Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1603.04509 · Physical Review A

Quantum-enhanced spectroscopy with entangled multiphoton states

Hossein T. Dinani, Manish K. Gupta, Jonathan P. Dowling, Dominic William Berry

Published Jun 7, 2016• 22 citations
arXivHTMLPDF

Abstract

Traditionally, spectroscopy is performed by examining the position of absorption lines. However, at frequencies near the transition frequency, additional information can be obtained from the phase shift. In this work we consider the information about the transition frequency obtained from both the absorption and the phase shift, as quantified by the Fisher information in an interferometric measurement. We examine the use of multiple single-photon states, NOON states, and numerically optimized states that are entangled and have multiple photons. We find the optimized states that improve over the standard quantum limit set by independent single photons for some atom number densities.

DOI
10.1103/physreva.93.063804

Related papers

Optimal conventional measurements for quantum-enhanced interferometry

Wei Zhong, Yixiao Huang, Xiaoguang Wang +1 more

A major obstacle to attaining the fundamental precision limit of phase estimation in interferometry is the identification and implementation of the optimal measurement. Here we demonstrate that this can be accomplished by the use of three conventional measurements among interferometers with Bayesian estimation techniques. Conditions that hold for the precision limit to be attained with these measurements are obtained by explicitly calculating the Fisher information. Fortunately, these conditions are naturally satisfied in most interferometric experiments. We apply our results to an atomic spectroscopy experiment and examine the robustness of phase sensitivity for the two-axis counter-twisted state suffering from detection noise.

arXiv:1611.07328•Physical Review A•May 2, 2017•18 citations

Quantum Optical Metrology Using Two-Photon Interference

Kyle Jordan

Optical quantum metrology uses specially-prepared states of light to probe sensitive samples. Choosing a suitable probe state allows one to extract more information per probe photon about an unknown parameter than is possible using any classical technique. In effect, these techniques improve the sensitivity of the measurement whenever the number of probe photons is constrained in some way. This thesis presents experimental and theoretical results on the use of pairs of time-frequency entangled photons in precision measurements. It begins with an overview of necessary background knowledge about quantum optics and quantum information. This is followed by a theoretical discussion on the estimation of a single delay using two-photon interference. We show that constraints on the probe photon's bandwidth complicate the measurement problem, requiring suitable optimization of the two-photon quantum state to avoid losing precision. We then consider the use of two-photon interference for linear spectroscopic measurements. Linear spectroscopy relates the absorption and phase spectrum of a sample to unknown electronic parameters. We describe a proof-of-principle experiment demonstrating that two-photon interferometric spectroscopy can be used for simultaneously measurement of both absorption and phase. This is followed by an information-theoretic discussion of the precision of this technique. For low losses, we show that the method provides phase sensitivity similar to classical interferometry while approaching the optimal absorption precision of any possible measurement. If the absorption and phase values are both related to a single unknown parameter, then our technique provides improved sensitivity to this parameter compared to both classical measurements and other quantum techniques in the presence of realistic levels of loss. We conclude with a discussion of quantum-optical coherence tomography, which is a two-photon interferometric method for determining the material structure of a sample. We present an ongoing experiment which aims to apply the method to tissue-like samples, where the quantum measurement is limited by a poor signal-to-noise ratio. Preliminary results demonstrate that this noise can be largely reduced by suitable frequency-domain filtering. This allows us to precisely determine the position of a scattering center using a few hundred detected photon pairs despite the presence of large amounts of noise. We follow this with a theoretical discussion of signal artifacts which are known to complicate the measured interferogram. We show these artifacts are due to a distinct interferometric effect, which can be distinguished from the signal of interest using the relative time delay between detected photons. We conclude with a brief discussion on possible techniques for artifact removal.

•Jan 22, 2026•0 citations

Optimal entangled coherent states in lossy quantum-enhanced metrology

Su‐Yong Lee, Yong Sup Ihn, Zaeill Kim

We investigate an optimal distance of two components in an entangled coherent state for quantum phase estimation in lossy interferometry. The optimal distance is obtained by an economical point, representing the quantum Fisher information that we can extract per input energy. Maximizing the formula of the quantum Fisher information over an input mean photon number, we show that, as the losses of the interferometer increase, it can be more beneficial to prepare an initially entangled coherent state that is less entangled. This represents that the optimal distance of the two-mode components decreases with more loss in the interferometry. Under the constraint of the input mean photon number, we obtain that the optimal entangled coherent state is more robust than a separable coherent state, even in a high photon loss rate. The optimal entangled coherent state preserves quantum advantage over the standard interferometric limit of the separable coherent state. We also show that the corresponding optimal measurement requires correlation measurement bases.

