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arXiv:1512.02534 · Physical Review A

Lifetimes of metastable ion clouds in a Paul trap: Power-law scaling

Daniel Weiss, Yunseong Nam, R. Blümel

Published Apr 27, 2016• 5 citations
arXivHTMLPDF

Abstract

It is well known that ions stored in a Paul trap, one of the most versatile tools in atomic, molecular, and optical (AMO) physics, may undergo a transition from a disordered cloud state to a geometrically well-ordered crystalline state, the Wigner crystal. In this paper we predict that close to the transition, the average lifetime ${\overline{\ensuremath{\tau}}}_{m}$ of the metastable cloud follows a power law, ${\overline{\ensuremath{\tau}}}_{m}\ensuremath{\sim}{(\ensuremath{\gamma}\ensuremath{-}{\ensuremath{\gamma}}_{c})}^{\ensuremath{-}\ensuremath{\beta}}$, where ${\ensuremath{\gamma}}_{c}$ is the value of the damping constant at which the transition occurs. The exponent $\ensuremath{\beta}$ depends on the trap control parameter $q$, but is independent of both the number of particles $N$ stored in the trap and the trap control parameter $a$, which determines the shape (oblate, prolate, or spherical) of the ion cloud. In addition, we find that for given $a$ and $q, {\ensuremath{\gamma}}_{c}$ scales approximately like ${\ensuremath{\gamma}}_{c}=Cln[ln(N)]+D$ as a function of $N$, where $C$ and $D$ are constants. Our predictions may be tested experimentally with equipment already available at many AMO laboratories. In addition to their importance in AMO trap physics, we also discuss possible applications of our results to other periodically driven many-particle systems, such as, e.g., particle accelerator beams, and, based on our trap results, conjecture that power laws characterize the phase transition to the Wigner crystal in all such systems.

