We report on the state of the art of quantum walk experiments with neutral atoms in state-dependent optical lattices. We demonstrate a novel state-dependent transport technique enabling the control of two spin-selective sublattices in a fully independent fashion. This transport technique allowed us to carry out a test of single-particle quantum interference based on the violation of the Leggett-Garg inequality and, more recently, to probe two-particle quantum interference effects with neutral atoms cooled into the motional ground state. These experiments lay the groundwork for the study of discrete-time quantum walks of strongly interacting, indistinguishable particles to demonstrate quantum cellular automata of neutral atoms.
We report on the state of the art of quantum walk experiments with neutral atoms in state-dependent optical lattices. We demonstrate a novel state-dependent transport technique enabling the control of two spin-selective sublattices in a fully independent fashion. This transport technique allowed us to carry out a test of single-particle quantum interference based on the violation of the Leggett-Garg inequality and, more recently, to probe two-particle quantum interference effects with neutral atoms cooled into the motional ground state. These experiments lay the groundwork for the study of discrete-time quantum walks of strongly interacting, indistinguishable particles to demonstrate quantum cellular automata of neutral atoms.
This thesis reports on a novel concept of state-dependent transport, which achieves an unprecedented control over the position of individual atoms in optical lattices. Utilizing this control I demonstrate an experimental violation of the Leggett Garg inequality, which rigorously excludes (i.e. falsifies) any explanation of quantum transport based on classical, well-defined trajectories. Furthermore, I demonstrate the generation of arbitrary low-entropy states of neutral atoms following a bottom-up approach by rearranging a dilute thermal ensemble into a predefined, ordered distribution in a one-dimensional optical lattice. Additionally, I probe two-particle quantum interference effects of two atom trajectories by realizing a microwave Hong-Ou-Mandel interferometer with massive particles, which are cooled into the vibrational ground state. The first part of this thesis reports on several new experimental tools and techniques: three-dimensional ground state cooling of single atoms, which are trapped in the combined potential of a polarization-synthesized optical lattice and a blue-detuned hollow dipole potential; A high-NA (0.92) objective lens achieving a diffraction limited resolution of 460 nm; and an improved super-resolution algorithm, which resolves the position of individual atoms in small clusters at high filling factors, even when each lattice site is occupied. The next part is devoted to the conceptually new optical-lattice technique that relies on a high-precision, high-bandwidth synthesis of light polarization. Polarization-synthesized optical lattices provide two fully controllable optical lattice potentials, each of them confining only atoms in either one of the two long-lived hyperfine states. By employing one lattice as the storage register and the other one as the shift register, I provide a proof of concept that selected regions of the periodic potential can be filled with one particle per site. In the following part I report on a stringent test of the non-classicality of the motion of a massive quantum particle, which propagates on a discrete lattice. Measuring temporal correlations of the position of single atoms performing a quantum walk, we observe a 6σ (standard deviation) violation of the Leggett-Garg inequality. The experiment is carried out using so-called ideal negative measurements – an essential requisite for any genuine Leggett-Garg test – which acquire information about the atom’s position while avoiding any direct interaction with it. This interaction-free measurement is based on our polarization-synthesized optical lattice, which allows us to directly probe the absence rather than the presence of atoms at a chosen lattice site. Beyond its fundamental aspect, I demonstrate the application of the Leggett-Garg correlation function as a witness of quantum superposition. The witness allows us to discriminate the quantumness of different types of walks spanning from merely classical to quantum dynamics and further to witness the decoherence of a quantum state. In the last experimental part I will discuss recent results on collisional losses due to inelastic collisions occurring at high two-atom densities and demonstrate a Hong-Ou-Mandel interference with massive particles. Our precise control over individual indistinguishable particles embodies a direct analogue of the original Hong-Ou-Mandel experiment. By carrying out a Monte Carlo analysis of our experimental data, I demonstrate a signature of the two-particle interference of two-atom trajectories with a statistical significance of 4σ. In the final part I will introduce several new experiments which can be realized with the tools and techniques developed in this thesis, spanning from the detection of topologically protected edge states to the prospect of building a one-million-operation quantum cellular automaton.