arXiv:1906.05402•Physical Review A•Jan 21, 2020•22 citations

Optimizing the multiphoton absorption properties of maximally path-entangled number states

William N. Plick, Christoph F. Wildfeuer, Petr M. Anisimov +1 more

In this paper we examine the $N$-photon absorption properties of maximally path-entangled number states ($N00N$ states). We consider two cases. The first involves the $N$-photon absorption properties of the ideal $N00N$ state, one that does not include spectral information. We study how the $N$-photon absorption probability of this state scales with $N$, confirming results presented by others in a previous paper by a different method. We compare this to the absorption probability of various other states. The second case is that of two-photon absorption for an $N=2$ $N00N$ state generated from a type-II spontaneous down-conversion event. In this situation we find that the absorption probability is both better than analogous coherent light (due to frequency entanglement) and highly dependent on the optical setup. We show that the poor production rates of quantum states of light may be partially mitigated by adjusting the spectral parameters to improve their two-photon absorption rates. This work has application to quantum imaging, particularly quantum lithography, where the $N$-photon absorbing process in the lithographic resist must be optimized for practical applications.

Physical Review A•Dec 9, 2009•9 citations

Quantum Fisher information of entangled coherent states in the presence of photon loss

Y. M. Zhang, Xinwei Li, Wen Yang +1 more

We investigate the performance of entangled coherent states for quantum-enhanced phase estimation. An exact analytical expression of quantum Fisher information is derived to show the role of photon losses on the ultimate phase sensitivity. We find a transition of the sensitivity from the Heisenberg scaling to the classical scaling due to quantum decoherence of the photon state. This quantum-classical transition is uniquely determined by the number of photons being lost, instead of the number of incident photons or the photon loss rate alone. Our results also reveal that a crossover of the sensitivity between the entangled coherent state and the NOON state can occur even for very small photon loss rate.

arXiv:1307.7353•Physical Review A•Oct 17, 2013•208 citations

Two-photon phase-sensing with single-photon detection

Panagiotis Vergyris, Charles Babin, Raphael Nold +6 more

Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realizing this experimentally is technologically demanding, as it requires coincident single-photon detection proportional to the number of photons involved, which represents a severe challenge for achieving a practical quantum advantage over classical methods. Here, we exploit advanced quantum state engineering based on superposing two photon-pair creation events to realize a new approach that bypasses this issue. In particular, optical phase shifts are probed with a two-photon quantum state whose information is subsequently effectively transferred to a single-photon state. Notably, without any multiphoton detection, we infer phase shifts by measuring the average intensity of the single-photon beam on a photodiode, in analogy to standard classical measurements. Importantly, our approach maintains the quantum advantage: twice as many interference fringes are observed for the same phase shift, corresponding to N = 2 path-entangled photons. Our results demonstrate that the advantages of quantum-enhanced phase sensing can be fully exploited in standard intensity measurements, paving the way toward resource-efficient and practical quantum optical metrology.