DOI
10.1103/physreva.93.043424

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It is well known that ions stored in a Paul trap, one of the most versatile tools in atomic, molecular, and optical (AMO) physics, may undergo a transition from a disordered cloud state to a geometrically well-ordered crystalline state, the Wigner crystal. In this paper we predict that close to the transition, the average lifetime \ensuremathτ‾m{\overline{\ensuremath{\tau}}}_{m}\ensuremathτ​m​ of the metastable cloud follows a power law, \ensuremathτ‾m\ensuremath∼(\ensuremathγ\ensuremath−\ensuremathγc)\ensuremath−\ensuremathβ{\overline{\ensuremath{\tau}}}_{m}\ensuremath{\sim}{(\ensuremath{\gamma}\ensuremath{-}{\ensuremath{\gamma}}_{c})}^{\ensuremath{-}\ensuremath{\beta}}\ensuremathτ​m​\ensuremath∼(\ensuremathγ\ensuremath−\ensuremathγc​)\ensuremath−\ensuremathβ, where \ensuremathγc{\ensuremath{\gamma}}_{c}\ensuremathγc​ is the value of the damping constant at which the transition occurs. The exponent \ensuremathβ\ensuremath{\beta}\ensuremathβ depends on the trap control parameter qqq, but is independent of both the number of particles NNN stored in the trap and the trap control parameter aaa, which determines the shape (oblate, prolate, or spherical) of the ion cloud. In addition, we find that for given aaa and q,\ensuremathγcq, {\ensuremath{\gamma}}_{c}q,\ensuremathγc​ scales approximately like \ensuremathγc=Cln[ln(N)]+D{\ensuremath{\gamma}}_{c}=Cln[ln(N)]+D\ensuremathγc​=Cln[ln(N)]+D as a function of NNN, where CCC and DDD are constants. Our predictions may be tested experimentally with equipment already available at many AMO laboratories. In addition to their importance in AMO trap physics, we also discuss possible applications of our results to other periodically driven many-particle systems, such as, e.g., particle accelerator beams, and, based on our trap results, conjecture that power laws characterize the phase transition to the Wigner crystal in all such systems.
Clouds of two to about fifty simultaneously stored, laser-cooled Mg+{\mathrm{Mg}}^{+}Mg+ ions in a Paul trap were observed in two phases, which are clearly distinguishable by their excitation spectra. Transitions between these phases can be induced either by a variation of the power of the laser radiation used to cool the ions or by a change of the size of the radio-frequency voltage applied to the trap. Transitions between a "crystalline" phase and a "gaseous" phase can be repeatedly observed by variation of the appropriate parameters. The two phases and the transitions between them have also been recorded by a photon-counting image system.
A charged-particle cloud in a Paul trap is a nonlinear system that exhibits deterministic heating, i.e., conversion of energy provided by the radio-frequency (rf) drive of the trap into the disordered, gaslike motions of the trapped particles. In the presence of weak damping clouds reach an equilibrium state in which heating and cooling balance. For large damping, a cloud may collapse into a crystal. While the rf heating power of a given cloud depends sensitively on its particle number, its equilibrium size, the damping, and the control parameters of the trap, we find that scaling the heating power of the cloud with respect to its associated Coulomb-decoupled, non-interacting-gas state, and its equilibrium size with respect to its crystal size, results in a single, universal heating curve, independent of particle number and trap control parameters.
Ca + ions confined as a cloud in a Paul trap were excited and cooled by radiation from two lasers, tuned to the 4s 2 S 1/2 − 4p 2 P 1/2 and 4p 2 P 1/2 − 3d 2 D 3/2 transitions. The strong fluorescence of these lines disappears when we excite the ions simultaneously by a third laser on the 3d 2 D 3/2 − 4p 2 P 3/2 line because of population trapping in the metastable 3d 2 D 5/2 state, into which the 4p 2 P 3/2 level decays. From the time dependence of the fluorescence after blocking the third laser we determined the lifetime of the 3d 2 D 5/2 level. Our result of τ = 1064(17) ms improves earlier results and agrees with the value recently computed by Liaw using the Brueckner approximation.
Providing ideal conditions for the study of ion-neutral collisions, we investigate here the properties of the saturated, steady state of a three-dimensional Paul trap, loaded from a magneto-optic trap. In particular, we study three assumptions that are sometimes made under saturated, steady-state conditions: (i) The pseudopotential provides a good approximation for the number, Ns, of ions in the saturation regime, (ii) the maximum of Ns occurs at a loading rate of approximately 1 ion per rf cycle, and (iii) the ion density is approximately constant. We find that none of these assumptions are generally valid. However, based on detailed classical molecular dynamics simulations, and as a function of loading rate and trap control parameter, we show where to find convenient dynamical regimes for ion-neutral collision experiments, or how to rescale to the pseudo-potential predictions. We also investigate the fate of the electrons generated during the loading process and present a new heating mechanism, insertion heating, that in some regimes of trapping and loading may rival and even exceed the rf-heating power of the trap.
The main objective of this study is to investigate the quantum mechanical lifetime of a trapped ion in a Paul trap. The motivation for this research is that there are several applications of trapped ion devices such as mass spectrometers, atomic clocks, and quantum computers. Active research is presently ongoing in the subject of an ion trapping by electric and magnetic fields. There are many classical studies of the characteristics of trapped ions, however there have been relatively few done quantum mechanically. It might be expected that purely quantum effects could play an important role in describing the trapped ions. So, those are the main factors behind the research on this topic. Time-dependent perturbation theory was used in this study which is to find the quantum mechanical lifetime of trapped ion in a Paul trap because time-dependent perturbation theory allows describing the complex system with the help of a simple system that can be calculated easily. It is shown that the lifetime of a trapped ion depends on its transition frequency and the transition between two allowed quantum states of the ion. The transition frequency of an ion has to be very close to the applied frequency of alternating current (AC). The results show that the lifetime of a trapped ion can be adjusted as desired for experimentation.