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arXiv:1512.05677 · Journal of Physics Conference Series

Evaluation of trap-induced systematic frequency shifts for a multi-ion optical clock at the 10−19level

Jonas Keller, T. Burgermeister, Dimitri Kalincev, J. Kiethe, T. E. Mehlstäubler

Published Jun 1, 2016• 29 citations
arXivHTMLPDF

Abstract

In order to improve the short-term stability of trapped-ion optical clocks, we are developing a frequency standard based on 115 In + / 172 Yb + Coulomb crystals. For this purpose, we have developed scalable segmented Paul traps which allow a high level of control for multiple ion ensembles. In this article, we detail on our recent results regarding the reduction of the leading sources of frequency uncertainty introduced by the ion trap: 2nd-order Doppler shifts due to micromotion and the heating of secular motion, as well as the black-body radiation shift due to warming of the trap. We show that the fractional frequency uncertainty due to each of these effects can be reduced to well below 10 -19 .

DOI
10.1088/1742-6596/723/1/012027

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In order to improve the short-term stability of trapped-ion optical clocks, we are developing a frequency standard based on 115 In + / 172 Yb + Coulomb crystals. For this purpose, we have developed scalable segmented Paul traps which allow a high level of control for multiple ion ensembles. In this article, we detail on our recent results regarding the reduction of the leading sources of frequency uncertainty introduced by the ion trap: 2nd-order Doppler shifts due to micromotion and the heating of secular motion, as well as the black-body radiation shift due to warming of the trap. We show that the fractional frequency uncertainty due to each of these effects can be reduced to well below 10 -19 .
We report on the design of a segmented linear Paul trap for optical clock applications using trapped ion Coulomb crystals. For an optical clock with an improved short-term stability and a fractional frequency uncertainty of 10−18, we propose 115In+ ions sympathetically cooled by 172Yb+. We discuss the systematic frequency shifts of such a frequency standard. In particular, we elaborate on high-precision calculations of the electric radiofrequency field of the ion trap using the finite element method. These calculations are used to find a scalable design with minimized excess micromotion of the ions at a level at which the corresponding second-order Doppler shift contributes less than 10−18 to the relative uncertainty of the frequency standard.
Single ion frequency standards have demonstrated in several experiments excellent results and are approaching fractional frequency uncertainties of 10^-18. As dominant contributions to the uncertainty are linked to the ion trap properties a further reduction would be possible by an improved ion trap. Due to the interrogation of a single ion these frequency standards are currently limited by the intrinsically low signal-to-noise ratio and require long averaging times on the order of several days. This limitation is critical for various applications that require a high frequency resolution on short timescales. One possibility to improve the clock stability is to increase the number of clock ions. However, this approach further increases the requirements for the ion trap. Therefore, for the realization of a multi-ion clock that aims at simultaneously reducing the frequency stability and uncertainty the control over the characteristics of the ion trap is crucial. This thesis continues previous work towards the realization of a multi-ion optical clock based on ion Coulomb crystals of 115In+ ions which are sympathetically cooled by 172Yb+ ions. The existing design for a segmented linear ion trap has been refined and a reliable trap manufacturing process for a trap based on gold coated aluminium nitride wafers has been developed. Manufacturing tolerances below 10 μm allowed to reduce the axial micromotion amplitudes substantially. For a region of more than 300 μm the uncertainty contribution of the three-dimensional micromotion amplitude is shown to be below 10^-19. Additionally the radial ion heating rate of the trap has been measured to be 1.1 phonons/s for a trap frequency of 490 kHz. The time dilation shift due to the heating rate on the radial trap axis is found to be (2.1 ± 0.3) x 10^-20 1/s. The trap design has also been optimized for a low trap temperature rise due to the applied rf voltage. Trap temperature measurements with Pt100 sensors installed on the trap showed a maximum temperature increase of 1.21 K at an rf voltage amplitude of 1 kV. By comparing the measurement results to FEM simulations the uncertainty contribution of the trap temperature to the black-body radiation shift has been deduced to be 2.4 x 10^-20. As the ion trap provides a high level of control on Coulomb crystals it also provides an ideal test bed for studying atomic many-body systems. This work presents results of the investigations on topological defects in two-dimensional Coulomb crystals. The emphasis was placed on the effects of mass defects and external electric fields on the stability of the topological defects. It is shown that these effects can be used to manipulate and create topological defects deterministically.
