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arXiv:1601.05642

Quantum fluctuation theorem for dissipative cyclotron motion

G. S. Agarwal, Sushanta Dattagupta

Published Jan 21, 2016• 2 citations
arXivHTMLPDF

Abstract

We examine the fluctuation theorems which traditionally have been studied for classical systems and enquire if they can be extended to the quantum domain, especially at low temperatures. The example chosen is that of a problem which has proven to be of great interest in the context of Landau diamagnetism viz. the quantized motion of an electron in a magnetic field and in a dissipative environment. It is established from first principles that the quantum work operator W has a Gaussian distribution even though the system under consideration has a four dimensional phase space. The parameter $α$ in the fluctuation theorem $p(W )/p(-W) = exp(αW)$ depends on the system dynamics and has characteristic quantum features, especially at low temperatures. Certain unique low temperature signatures are also discussed.

DOI
10.48550/arxiv.1601.05642

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We examine the fluctuation theorems which traditionally have been studied for classical systems and enquire if they can be extended to the quantum domain, especially at low temperatures. The example chosen is that of a problem which has proven to be of great interest in the context of Landau diamagnetism viz. the quantized motion of an electron in a magnetic field and in a dissipative environment. It is established from first principles that the quantum work operator W has a Gaussian distribution even though the system under consideration has a four dimensional phase space. The parameter ααα in the fluctuation theorem p(W)/p(−W)=exp(αW)p(W )/p(-W) = exp(αW)p(W)/p(−W)=exp(αW) depends on the system dynamics and has characteristic quantum features, especially at low temperatures. Certain unique low temperature signatures are also discussed.
Starting from a quantum Langevin equation (QLE) of a charged particle coupled to a heat bath in the presence of an external magnetic field, we present a fully dynamical calculation of the susceptibility tensor. In a different ‘equilibrium approach’, we further evaluate the position autocorrelation function by using the Gibbs ensemble. This quantity is shown to be related to the imaginary part of the dynamical susceptibility, thereby validating the fluctuation–dissipation theorem in the context of dissipative diamagnetism. Finally, we present an overview of coherence-to-decoherence transition in the realm of dissipative diamagnetism at zero temperature. The analysis underscores the importance of the details of the relevant physical quantity, as far as coherence-to-decoherence transition is concerned.
We explore some aspects of nonequilibrium statistical mechanics of classical and quantum systems. Two chapters are devoted to fluctuation theorems which were originally derived for classical systems. The main challenge in formulating them in quantum mechanics is the fact that fundamental quantities of interest, like work, are defined via the classical concept of a phase space trajectory. We utilize the decoherent histories conceptual framework, in which classical trajectories emerge in quantum mechanics as a result of coarse graining, and provide a first-principles analysis of the nonequilibrium work relation of Jarzynski and Crooks's fluctuation theorem for a quantum system interacting with a general environment based on the quantum Brownian motion (QBM) model. We indicate a parameter range at low temperatures where the theorems might fail in their original form. Fluctuation theorems of Jarzynski and Crooks for systems obeying classical Hamiltonian dynamics are derived under the assumption that the initial conditions are sampled from a canonical ensemble, even though the equilibrium state of an isolated system is typically associated with the microcanonical ensemble. We address this issue through an exact analysis of the classical Brownian motion model. We argue that a stronger form of ensemble equivalence than usually discussed in equilibrium statistical mechanics is required for these theorems to hold in the infinite environment limit irrespective of the ensemble used, and proceed to prove it for this model. An exact expression for the probability distribution of work is obtained for finite environments. Intuitively one expects a system to relax to an equilibrium state when brought into contact with a thermal environment. Yet it is important to have rigorous results that provide conditions for equilibration and characterize the equilibrium state. We consider the dynamics of open quantum systems using the Langevin and master equations and rigorously show that under fairly general conditions quantum systems interacting with a heat bath relax to the equilibrium state defined as the reduced thermal state of the system plus environment, even in the strong coupling regime. Our proof is valid to second-order in interaction strength for general systems and exact for the linear QBM model, for which we also show the equivalence of multi-time correlations. In the final chapter we give a sampling of our investigations into macroscopic quantum phenomena. We work out in detail a specific example of how and under what conditions the center of mass (CoM) coordinate of a macroscopic object emerges as the relevant degree of freedom. Interaction patterns are studied in terms of the couplings they induce between the CoM and relative coordinates of two macroscopic objects. We discuss the implications of these interaction patterns on macroscopic entanglement.
