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arXiv:1603.06473 · Physical review. B./Physical review. B

Singular ferromagnetic susceptibility of the transverse-field Ising antiferromagnet on the triangular lattice

Sounak Biswas, Kedar Damle

Published Feb 8, 2018• 15 citations
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Abstract

A transverse magnetic field $\mathrm{\ensuremath{\Gamma}}$ is known to induce antiferromagnetic three-sublattice order of the Ising spins ${\ensuremath{\sigma}}^{z}$ in the triangular lattice Ising antiferromagnet at low enough temperature. This low-temperature order is known to melt on heating in a two-step manner, with a power-law ordered intermediate temperature phase characterized by power-law correlations at the three-sublattice wave vector $\mathbf{Q}$: $\ensuremath{\langle}{\ensuremath{\sigma}}^{z}(\stackrel{P\vec}{R}){\ensuremath{\sigma}}^{z}(0)\ensuremath{\rangle}\ensuremath{\sim}cos(\mathbf{Q}\ifmmode\cdot\else\textperiodcentered\fi{}\stackrel{P\vec}{R})/{|\stackrel{P\vec}{R}|}^{\ensuremath{\eta}(T)}$ with the temperature-dependent power-law exponent $\ensuremath{\eta}(T)\ensuremath{\in}(1/9,1/4)$. Here, we use a quantum cluster algorithm to study the ferromagnetic easy-axis susceptibility ${\ensuremath{\chi}}_{u}(L)$ of an $L\ifmmode\times\else\texttimes\fi{}L$ sample in this power-law ordered phase. Our numerical results are consistent with a recent prediction of a singular $L$ dependence ${\ensuremath{\chi}}_{u}(L)\ensuremath{\sim}{L}^{2\ensuremath{-}9\ensuremath{\eta}}$ when $\ensuremath{\eta}(T)$ is in the range $(1/9,2/9)$. This finite-size result implies, via standard scaling arguments, that the ferromagnetic susceptibility ${\ensuremath{\chi}}_{u}(B)$ to a uniform field $B$ along the easy axis is singular at intermediate temperatures in the small $B$ limit, ${\ensuremath{\chi}}_{u}(B)\ensuremath{\sim}{|B|}^{\ensuremath{-}\frac{4\ensuremath{-}18\ensuremath{\eta}}{4\ensuremath{-}9\ensuremath{\eta}}}$ for $\ensuremath{\eta}(T)\ensuremath{\in}(1/9,2/9)$, although there is no ferromagnetic long-range order in the low temperature state. Additionally we establish similar two-step melting behavior (via a study of the order parameter susceptibility ${\ensuremath{\chi}}_{\mathbf{Q}}$) in the case of the ferrimagnetic three-sublattice ordered phase which is stabilized by ferromagnetic next-neighbor couplings (${J}_{2}$) and confirm that the ferromagnetic susceptibility obeys the predicted singular form in the associated power-law ordered phase.