Trapped-ion optical clocks are capable of achieving systematic fractional frequency uncertainties of 10−1810^{-18}10−18 and possibly below. However, the stability of current ion clocks is fundamentally limited by the weak signal of single-ion interrogation. We present an operational, versatile platform for extending clock spectroscopy to arrays of Coulomb crystals consisting of several tens of ions, while allowing systematic shifts as low as 10−1910^{-19}10−19. The concept is applicable to all clock transitions with low differential electric quadrupole moments. We observe 3D excess micromotion amplitudes of all individual ions inside a Coulomb crystal with nm resolution and prove that the related frequency shifts can be controlled simultaneously at the 10−1910^{-19}10−19 level. Using this method, we demonstrate regions of 400400400 μ\muμm and 222 mm length in our trap array with time dilation shifts due to micromotion close to 1×10−191\times10^{-19}1×10−19 and below 10−1810^{-18}10−18, respectively. Further measurements of the trapping environment and cooling dynamics calculations for mixed In+{}^++ / Yb+{}^++ crystals show that achievable clock uncertainties due to multi-ion operation in our setup are below 1×10−191\times10^{-19}1×10−19. This work will enable clock operation with multiple ions and open up the possibility of new interrogation schemes which allow optical clock stabilities beyond classical limits.
As relative systematic frequency uncertainties in trapped-ion spectroscopy are approaching the low 10−18 range, motional frequency shifts account for a considerable fraction of the uncertainty budget. Micromotion, a driven motion fundamentally connected to the principle of the Paul trap, is a particular concern in these systems. In this article, we experimentally investigate at this level three common methods for minimizing and determining the micromotion amplitude. We develop a generalized model for a quantitative application of the photon-correlation technique, which is applicable in the commonly encountered regime where the transition linewidth is comparable to the rf drive frequency. We show that a fractional frequency uncertainty due to the 2nd-order Doppler shift below |Δν/ν|=1×10−20 can be achieved. The quantitative evaluation is verified in an interleaved measurement with the conceptually simpler resolved sideband method. If not performed deep within the Lamb-Dicke regime, a temperature-dependent offset at the level of 10−19 is observed in resolved sideband measurements due to sampling of intrinsic micromotion. By direct comparison with photon-correlation measurements, we show that the simple to implement parametric heating method is sensitive to micromotion at the level of |Δν/ν|=1×10−20 as well.
We recently reported a 5×10-17level frequency comparison of two40Ca+optical clocks, one of which has fractional frequency uncertainty of 3.4×10-17, limited by the BBR effect. Here we present progress towards a40Ca+optical clock with uncertainty at the 10-18level. The differential static scalar polarizability Δα0 of the40Ca+ion clock transition is obtained by precisely measuring the “magic” rf drive frequency. Δα0 is measured as -7.2653(44)x10-40J m2/V2, the blackbody radiation shift is then calculated to be 0.3790(2) Hz at 300 K. The contribution of the blackbody shift coefficient to the uncertainty of the optical clock at room temperature is reduced to 5.6×10-19, the excess micromotion induced clock uncertainty is also reduced to the 10-19level by choosing the appropriate trap drive frequency. With a suppression of the BBR field temperature uncertainty to the sub-Kelvin level and improved clock stability, a robust, relatively low-cost40Ca+ion clock with uncertainty at 10-18level can be made.
An overview of the key methods used to reduce the uncertainty of the systematic shifts of the strontium ion optical frequency standard is presented. An uncertainty of 10 mHz at a clock frequency of 445 THz is obtained, limited by the uncertainty of the blackbody radiation shift. The uncertainty estimates of other shifts such as micromotion and electric quadrupole shifts are on the order of 1 mHz or less. The effectiveness of the methods used to reduce or cancel the shifts is illustrated with experiments comparing two ion traps. One has strong micromotion levels while the other, the reference trap, provides good control over the shifts. Despite nominal shifts of 70 Hz in the trap with large micromotion levels, the agreement with the reference trap is at the sub-Hz level.