We investigate the quantum dynamics of a generic model of light-matter interaction in the context of high-impedance waveguides, focusing on the behavior of the photonic states generated in the waveguide. The model treated consists simply of a two-level system coupled to a bosonic bath (the Ohmic spin-boson model). Quantum quenches as well as scattering of an incident coherent pulse are studied using two complementary methods. First, we develop an approximate ansatz for the electromagnetic waves based on a single multimode coherent state wave function; formally, this approach combines in a single framework ideas from adiabatic renormalization, the Born-Markov approximation, and input-output theory. Second, we present numerically exact results for scattering of a weak intensity pulse by using numerical renormalization group (NRG) calculations. NRG provides a benchmark for any linear response property throughout the ultrastrong-coupling regime. We find that in a sudden quantum quench, the coherent state approach produces physical artifacts, such as improper relaxation to the steady state. These previously unnoticed problems are related to the simplified form of the ansatz that generates spurious correlations within the bath. In the scattering problem, NRG is used to find the transmission and reflection of a single photon, as well as the inelastic scattering of that single photon. Simple analytical formulas are established and tested against the NRG data that predict quantitatively the transport coefficients for up to moderate environmental impedance. These formulas resolve pending issues regarding the presence of inelastic losses in the spin-boson model near absorption resonances, and could be used for comparison to experiments in Josephson waveguide quantum electrodynamics. Finally, the scattering results using the coherent state wave-function approach are compared favorably to the NRG results for very weak incident intensity. We end our study by presenting results at higher power where the response of the system is nonlinear.
We investigate the quantum dynamics of a generic model of light-matter interaction in the context of high-impedance waveguides, focusing on the behavior of the photonic states generated in the waveguide. The model treated consists simply of a two-level system coupled to a bosonic bath (the Ohmic spin-boson model). Quantum quenches as well as scattering of an incident coherent pulse are studied using two complementary methods. First, we develop an approximate ansatz for the electromagnetic waves based on a single multimode coherent state wave function; formally, this approach combines in a single framework ideas from adiabatic renormalization, the Born-Markov approximation, and input-output theory. Second, we present numerically exact results for scattering of a weak intensity pulse by using numerical renormalization group (NRG) calculations. NRG provides a benchmark for any linear response property throughout the ultrastrong-coupling regime. We find that in a sudden quantum quench, the coherent state approach produces physical artifacts, such as improper relaxation to the steady state. These previously unnoticed problems are related to the simplified form of the ansatz that generates spurious correlations within the bath. In the scattering problem, NRG is used to find the transmission and reflection of a single photon, as well as the inelastic scattering of that single photon. Simple analytical formulas are established and tested against the NRG data that predict quantitatively the transport coefficients for up to moderate environmental impedance. These formulas resolve pending issues regarding the presence of inelastic losses in the spin-boson model near absorption resonances, and could be used for comparison to experiments in Josephson waveguide quantum electrodynamics. Finally, the scattering results using the coherent state wave-function approach are compared favorably to the NRG results for very weak incident intensity. We end our study by presenting results at higher power where the response of the system is nonlinear.
We study the strong coupling dynamics as well as transport properties of photons in the two-bath spin-boson model, in which a spin-1/2 particle is frustratingly coupled to two independent Ohmic bosonic baths. Using a combination of numerical and analytical methods, we show that the frustration in this model gives rise to rich physics in a very wide range of energies. This is in contrast to the one-bath spin-boson model, where the non-trivial physics occurs at an energy scale close to the renormalized spin frequency. The renormalized spin frequency in the two-bath spin-boson model is still important, featuring in different observables, including the non-equiblirum dynamics of both the spin and the baths along with the elastic transport properties of a photon. The latter however reveals a much more complex structure. The elastic scattering displays non-monotonic behavior at high frequencies, and is very different in the two channels: intra- and inter-bath scattering. The photon can also be inelastically scattered, a process in which it is split into several photons of smaller energies. We show that such inelastic processes are highly anisotropic, with the outgoing particles being preferentially emitted into only one of the baths. Moreover, the inelastic scattering rate is parameterically larger than in the one-bath case, and can even exceed the total elastic rate. Our results can be verified with state-of-the-art circuit and cavity quantum electrodynamics experiments.
We develop a semianalytical approach beyond the Born-Markov approximation to study the quench dynamics of the spin-boson model in the strong-coupling regime ($\ensuremath{\alpha}\ensuremath{\le}1/2$) for the Ohmic bath. The basic idea in our approach is to write an effective time-dependent model for the dynamics of the system coupled to the bosonic bath after integrating out high-frequency bath modes. By applying this procedure to the Heisenberg equations of motion, we derive a set of flow equations for the system parameters as a function of time. The final flow equations look similar to those of the equilibrium renormalization-group theory; however, in our derivation the scaling parameter is set by the real time. We solve the equations of motion with time-dependent renormalized parameters and show that the resulting dynamics is in decent agreement with the exact NRG calculations as well as the noninteracting blip approximation that is a well-known good solution in this limit.