DOI
10.1103/physrevb.97.085114

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A transverse magnetic field \ensuremathΓ\mathrm{\ensuremath{\Gamma}}\ensuremathΓ is known to induce antiferromagnetic three-sublattice order of the Ising spins \ensuremathσz{\ensuremath{\sigma}}^{z}\ensuremathσz in the triangular lattice Ising antiferromagnet at low enough temperature. This low-temperature order is known to melt on heating in a two-step manner, with a power-law ordered intermediate temperature phase characterized by power-law correlations at the three-sublattice wave vector Q\mathbf{Q}Q: \ensuremath{\langle}{\ensuremath{\sigma}}^{z}(\stackrel{P\vec}{R}){\ensuremath{\sigma}}^{z}(0)\ensuremath{\rangle}\ensuremath{\sim}cos(\mathbf{Q}\ifmmode\cdot\else\textperiodcentered\fi{}\stackrel{P\vec}{R})/{|\stackrel{P\vec}{R}|}^{\ensuremath{\eta}(T)} with the temperature-dependent power-law exponent \ensuremathη(T)\ensuremath∈(1/9,1/4)\ensuremath{\eta}(T)\ensuremath{\in}(1/9,1/4)\ensuremathη(T)\ensuremath∈(1/9,1/4). Here, we use a quantum cluster algorithm to study the ferromagnetic easy-axis susceptibility \ensuremathχu(L){\ensuremath{\chi}}_{u}(L)\ensuremathχu​(L) of an L\ifmmode×\else\texttimes\fiLL\ifmmode\times\else\texttimes\fi{}LL\ifmmode×\else\texttimes\fiL sample in this power-law ordered phase. Our numerical results are consistent with a recent prediction of a singular LLL dependence \ensuremathχu(L)\ensuremath∼L2\ensuremath−9\ensuremathη{\ensuremath{\chi}}_{u}(L)\ensuremath{\sim}{L}^{2\ensuremath{-}9\ensuremath{\eta}}\ensuremathχu​(L)\ensuremath∼L2\ensuremath−9\ensuremathη when \ensuremathη(T)\ensuremath{\eta}(T)\ensuremathη(T) is in the range (1/9,2/9)(1/9,2/9)(1/9,2/9). This finite-size result implies, via standard scaling arguments, that the ferromagnetic susceptibility \ensuremathχu(B){\ensuremath{\chi}}_{u}(B)\ensuremathχu​(B) to a uniform field BBB along the easy axis is singular at intermediate temperatures in the small BBB limit, \ensuremathχu(B)\ensuremath∼∣B∣\ensuremath−4\ensuremath−18\ensuremathη4\ensuremath−9\ensuremathη{\ensuremath{\chi}}_{u}(B)\ensuremath{\sim}{|B|}^{\ensuremath{-}\frac{4\ensuremath{-}18\ensuremath{\eta}}{4\ensuremath{-}9\ensuremath{\eta}}}\ensuremathχu​(B)\ensuremath∼∣B∣\ensuremath−4\ensuremath−9\ensuremathη4\ensuremath−18\ensuremathη​ for \ensuremathη(T)\ensuremath∈(1/9,2/9)\ensuremath{\eta}(T)\ensuremath{\in}(1/9,2/9)\ensuremathη(T)\ensuremath∈(1/9,2/9), although there is no ferromagnetic long-range order in the low temperature state. Additionally we establish similar two-step melting behavior (via a study of the order parameter susceptibility \ensuremathχQ{\ensuremath{\chi}}_{\mathbf{Q}}\ensuremathχQ​) in the case of the ferrimagnetic three-sublattice ordered phase which is stabilized by ferromagnetic next-neighbor couplings (J2{J}_{2}J2​) and confirm that the ferromagnetic susceptibility obeys the predicted singular form in the associated power-law ordered phase.
Melting of three-sublattice order in triangular lattice Ising antiferromagnets: Power-law order, Z6Z_6Z6​ parafermionic multicriticality, and weakly first order transitions
The nature of the thermal melting process by which triangular-lattice Ising antiferromagnets lose their low-temperature ferrimagnetic three-sublattice order depends on the range of the interactions: It changes character when second and third neighbour ferromagnetic interactions become comparable to the nearest-neighbour antiferromagnetic coupling. We present a detailed numerical characterization of the corresponding threshold at which two-step melting of three-sublattice order gives way to a direct first-order transition at which this order is lost. The multicritical behaviour at this threshold is argued to be in the universality class of the Z6Z_6Z6​ parafermion conformal field theory with central charge c=5/4c=5/4c=5/4. The presence of this multicritical threshold influences the melting behaviour and long-wavelength properties over a fairly large range of parameters, and at temperatures that are of the same order as the exchange interactions. It is therefore of potential experimental relevance in the context of easy-axis triangular lattice antiferromagnets that display such low temperature ordering.
