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arXiv:1605.05132 · Physical Review A

Single-atom single-photon coupling facilitated by atomic-ensemble dark-state mechanisms

Andrew C. J. Wade, Marco Mattioli, Klaus Mølmer

Published Nov 16, 2016• 32 citations
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Abstract

We propose to couple single atomic qubits to photons incident on a cavity containing an atomic ensemble of a different species that mediates the coupling via Rydberg interactions. Subject to a classical field and the cavity field, the ensemble forms a collective dark state which is resonant with the input photon, while excitation of a qubit atom leads to a secondary ``dark'' state that splits the cavity resonance. The two different dark-state mechanisms yield zero and $\ensuremath{\pi}$ reflection phase shifts and can be used to implement quantum gates between atomic and optical qubits.

DOI
10.1103/physreva.94.053830

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We propose to couple single atomic qubits to photons incident on a cavity containing an atomic ensemble of a different species that mediates the coupling via Rydberg interactions. Subject to a classical field and the cavity field, the ensemble forms a collective dark state which is resonant with the input photon, while excitation of a qubit atom leads to a secondary ``dark'' state that splits the cavity resonance. The two different dark-state mechanisms yield zero and \ensuremathπ\ensuremath{\pi}\ensuremathπ reflection phase shifts and can be used to implement quantum gates between atomic and optical qubits.
We propose to use the interaction between a single qubit atom and a surrounding ensemble of three level atoms to control the phase of light reflected by an optical cavity. Our scheme employs an ensemble dark resonance that is perturbed by the qubit atom to yield a single-atom single photon gate. We show here that off-resonant excitation towards Rydberg states with strong dipolar interactions offers experimentally-viable regimes of operations with low errors (in the 10 −3 range) as required for fault-tolerant optical-photon, gate-based quantum computation. We also propose and analyze an implementation within microwave circuit-QED, where a strongly-coupled ancilla superconducting qubit can be used in the place of the atomic ensemble to provide high-fidelity coupling to microwave photons.
The realization of a Jaynes-Cummings model in the optical domain is proposed for an atomic ensemble. The scheme exploits the collective coupling of the atoms to a quantized cavity mode and the nonlinearity introduced by coupling to high-lying Rydberg states. A two-photon transition resonantly couples the single-atom ground state $|g\ensuremath{\rangle}$ to a Rydberg state $|e\ensuremath{\rangle}$ via a nonresonant intermediate state $|i\ensuremath{\rangle}$, but due to the interaction between Rydberg atoms only a single atom can be resonantly excited in the ensemble. This restricts the state space of the ensemble to the collective ground state $|G\ensuremath{\rangle}$ and the collectively excited state $|E\ensuremath{\rangle}$ with a single Rydberg excitation distributed evenly on all atoms. The collectively enhanced coupling of all atoms to the cavity field with coherent coupling strengths which are much larger than the decay rates in the system leads to the strong coupling regime of the resulting effective Jaynes-Cummings model. We use numerical simulations to show that the cavity transmission can be used to reveal detailed properties of the Jaynes-Cummings ladder of excited states and that the atomic nonlinearity gives rise to highly nontrivial photon emission from the cavity. Finally, we suggest that the absence of interactions between remote Rydberg atoms may, due to a combinatorial effect, induce a cavity-assisted excitation blockade whose range is larger than the typical Rydberg dipole-dipole interaction length.
In Chapter 7 we discussed the interaction between atoms and photons. We found that the coupling between a single atom and a single photon is rather weak, unless the atom and the photon are contained within a small cavity. The only way to significantly affect a free atom with light is to use a state of light with many photons, and in particular we showed how to use classical laser fields to prepare particular atomic states. However, there is another way of enhancing the interaction in a useful way. We can use many atoms rather than a single one. In this chapter, we will show that the interaction between a single photon and an ensemble of atoms can be greatly increased through the phenomenon of collective enhancement. We will show that this gives an atomic ensemble a relatively large susceptibility, and that multilevel atoms can be used to generate large optical nonlinearities. These offer the possibility of slowing, and even stopping, a beam of light; a phenomenon that goes hand in hand with electromagnetically induced transparency. We will discuss how a quantum state of light can be stored in and retrieved from an ensemble of atoms, and how the states of different atomic ensembles can be entangled with one another. We will show that collective states of atoms can even be used as a single qubit or several qubits, and finally, we will show that atomic ensembles can be use to mediate a photon–photon interaction.
We demonstrate a new approach for creating deterministic photon-photon interactions for optical quantum engineering, based on a single-ended medium-finesse optical cavity containing a mesoscopic atomic ensemble. This ensemble is made transparent by a laser beam mapping intracavity photons into Rydberg polaritons. The transparency vanishes when the cloud, acting as a single collective two-level "superatom" with an enhanced coupling to light, is driven from the ground to a Rydberg state. We observe collectively-enhanced Rabi oscillations between these states, optically discriminate them in a single shot with a 95% effciency, and show that a change between the two internal states of the superatom induces a π phase rotation on the light reflected off of the cavity. These ingredients form a complete set of tools for implementing deterministic photonic entangling gates and for generating highly non-classical light without the need for a low-volume high-finesse cavity.
Quantum controlled-phase-flip (CPF) gate between a flying photon qubit and a stationary atomic qubit could allow the linking of distant computational nodes in a quantum network. Here we present a scheme to realize quantum CPF gate between a flying optical photon and an atomic ensemble based on cavity input-output process and Rydberg blockade. When a flying single-photon pulse is reflected off the cavity containing a Rydberg atomic ensemble, the dark resonance and Rydberg blockade induce a conditional phase shift for the photon pulse, thus we can achieve the CPF gate between the photon and the atomic ensemble. Assisted by Rydberg blockade interaction, our scheme works in the N-atoms strong-coupling regime and significantly relaxes the requirement of strong coupling of single atom to photon in the optical cavity.
Interacting Rydberg excitations in cold atomic ensembles can exhibit large quantum nonlinearities that enable engineering of strong interactions between individual photons. Consequently, Rydberg ensembles are a promising platform for quantum information applications and the study of more fundamental physics of few- and many-body phenomena with interacting photons. This thesis presents a series of experiments that study and exploit different regimes of Rydberg-mediated interactions. We report the realization of an efficient on-demand single-photon source. The strong long-range Rydberg interactions allow the excitation of only a single collective Rydberg state within the entire atomic medium. The collective excitation can be subsequently retrieved as a single-photon. We use this scheme to generate highly pure and highly indistinguishable photons, which are suitable for scalable quantum information applications. These photons can be compatible with other atomic systems due to their narrow bandwidth, which makes building practical hybrid quantum systems feasible. Here, we demonstrate high visibility two-photon quantum interference between our Rydberg-produced photons, and photons emitted by a remote single-trapped ion. We also study Rydberg atoms under electromagnetically induced transparency conditions, where coherent superpostions of photons and Rydberg excitations propagate through the atomic medium as lossless dark-state polaritons. In the experiment, we use the external control fields to tune the interactions to a many-body regime where we can observe resonant scattering of dark-state polaritons to lossy channels. We show that the enhanced scattering process arises as a pure three-body effect.