The present work investigates the state-selective transport of single neutral cesium atoms in a one-dimensional optical lattice. It demonstrates experimental applications of this transport, including a single atom interferometer, a quantum walk and controlled two-atom collisions. The atoms are stored one by one in an optical lattice formed by a standing wave dipole trap. Their positions are determined with sub-micrometer precision, while atom pair separations are reliably inferred down to neighboring lattice sites using real-time numerical processing. Using microwave pulses in the presence of a magnetic field gradient, the internal qubit states, encoded in the hyperfine levels of the atoms, can be separately initialized and manipulated. This allows us to perform arbitrary single-qubit operations and prepare arbitrary patterns of atoms in the lattice with single-site precision. Chapter 1 presents the experimental setup for trapping a small number of cesium atoms in a one-dimensional optical lattice. Chapter 2 is devoted to fluorescence imaging of atoms, discussing the imaging setup, numeric methods and their performance in detail. Chapter 3 focuses on engineering of internal states of trapped atoms in the lattice using optical methods and microwave radiation. It provides a detailed investigation of coherence properties of our experimental system. Finally manipulation of individual atoms with almost single-site resolution and preparation of regular strings of atoms with predefined distances are presented. In Chapter 4, basic concepts, the experimental realization and the performance of the state-selective transport of neutral atoms over several lattice sites are presented and discussed in detail. Coherence properties of this transport are investigated in Chapter 5, using various two-arms single atom interferometer sequences in which atomic matter waves are split, delocalized, merged and recombined on the initial lattice site, while the interference contrast and the accumulated phase difference are measured. By delocalizing a single atom over several lattice sites, possible spatial inhomogeneities of fields along the lattice axis in the trapping region are probed. In Chapter 6, experimental realization of a discrete time quantum walk on a line with single optically trapped atoms is presented as an advanced application of multiple path quantum interference in the context of quantum information processing. Using this simple example of a quantum walk, fundamental properties of and differences between the quantum and classical regimes are investigated and discussed in detail. Finally, by combining preparation of atom strings, position-dependent manipulation of qubit states and state-selective transport, in Chapter 7, two atoms are deterministically brought together into contact, forming a starting point for investigating two-atom interactions on the most fundamental level. Future prospects and suggestions are finally presented in Chapter 8.
Advances in the preparation and detection, but most importantly in the coherent manipulation of single neutral atoms have allowed the observation of intriguing phenomena of quantum physics in recent years. We discuss developments to prepare and detect single neutral atoms in a one-dimensional optical lattice potential with single site resolution. Moreover, using two different experimental techniques, a state-dependent optical lattice potential on the one hand and a high-finesse optical cavity on the other hand, we have obtained coherent control over single neutral atoms. The former has enabled us to observe the quantum walk of atoms in position space, and to coherently control the motion of trapped atoms via microwave radiation. The latter offers a means to non-destructively detect the atomic spin state, thereby revealing quantum jumps of single atoms, or the altered optical properties of single atoms when subject to electromagnetically-induced transparency.
The quantum walk is the quantum analog of the well-known random walk, which forms the basis for models and applications in many realms of science. Its properties are markedly different from the classical counterpart and might lead to extensive applications in quantum information science. In our experiment, we implemented a quantum walk on the line with single neutral atoms by deterministically delocalizing them over the sites of a one-dimensional spin-dependent optical lattice. With the use of site-resolved fluorescence imaging, the final wave function is characterized by local quantum state tomography, and its spatial coherence is demonstrated. Our system allows the observation of the quantum-to-classical transition and paves the way for applications, such as quantum cellular automata.
We investigate continuous-time quantum walks of two indistinguishable particles (bosons, fermions or hard-core bosons) in one-dimensional lattices with nearest-neighbour interactions. The two interacting particles can undergo independent- and/or co-walking dependent on both quantum statistics and interaction strength. We find that two strongly interacting particles may form a bound state and then co-walk like a single composite particle with statistics-dependent propagation speed. Such an effective single-particle picture of co-walking is analytically derived in the context of degenerate perturbation and the analytical results are well consistent with direct numerical simulation. In addition to implementing universal quantum computation and observing bound states, two-particle quantum walks offer a novel route to detecting quantum statistics. Our theoretical results can be examined in experiments of light propagations in two-dimensional waveguide arrays or spin-impurity dynamics of ultracold atoms in one-dimensional optical lattices.