We point out and explicitly demonstrate a close connection that exists between featureless Mott insulators and fractional quantum Hall liquids. Using magnetic Wannier states as the single-particle basis in the lowest Landau level (LLL), we demonstrate that the Hamiltonian of interacting bosons in the LLL maps onto a Hamiltonian of a featureless Mott insulator on triangular lattice, formed by the magnetic Wannier states. The Hamiltonian is remarkably simple and consists only of short-range repulsion and ring-exchange terms.
A number of lattices exhibit moat-like band structures, i.e. a band with infinitely degenerate energy minima attained along a closed line in the Brillouin zone. If such a lattice is populated with hard-core bosons, the degeneracy prevents their condensation. At half-filling, the system is equivalent to
s=1/2 XY model at zero magnetic field, while absence of condensation translates into the absence of magnetic order in the XY plane. Here we show that the ground state breaks the time-reversal as well as inversion symmetries. This state, which may be identified with the chiral spin liquid, has a bulk gap and chiral gapless edge excitations. The applications of the developed analytical theory include an explanation of recent numerical findings and a suggestion for the chiral spin liquid realizations in experiments with cold atoms in optical lattices.
A number of lattices exhibit moatlike band structures, i.e., a band with infinitely degenerate energy minima attained along a closed line in the Brillouin zone. If such a lattice is populated with hard-core bosons, the degeneracy prevents their condensation. At half-filling, the system is equivalent to the s=1/2 XY model at a zero magnetic field, while the absence of condensation translates into the absence of magnetic order in the XY plane. Here, we show that the ground state breaks time reversal as well as inversion symmetries. This state, which may be identified with the chiral spin liquid, has a bulk gap and chiral gapless edge excitations. The applications of the developed analytical theory include an explanation of recent numerical findings and a suggestion for the chiral spin liquid realizations in experiments with cold atoms in optical lattices.
Frustrated magnetism provides a rich platform for realizing exotic quantum phases in condensed matter systems. Among these, quantum spin liquids (QSLs) are a particularly intriguing class of states that exhibit no magnetic ordering and preserve all symmetries down to zero temperature. Just as conventional magnets can be thought of as spin crystals,QSLs represent their liquid analogs. This thesis explores two broad types of QSLs in two-dimensional magnets, with a focus on their dynamic properties and the nature of transitions from conventional magnetic states into QSL phases. QSLs are topological phases that host fractionalized excitations known as spinons. In these states, mobile spinons are coupled to an emergent gauge field, forming a highly entangled phase of matter. The first part of this thesis focuses on Dirac spin liquids (DSLs), a class of QSLs where spinons exhibit a gapless Dirac dispersion. To study the dynamicsof these spin liquids beyond leading-order mean-field theory, we develop a novel large-N fermionic limit of gapless spinons. In this limit, all gauge excitations are suppressed, and the leading-order corrections instead arise from order parameter fluctuations, which may condense and drive transitions into symmetry-broken phases from the parent DSL. Incorporating random phase approximation (RPA) corrections to the spin susceptibility, we find that sharp, spin-wave–like modes are recovered in the excitation spectrum. This methodology successfully captures characteristic features of the dynamics near phase transitions and in weakly symmetry-broken phases proximate to a DSL. We apply this approach to microscopic models, including the J1-J2 XXZ model on the triangular lattice and the J1-J3 XXZ model on the honeycomb lattice. These models closely represent a wide range of frustrated materials, such as triangular and honeycomb cobaltates and triangular ytterbium compounds. Our theoretical predictions show excellent agreement with experimentally measured inelastic neutron scattering spectra from these materials. Gapless spinons can also sometimes become gapped through chiral symmetry breaking, leading to the formation of a chiral spin liquid (CSL). The CSL is an archetypal bosonic realization of a fractional quantum Hall (FQH) state at half-filling, and has been proposed as a time-reversal–breaking ground state in a variety of frustrated spin models. The second part of this thesis addresses the intriguing possibility of realizing a CSL through the "melting" of a chiral spin crystal—a conventional magnet with non-coplanar ordering. Such a transition offers a physically appealing analogue to the melting of a Wigner crystal into a fermionic FQH liquid. Focusing on the kagome lattice, where chiral interactions are knownto stabilize a CSL ground state, we study the effects of additional long-range Heisenberg interactions and demonstrate a phase transition into a non-coplanar octahedral magnetic order. To describe the universal class of transition between a CSL and a non-coplanar anti-ferromagnetic order, we then develop a novel Chern-Simons–matter field theory framework, constrained by symmetry principles and symmetry fractionalization patterns. This thesis thus provides new insights into the dynamical signatures and phase transitions of quantum spin liquids, offering a bridge between theoretical models and experimental observations in frustrated magnetic systems.
In the physics of the fractional quantum Hall (FQH) effect, a zoo of Abelian topological phases can be obtained by varying the magnetic field. Aiming to reach the same phenomenology in spin like systems, we propose a family of
SU(N)-symmetric models in the fundamental representation, on the square lattice with short-range interactions restricted to triangular units, a natural generalization for arbitrary
N of an SU(3) model studied previously where time-reversal symmetry is broken explicitly. Guided by the recent discovery of
SU(2)1 and
SU(3)1 chiral spin liquids (CSL) on similar models we search for topological
SU(N)1 CSL in some range of the Hamiltonian parameters via a combination of complementary numerical methods such as exact diagonalizations (ED), infinite density matrix renormalization group (iDMRG) and infinite Projected Entangled Pair State (iPEPS). Extensive ED on small (periodic and open) clusters up to
N=10 and an innovative
SU(N)-symmetric version of iDMRG to compute entanglement spectra on (infinitely long) cylinders in all topological sectors provide unambiguous signatures of the
SU(N)1 character of the chiral liquids. An SU(4)-symmetric chiral PEPS, constructed in a manner similar to its SU(2) and SU(3) analogs, is shown to give a good variational ansatz of the
N=4 ground state, with chiral edge modes originating from the PEPS holographic bulk-edge correspondence. Finally, we discuss the possible observation of such Abelian CSL in ultracold atom setups where the possibility of varying
N provides a tuning parameter similar to the magnetic field in the physics of the FQH effect.
Despite rapid progress in understanding gapped topological states, much less is known about gapless topological phases of matter, especially in strongly correlated electrons. In this work, we discuss a large class of robust gapless quantum spin liquids in frustrated magnets made of half-integer spins, which are described by gapless fermionic spinons coupled to dynamical
Z2 gauge fields. Requiring
U(1) spin conservation, time-reversal, and certain space-group symmetries, we show that certain spinon symmetry fractionalization class necessarily leads to a gapless spectrum. These gapless excitations are stable against any perturbations, as long as the required symmetries are preserved. Applying these gapless criteria to spin-
21 systems on square, triangular, and kagome lattices, we show that all gapped symmetric
Z2 spin liquids in Abrikosov-fermion representation can also be realized in Schwinger-boson representation. This leads to 64 gapped
Z2 spin liquids on square lattice, and 8 gapped states on both kagome and triangular lattices.