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arXiv:1602.08645 · Nature Communications

Quantum lock-in force sensing using optical clock Doppler velocimetry

Ravid Shaniv, Roee Ozeri

Published Feb 10, 2017• 45 citations
arXivHTMLPDF

Abstract

Abstract Force sensors are at the heart of different technologies such as atomic force microscopy or inertial sensing. These sensors often rely on the measurement of the displacement amplitude of mechanical oscillators under applied force. The best sensitivity is typically achieved when the force is alternating at the mechanical resonance frequency of the oscillator, thus increasing its response by the mechanical quality factor. The measurement of low-frequency forces, that are below resonance, is a more difficult task as the resulting oscillation amplitudes are significantly lower. Here we use a single-trapped 88Sr+ ion as a force sensor. The ion is electrically driven at a frequency much lower than the trap resonance frequency. We measure small amplitude of motion by measuring the periodic Doppler shift of an atomic optical clock transition, enhanced using the quantum lock-in technique. We report frequency force detection sensitivity as low as 2.8 × 10−20 NHz−1/2.

DOI
10.1038/ncomms14157

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Abstract Force sensors are at the heart of different technologies such as atomic force microscopy or inertial sensing. These sensors often rely on the measurement of the displacement amplitude of mechanical oscillators under applied force. The best sensitivity is typically achieved when the force is alternating at the mechanical resonance frequency of the oscillator, thus increasing its response by the mechanical quality factor. The measurement of low-frequency forces, that are below resonance, is a more difficult task as the resulting oscillation amplitudes are significantly lower. Here we use a single-trapped 88Sr+ ion as a force sensor. The ion is electrically driven at a frequency much lower than the trap resonance frequency. We measure small amplitude of motion by measuring the periodic Doppler shift of an atomic optical clock transition, enhanced using the quantum lock-in technique. We report frequency force detection sensitivity as low as 2.8 × 10−20 NHz−1/2.
The ability to detect extremely small forces is vital for a variety of disciplines including precision spin-resonance imaging, microscopy, and tests of fundamental physical phenomena. Current force-detection sensitivity limits have surpassed 1 aN/HzaN/\sqrt{Hz}aN/Hz​ (atto =10−18=10^{-18}=10−18) through coupling of micro or nanofabricated mechanical resonators to a variety of physical systems including single-electron transistors, superconducting microwave cavities, and individual spins. These experiments have allowed for probing studies of a variety of phenomena, but sensitivity requirements are ever-increasing as new regimes of physical interactions are considered. Here we show that trapped atomic ions are exquisitely sensitive force detectors, with a measured sensitivity more than three orders of magnitude better than existing reports. We demonstrate detection of forces as small as 174 yNyNyN (yocto =10−24=10^{-24}=10−24), with a sensitivity 390±150\pm150±150 yN/HzyN/\sqrt{Hz}yN/Hz​ using crystals of n=60n=60n=60 9^{9}9Be+^{+}+ ions in a Penning trap. Our technique is based on the excitation of normal motional modes in an ion trap by externally applied electric fields, detection via and phase-coherent Doppler velocimetry, which allows for the discrimination of ion motion with amplitudes on the scale of nanometers. These experimental results and extracted force-detection sensitivities in the single-ion limit validate proposals suggesting that trapped atomic ions are capable of detecting of forces with sensitivity approaching 1 yN/HzyN/\sqrt{Hz}yN/Hz​. We anticipate that this demonstration will be strongly motivational for the development of a new class of deployable trapped-ion-based sensors, and will permit scientists to access new regimes in materials science.
We report phase-coherent Doppler detection of optical dipole forces using large ion crystals in a Penning trap. The technique is based on laser Doppler velocimetry using a cycling transition in 9Be+ near 313 nm and the center-of-mass (COM) ion motional mode. The optical dipole force is tuned to excite the COM mode, and measurements of photon arrival times synchronized with the excitation potential show oscillations with a period commensurate with the COM motional frequency. Experimental results compare well with a quantitative model for a driven harmonic oscillator. This technique permits characterization of motional modes in ion crystals; the measurement of both frequency and phase information relative to the driving force is a key enabling capability--comparable to lockin detection - providing access to a parameter that is typically not available in time-averaged measurements. This additional information facilitates discrimination of nearly degenerate motional modes.
Mechano-optical transducers are devices that convert a force or displacement signal to an optical one, enabling ultrasensitive mechanical detection. Currently, ultraweak DC force sensors with high spatial resolution are in high demand for the search of possible exotic spin-dependent interactions beyond the standard model in sub-millimeter scale. Here, we demonstrate a mechano-optical transducer of a single trapped ion with the force sensitivity about 600 zN/Hz for the DC force. This method utilizes the Doppler shift of the time-resolved fluorescence to detect the ion's micromotion that is coupled to a vector force. By alternating the directions of the detection laser beams, the vector DC forces can be precisely measured. Such a mechano-optical transducer provides sub-attonewton sensitivity with the spatial resolution in single-atom level, enabling various uses for both scientific and industrial purposes.
In traditional mechanics, harmonic oscillators can be used to measure force, acceleration, or rotation. Herein, we describe a quantum harmonic oscillator based on a Penning-trapped calcium ion crystal. Similar to traditional oscillators, the Coriolis force-induced axial oscillation amplitude is precisely measured to determine the input velocity. We show that the magnetron motion can be controlled through the rotating wall driving and treated as the driving oscillator. The Coriolis force couples with the magnetron motion and induces vibration in the axial direction or the z direction. The center of mass motion of the ion crystal in the axial direction could be precisely detected by the entanglement between the spins of the ions and the harmonic motion through lasers. The frequency of the magnetron motion needs to meet that of the axial motion under certain conditions, and, thus, the axial motion could be tuned to the resonance peak for maximum detection signal. We provided the parameter spaces for the matching of the magnetron frequencies with those of the axial frequencies. The measurement sensitivity was calculated in detail, and results show that a rotation angular velocity of 3.0×10−9rad/s/Hz could be achieved with 10 000 ions. Amplitude sensing could reach a sensitivity of 0.4 pm/Hz. With spin squeezing, the sensitivity could be further improved.
We present a technique to measure the amplitude of a center-of-mass (c.m.) motion of a two-dimensional ion crystal of ∼100 ions. By sensing motion at frequencies far from the c.m. resonance frequency, we experimentally determine the technique's measurement imprecision. We resolve amplitudes as small as 50 pm, 40 times smaller than the c.m. mode zero-point fluctuations. The technique employs a spin-dependent, optical-dipole force to couple the mechanical oscillation to the electron spins of the trapped ions, enabling a measurement of one quadrature of the c.m. motion through a readout of the spin state. We demonstrate sensitivity limits set by spin projection noise and spin decoherence due to off-resonant light scattering. When performed on resonance with the c.m. mode frequency, the technique demonstrated here can enable the detection of extremely weak forces (<1 yN) and electric fields (<1 nV/m), providing an opportunity to probe quantum sensing limits and search for physics beyond the standard model.
Detection of the weakest forces in nature is aided by increasingly sensitive measurements of the motion of mechanical oscillators. However, the attainable knowledge of an oscillator's motion is limited by quantum fluctuations that exist even if the oscillator is in its lowest possible energy state. We demonstrate a technique for amplifying coherent displacements of a mechanical oscillator with initial magnitudes well below these zero-point fluctuations. When applying two orthogonal squeezing interactions, one before and one after a small displacement, the displacement is amplified, ideally with no added quantum noise. We implemented this protocol with a trapped-ion mechanical oscillator and determined an increase by a factor of up to 7.3 (±0.3) in sensitivity to small displacements.