Motivated by recent experiments with a Penning ion trap quantum simulator, we perform numerically exact Stochastic Series Expansion quantum Monte Carlo simulations of long-range transverse-field Ising models on a triangular lattice for different decay powers $\ensuremath{\alpha}$ of the interactions. The phase boundary for the ferromagnet is obtained as a function of $\ensuremath{\alpha}$. For antiferromagnetic interactions, there is strong indication that the transverse field stabilizes a clock ordered phase with sublattice magnetization $(M,\ensuremath{-}\frac{M}{2},\ensuremath{-}\frac{M}{2})$ with unsaturated M<1M<1M<1 in a process known as ``order by disorder'' similar to the nearest-neighbor antiferromagnet on the triangular lattice. Connecting the known limiting cases of nearest-neighbor and infinite-range interactions, a semiquantitative phase diagram is obtained. Magnetization curves for the ferromagnet for experimentally relevant system sizes and with open boundary conditions are presented.
By combining all available information it is possible to extend the numerical knowledge of the high- and low-temperature zero-field isothermal susceptibility of the Ising model. Estimates of the third most singular term of the ferromagnetic singularity are obtained, using both direct estimates and an extension of the Generalized Law of Corresponding States. A recent conjecture of Barouch, McCoy and Wu (1973) concerning the equality of the constant term in the asymptotic expansion of the high- and low-temperature ferromagnetic susceptibility is confirmed numerically. Finally, a non-physical critical exponent of the low-temperature susceptibility of the triangular lattice is identified.
The ground-state properties of the triangular antiferromagnetic Ising model with Ising constant J in a transverse field h are investigated by a real-space renormalisation group method. For h=0, the known properties (energy=-J, finite entropy, no order) are recovered. For h not=0, the ground state remains highly degenerate, no order exists and the correlation function exhibits power-law behaviour up to (h/J)c approximately=1.41, where a phase transition takes place to a non-degenerate ground state. At h/J=(h/J)c, power-law behaviour is still observed for the correlation function but with a different exponent. Just above this region a gap Delta opens ( Delta approximately ((h/J)-(h/J)c)s with s=0.8) and the coherence length of the correlation function xi diverges as xi varies as ((h/J)-(h/J)c)-v with v=0.8. This corresponds to a three-dimensional classical model where h is replaced by the temperature. In this type of system, where the ground state has a degeneracy proportional to N2/3 it is predicted that a transition will occur at a finite T c to a low-temperature phase without order but with power-law behaviour for the correlation function, as for the classical XY model in two dimensions.
Working within the stochastic series expansion framework, we introduce and characterize a plaquette-based quantum cluster algorithm for quantum Monte Carlo simulations of transverse field Ising models with frustrated Ising exchange interactions. As a demonstration of the capabilities of this algorithm, we show that a relatively small ferromagnetic next-nearest-neighbor coupling drives the transverse field Ising antiferromagnet on the triangular lattice from an antiferromagnetic three-sublattice ordered state at low temperature to a ferrimagnetic three-sublattice ordered state.
The rare-earth magnet TmMgGaO 4 is proposed to be an intrinsic quantum Ising magnet described by the antiferromagnetic transverse field Ising model (TFIM) on a triangular lattice, where the relevant degrees of freedom are the nondegenerate dipole-multipole doublets of the Tm 3+ ions and the transverse field has an intrinsic origin from the weak splitting of the doublet.We compare this special doublet of Tm 3+ with the dipole-octupole Kramers doublet.We study the proposed effective model for the Tm-based triangular lattice and consider the effects of external magnetic fields and finite temperatures.From the orthogonal operator approach, we show that the TFIM with the three-sublattice intertwined ordered state agrees with the experiments and further clarify the discrepancy in the numbers of the magnetic sublattices and the measured magnon branches.We make specific predictions for the evolution of the magnetic properties with the external magnetic field.Furthermore, we demonstrate that an emergent U(1) symmetry emerges in thermal melting of the underlying orders and at the criticality, and summarize the previously known signatures related to the finite-temperature Berezinskii-Kosterlitz-Thouless physics.We discuss the broad relevance of intrinsic quantum Ising magnets to many other systems, especially Tm-based materials.