Starting from the paradigmatic spin-boson model (SBM), we investigate the static and dynamical properties of a system of two distant two-level emitters coupled to a one-dimensional Ohmic waveguide beyond the rotating wave approximation. Employing static and dynamical polaron Ans\"atze we study the effects of finite separation distance on the behavior of the photon-mediated Ising-like interaction, qubit frequency renormalization, ground-state magnetization, and entanglement entropy of the two-qubit system. Based on previous works we derive an effective approximate Hamiltonian for the two-impurity SBM that preserves the excitation-number and thus facilitates the analytical treatment. In particular, it allows us to introduce non-Markovianity arising from delay-feedback effects in two distant emitters in the so-called ultrastrong coupling (USC) regime. We test our results with numerical simulations performed over a discretized circuit-QED model, finding perfect agreement with previous results, and showing interesting dynamical effects arising in ultrastrong waveguide QED with distant emitters. In particular, we revisit the Fermi two-atom problem showing that, in the USC regime, initial correlations yield two different evolutions for symmetric and antisymmetric states even before the emitters become causally connected. Finally, we demonstrate that the collective dynamics, e.g., superradiance or subradiance, are affected not only by the distance between emitters, but also by the coupling, due to significant frequency renormalization. This constitutes another dynamical consequence of the USC regime.
The study of waveguide-QED systems, where a continuum of quantum field modes is coupled to qubits or two-level systems, has improved our ability to manipulate quantum light-matter interactions on chip. In the typical theoretical approaches to waveguide QED, there are a few necessary approximations, e.g., considering the system in the weak excitation regime, or treating the waveguide as a bath. However, these inherent approximations can break down with short pulse excitation. Here, we investigate the few-photon quantum nonlinear response of chiral qubits, when excited with one and two-photon Fock states. Our theory uses a numerically exact approach, based on Matrix Product States, avoiding the limitations of the usual waveguide-QED approximations. Using a chiral-emitter waveguide system, we show explicitly the breakdown of the weak excitation approximation, and study the single and two-photon nonlinear responses. We demonstrate the impact on the qubit population, and discuss how the phase change can be examined from the photon quantum correlation functions, seeing a radical departure from scattering theory solutions.
Waveguide circuit quantum electrodynamics (waveguide circuit QED) studies light-matter interaction with superconducting circuits in one dimension. In circuit QED, natural atoms are replaced by superconducting qubits consisting of a non-linear Josephson junction, resulting in an anharmonic energy spectrum just like real atoms. With superconducting qubits, it is possible to study quantum optical phenomena and reach new regimes hard to achieve with real atoms due to weak coupling to the electromagnetic field. The reduction to one dimension in waveguide QED increases the electromagnetic field's directionality, which results in reduced losses. In this thesis, we first introduce circuit quantisation, giving the basis for the next part, where we investigate a transmon, a charge-insensitive artificial atom, coupled to a semi-infinite transmission line. An atom coupled to a semi-infinite waveguide is referred to as an atom in front of a mirror and is the subject of all appended papers. We proceed by summarising Paper I and III's main results: in Paper I, we investigate the spontaneous emission of a transmon coupled to a semi-infinite transmission line, where we take time-delay effects into account. We find that the system dynamics strongly depend on the coupling strength to the transmission line and the atom's position with respect to the electromagnetic field, leading to the Purcell effect or the convergence to a dark state with finite excitation probability. In the high-impedance regime, which we investigate in Paper III, the properties of the transmon coupled to the high-impedance transmission line change drastically. It becomes highly reflective and creates its own cavity with the mirror, resulting in the emergence of cavity modes and vacuum Rabi oscillations in the spontaneous emission dynamics. In the next chapter of the thesis, we demonstrate how to quantise an electromagnetic field and derive a light-matter interaction Hamiltonian within dipole approximation. We then give an introduction to open quantum systems and derive the quantum-optical master equation in Lindblad form. Furthermore, we introduce the dressed state picture, where the interaction of light and matter is so strong that the individual energy levels of light and matter are no longer separable. Both the quantum optical master equation and the dressed state picture are relevant in Paper II and IV. In Paper II, an experimental collaboration, we perform several experiments to characterise and discriminate different decay rates of a superconducting qubit coupled to the end of a transmission line. One experiment measured the atomic fluorescence spectral density, which shows an asymmetry for off-resonant driving, resulting from pure dephasing: an effect that we explain in more detail in this thesis and Paper II. In Paper IV, we theoretically investigate amplification mechanisms realised by different set-ups of an atom coupled to a semi-infinite waveguide. In the considered systems, the amplification of a probe field happens either due to population inversion between the pure states or dressed states or multi-photon processes. We find that compared to an open waveguide, we can achieve a higher gain in the amplification with a semi-infinite waveguide.
We have studied the characteristic feature of coherent photon transport in a semiconductor waveguide. We have presented a semiconductor master equation formalism that accurately simulated coherent input or output coupling of semiconductor cavity quantum electrodynamics systems such as planar photonic crystals and micropillar cavities. The role of quantized multiphoton effects pointed out the possible failure of weak excitation approximation, which was found to fail even for low input powers and small mean cavity photon numbers. For increasing field strengths, possible failure of the semiclassical approach was taken into account. In the weak coupling regime, higher order quantum correlation effects, were shown to be significant. We have introduced the general theoretical technique to simulate coherent photon transport outside both the weak excitation approximation and the semi classical approximation. Electron-phonon interactions at a microscopic level were derived using polaron transformation. We have demonstrated that substantial deviations from the weak excitation approximation resulted for very small mean photon numbers. We have modified the master equation approach to include the mechanism of electron-acoustic scattering and studied the impact of electron-phonon interaction on incoherent scattering and coherent renormalization of the exciton cavity coupling rate, qualitative differences from simple Lorentzian decay model containing quantum dot were found. We have also studied the transmission of light in the strong coupling regime and simulated a phase gate. We have found that coupling to an acoustic phonon bath caused considerable qualitative changes in light propagation characteristics modeled by a simple pure dephasing process. We have used the model to simulate a conditional phasegate. The obtained results were found in good agreement with previously obtained results.