the excited atomic fragments of Rb*2 dissociation. More precisely, changes in the Rb excited state number densities alter the third-order nonlinear susceptibility chi(3) of the Rb vapor, which affects generation of the output signal wave by FWM. Dissociation into several product states is detected, and their branching ratios are estimated. Thus, atomic wavepackets, combined with FWM, appear to be a sensitive new multichannel spectroscopic means to study the fundamental process of molecular dissociation.
Temporal dissipative solitons are central to nonlinear photonics, yet conventional platforms such as optical fibers and microresonators provide limited dispersion tunability and weak nonlinearities. Here, we demonstrate a highly tunable soliton platform based on atom–light interactions in a rubidium vapor optical parametric oscillator. A continuous-wave pump drives four-wave mixing in the vapor, generating probe and conjugate fields, one of which is fed back through a fiber loop to form the oscillator. By tuning the pump intensity and detuning, we control the dispersive properties and third-order nonlinearity of the medium, enabling the formation of diverse nonlinear states including bright and dark solitons, soliton crystals, dark–bright soliton pairs, platicons, and breather solitons. Unlike conventional systems, solitons emerge spontaneously without cavity scanning or pulsed excitation. The system isolates gain, dispersion, and nonlinearity within the atomic medium, allowing flexible cavity-length tuning without modifying other operating parameters. We introduce the technique of characterizing the solitonic states through the linewidth of the output intensity power spectrum, which remains independent of cavity length and is limited only by the experimental apparatus, indicating a high degree of phase coherence. This contrasts with conventional mode-locked states, for which the linewidth scales inversely with the square of the cavity length. With pulse durations of ∼100 ns determined by the gain bandwidth of the four-wave mixing, the solitons can be directly detected for rapid and complete characterization. This platform offers a versatile route for exploring nonlinear optical dynamics and developing applications in quantum photonics and communication.
Phase-sensitive nonlinear gain processes have been implemented as noise-reduced optical amplifiers, which have the potential to achieve signal-to-noise ratios beyond the classical limit. We experimentally demonstrate a novel phase-sensitive four-wave mixing amplification process in a single atomic vapor cell with only two input frequencies and two input vacuum modes. The amount of phase sensitivity depends on the power ratio between the inserted probes as well as on the input frequency of the probes. We find that, for certain phase values, the intensity noise of an output mode is lower than that of its phase-insensitive counterpart.