At non-zero temperature classical systems exhibit statistical fluctuations of thermodynamic quantities arising from the variation of the system's initial conditions and its interaction with the environment. The fluctuating work, for example, is characterised by the ensemble of system trajectories in phase space and, by including the probabilities for various trajectories to occur, a work distribution can be constructed. However, without phase space trajectories, the task of constructing a work probability distribution in the quantum regime has proven elusive. Here we use quantum trajectories in phase space and define fluctuating work as power integrated along the trajectories, in complete analogy to classical statistical physics. The resulting work probability distribution is valid for any quantum evolution, including cases with coherences in the energy basis. We demonstrate the quantum work probability distribution and its properties with an exactly solvable example of a driven quantum harmonic oscillator. An important feature of the work distribution is its dependence on the initial statistical mixture of pure states, which is reflected in higher moments of the work. The proposed approach introduces a fundamentally different perspective on quantum thermodynamics, allowing full thermodynamic characterisation of the dynamics of quantum systems, including the measurement process.
Abstract This review provides a brief and quick introduction to the quantum Langevin equation for an oscillator, while focusing on the steady-state thermodynamic aspects. A derivation of the quantum Langevin equation is carefully outlined based on the microscopic model of the heat bath as a collection of a large number of independent quantum oscillators, the so-called independent-oscillator model. This is followed by a discussion on the relevant ‘weak-coupling’ limit. In the steady state, we analyze the quantum counterpart of energy equipartition theorem which has generated a considerable amount of interest in recent literature. The free energy, entropy, specific heat, and third law of thermodynamics are discussed for one-dimensional quantum Brownian motion in a harmonic well. Following this, we explore some aspects of dissipative diamagnetism in the context of quantum Brownian oscillators, emphasizing upon the role of confining potentials and also upon the environment-induced classical-quantum crossover. We discuss situations where the system-bath coupling is via the momentum variables by focusing on a gauge-invariant model of momentum-momentum coupling in the presence of a vector potential; for this problem, we derive the quantum Langevin equation and discuss quantum thermodynamic functions. Finally, the topic of fluctuation theorems is discussed (albeit, briefly) in the context of classical and quantum cyclotron motion of a particle coupled to a heat bath.
We present a detailed study of the quantum dissipative dynamics of a charged particle in a magnetic field. Our focus of attention is the effect of dissipation on the low- and high-temperature behaviors of the specific heat at constant volume. After providing a brief overview of two distinct approaches to the statistical mechanics of dissipative quantum systems, viz., the ensemble approach of Gibbs and the quantum Brownian motion approach due to Einstein, we present exact analyses of the specific heat. While the low-temperature expressions for the specific heat, based on the two approaches, are in conformity with power-law temperature dependence, predicted by the third law of thermodynamics, and the high-temperature expressions are in agreement with the classical equipartition theorem, there are surprising differences between the dependencies of the specific heat on different parameters in the theory, when calculations are done from these two distinct methods. In particular, we find puzzling influences of boundary confinement and the bath-induced spectral cutoff frequency. Further, when it comes to the issue of approach to equilibrium, based on the Einstein method, the way the asymptotic limit (t-->infinity) is taken seems to assume significance.
The Schrodinger equation with Gaussian dynamic fluctuating potentials is considered. This model gives a convenient example of an open quantum system coupled to a given external environment. The evolution equations for averaged correlators are derived and it is shown that a system coupled to a thermoequilibrium environment tends asymptotically with time to a thermodynamic density matrix. At high temperatures the quantum evolution equation for the density matrix can be approximated by the quasiclassical Fokker-Planck equation. The generalisation for multiparticle systems is also given. The results are illustrated by the particular examples of coupling with phonons and of two-level systems. Finally, it is shown how the problem can be reformulated in terms of continuous stochastic evolution in the space of psi functions and a corresponding functional formalism based on the continuous Fokker-Planck equation in the space of psi functions.