arXiv:2007.02586•Applied Physics Letters•Jul 13, 2020•15 citations
Traditionally, spectroscopy is performed by examining the position of absorption lines. However, at frequencies near the transition frequency, additional information can be obtained from the phase shift. In this work we consider the information about the transition frequency obtained from both the absorption and the phase shift, as quantified by the Fisher information in an interferometric measurement. We examine the use of multiple single-photon states, NOON states, and numerically optimized states that are entangled and have multiple photons. We find the optimized states that improve over the standard quantum limit set by independent single photons for some atom number densities.
A major obstacle to attaining the fundamental precision limit of phase estimation in interferometry is the identification and implementation of the optimal measurement. Here we demonstrate that this can be accomplished by the use of three conventional measurements among interferometers with Bayesian estimation techniques. Conditions that hold for the precision limit to be attained with these measurements are obtained by explicitly calculating the Fisher information. Fortunately, these conditions are naturally satisfied in most interferometric experiments. We apply our results to an atomic spectroscopy experiment and examine the robustness of phase sensitivity for the two-axis counter-twisted state suffering from detection noise.
Optical quantum metrology uses specially-prepared states of light to probe sensitive samples. Choosing a suitable probe state allows one to extract more information per probe photon about an unknown parameter than is possible using any classical technique. In effect, these techniques improve the sensitivity of the measurement whenever the number of probe photons is constrained in some way. This thesis presents experimental and theoretical results on the use of pairs of time-frequency entangled photons in precision measurements. It begins with an overview of necessary background knowledge about quantum optics and quantum information. This is followed by a theoretical discussion on the estimation of a single delay using two-photon interference. We show that constraints on the probe photon's bandwidth complicate the measurement problem, requiring suitable optimization of the two-photon quantum state to avoid losing precision. We then consider the use of two-photon interference for linear spectroscopic measurements. Linear spectroscopy relates the absorption and phase spectrum of a sample to unknown electronic parameters. We describe a proof-of-principle experiment demonstrating that two-photon interferometric spectroscopy can be used for simultaneously measurement of both absorption and phase. This is followed by an information-theoretic discussion of the precision of this technique. For low losses, we show that the method provides phase sensitivity similar to classical interferometry while approaching the optimal absorption precision of any possible measurement. If the absorption and phase values are both related to a single unknown parameter, then our technique provides improved sensitivity to this parameter compared to both classical measurements and other quantum techniques in the presence of realistic levels of loss. We conclude with a discussion of quantum-optical coherence tomography, which is a two-photon interferometric method for determining the material structure of a sample. We present an ongoing experiment which aims to apply the method to tissue-like samples, where the quantum measurement is limited by a poor signal-to-noise ratio. Preliminary results demonstrate that this noise can be largely reduced by suitable frequency-domain filtering. This allows us to precisely determine the position of a scattering center using a few hundred detected photon pairs despite the presence of large amounts of noise. We follow this with a theoretical discussion of signal artifacts which are known to complicate the measured interferogram. We show these artifacts are due to a distinct interferometric effect, which can be distinguished from the signal of interest using the relative time delay between detected photons. We conclude with a brief discussion on possible techniques for artifact removal.
We investigate an optimal distance of two components in an entangled coherent state for quantum phase estimation in lossy interferometry. The optimal distance is obtained by an economical point, representing the quantum Fisher information that we can extract per input energy. Maximizing the formula of the quantum Fisher information over an input mean photon number, we show that, as the losses of the interferometer increase, it can be more beneficial to prepare an initially entangled coherent state that is less entangled. This represents that the optimal distance of the two-mode components decreases with more loss in the interferometry. Under the constraint of the input mean photon number, we obtain that the optimal entangled coherent state is more robust than a separable coherent state, even in a high photon loss rate. The optimal entangled coherent state preserves quantum advantage over the standard interferometric limit of the separable coherent state. We also show that the corresponding optimal measurement requires correlation measurement bases.
In this paper we examine the NNN-photon absorption properties of maximally path-entangled number states (N00NN00NN00N states). We consider two cases. The first involves the NNN-photon absorption properties of the ideal N00NN00NN00N state, one that does not include spectral information. We study how the NNN-photon absorption probability of this state scales with NNN, confirming results presented by others in a previous paper by a different method. We compare this to the absorption probability of various other states. The second case is that of two-photon absorption for an N=2N=2N=2 N00NN00NN00N state generated from a type-II spontaneous down-conversion event. In this situation we find that the absorption probability is both better than analogous coherent light (due to frequency entanglement) and highly dependent on the optical setup. We show that the poor production rates of quantum states of light may be partially mitigated by adjusting the spectral parameters to improve their two-photon absorption rates. This work has application to quantum imaging, particularly quantum lithography, where the NNN-photon absorbing process in the lithographic resist must be optimized for practical applications.
We investigate the performance of entangled coherent states for quantum-enhanced phase estimation. An exact analytical expression of quantum Fisher information is derived to show the role of photon losses on the ultimate phase sensitivity. We find a transition of the sensitivity from the Heisenberg scaling to the classical scaling due to quantum decoherence of the photon state. This quantum-classical transition is uniquely determined by the number of photons being lost, instead of the number of incident photons or the photon loss rate alone. Our results also reveal that a crossover of the sensitivity between the entangled coherent state and the NOON state can occur even for very small photon loss rate.
Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realizing this experimentally is technologically demanding, as it requires coincident single-photon detection proportional to the number of photons involved, which represents a severe challenge for achieving a practical quantum advantage over classical methods. Here, we exploit advanced quantum state engineering based on superposing two photon-pair creation events to realize a new approach that bypasses this issue. In particular, optical phase shifts are probed with a two-photon quantum state whose information is subsequently effectively transferred to a single-photon state. Notably, without any multiphoton detection, we infer phase shifts by measuring the average intensity of the single-photon beam on a photodiode, in analogy to standard classical measurements. Importantly, our approach maintains the quantum advantage: twice as many interference fringes are observed for the same phase shift, corresponding to N = 2 path-entangled photons. Our results demonstrate that the advantages of quantum-enhanced phase sensing can be fully exploited in standard intensity measurements, paving the way toward resource-efficient and practical quantum optical metrology.