Decoherence is an essential mechanism that defines the boundary between classical and quantum behaviours, while imposing technological bounds for quantum devices. Little is known about quantum coherence of mechanical systems, as opposed to electromagnetic degrees of freedom. But decoherence can also be thought of in a purely classical context, as the loss of phase coherence in the classical phase space. Indeed the bridge between quantum and classical physics is under intense investigation, using, in particular, classical nanomechanical analogues of quantum phenomena. In the present work, by separating pure dephasing from dissipation, we quantitatively model the classical decoherence of a mechanical resonator: through the experimental control of frequency fluctuations, we engineer artificial dephasing. Building on the fruitful analogy introduced between spins/quantum bits and nanomechanical modes, we report on the methods available to define pure dephasing in these systems, while demonstrating the intrinsic almost-ideal properties of silicon nitride beams. These experimental and theoretical results, at the boundary between classical nanomechanics and quantum information fields, are prerequisite in the understanding of decoherence processes in mechanical devices, both classical and quantum. Introduction and background. Frequency noise in nano-mechanical systems (NEMS) is a topic intensely studied these last years, for both fundamental and practical reasons (references [ 13 – 23 ] of the paper): the frequency fluctuations can have an intrinsic origin linked to essential material properties, but they also limit the resolution of actual devices used as sensors. Recently, the Delft group proposed to analyze the effects of this noise on the dynamics of NEMS within a framework analogous to one of Nuclear Magnetic Resonance (NMR), or quantum bits (2014 Nat. Commun. 5 5819 ). Main results. Building on the analogy, in this paper we engineer frequency noise to study its impact on nano-resonators. We present a model experiment, with the full theory enabling the fit of data without free parameters. The effect of frequency noise is analogous to 'pure dephasing' in quantum bits, even though the device is a classical harmonic oscillator. As such, the analogy is very informative and interrogates the crossover between classical and quantum physics; it enters the class of 'classical analogues of quantum phenomena' studied in recent model nano-mechanical experiments (e.g. reference [ 10 ]). Wider implications. This is a broad topic that is of interest to many areas of science, far beyond NEMS and NMR. For the focused audience, we present the methods to quantitatively describe this 'classical pure dephasing' of NEMS, which can be used e.g. with carbon-based systems. As a conclusion, our results are a new tool for the understanding of classical decoherence in nano-resonators, and a pre-requisite for future experiments on quantum NEMS.
Decoherence is an essential mechanism that defines the boundary between classical and quantum behaviours, while imposing technological bounds for quantum devices. Little is known about quantum coherence of mechanical systems, as opposed to electromagnetic degrees of freedom. But decoherence can also be thought of in a purely classical context, as the loss of phase coherence in the classical phase space. Indeed the bridge between quantum and classical physics is under intense investigation, using, in particular, classical nanomechanical analogues of quantum phenomena. In the present work, by separating pure dephasing from dissipation, we quantitatively model the classical decoherence of a mechanical resonator: through the experimental control of frequency fluctuations, we engineer artificial dephasing. Building on the fruitful analogy introduced between spins/quantum bits and nanomechanical modes, we report on the methods available to define pure dephasing in these systems, while demonstrating the intrinsic almost-ideal properties of silicon nitride beams. These experimental and theoretical results, at the boundary between classical nanomechanics and quantum information fields, are prerequisite in the understanding of decoherence processes in mechanical devices, both classical and quantum. Introduction and background. Frequency noise in nano-mechanical systems (NEMS) is a topic intensely studied these last years, for both fundamental and practical reasons (references [ 13 – 23 ] of the paper): the frequency fluctuations can have an intrinsic origin linked to essential material properties, but they also limit the resolution of actual devices used as sensors. Recently, the Delft group proposed to analyze the effects of this noise on the dynamics of NEMS within a framework analogous to one of Nuclear Magnetic Resonance (NMR), or quantum bits (2014 Nat. Commun. 5 5819 ). Main results. Building on the analogy, in this paper we engineer frequency noise to study its impact on nano-resonators. We present a model experiment, with the full theory enabling the fit of data without free parameters. The effect of frequency noise is analogous to 'pure dephasing' in quantum bits, even though the device is a classical harmonic oscillator. As such, the analogy is very informative and interrogates the crossover between classical and quantum physics; it enters the class of 'classical analogues of quantum phenomena' studied in recent model nano-mechanical experiments (e.g. reference [ 10 ]). Wider implications. This is a broad topic that is of interest to many areas of science, far beyond NEMS and NMR. For the focused audience, we present the methods to quantitatively describe this 'classical pure dephasing' of NEMS, which can be used e.g. with carbon-based systems. As a conclusion, our results are a new tool for the understanding of classical decoherence in nano-resonators, and a pre-requisite for future experiments on quantum NEMS.
The efficiency of the future devices for quantum information processing is limited mostly by the finite decoherence rates of the individual qubits and quantum gates. Recently, substantial progress was achieved in enhancing the time within which a solid-state qubit demonstrates coherent dynamics. This progress is based mostly on a successful isolation of the qubits from external decoherence sources obtained by engineering. Under these conditions, the material-inherent sources of noise start to play a crucial role. In most cases, quantum devices are affected by noise decreasing with frequency f approximately as 1/f. According to the present point of view, such noise is due to material- and device-specific microscopic degrees of freedom interacting with quantum variables of the nanodevice. The simplest picture is that the environment that destroys the phase coherence of the device can be thought of as a system of two-state fluctuators, which experience random hops between their states. If the hopping times are distributed in an exponentially broad domain, the resulting fluctuations have a spectrum close to 1/f in a large frequency range. This paper reviews the current state of the theory of decoherence due to degrees of freedom producing 1/f noise. Basic mechanisms of such noises in various nanodevices are discussed and several models describing the interaction of the noise sources with quantum devices are reviewed. The main focus of the review is to analyze how the 1/f noise destroys their coherent operation. The start is from individual qubits concentrating mostly on the devices based on superconductor circuits and then some special issues related to more complicated architectures are discussed. Finally, several strategies for minimizing the noise-induced decoherence are considered.
The coupling of nanomechanical resonators to controllable quantum systems represents a growing and promising area of research. Recent advances in this field have brought to astonishing results, such as the initialization of a mechanical resonator into its quantum ground state and even the preparation of non-classical coherent states of motion. These achievements open up appealing scenarios to quantum information technologies and to the exploration of the quantum-classical boundary. From an application perspective, such quantum-mechanical hybrid systems provide a versatile and attractive tool for a variety of precision measurements, like ultra-sensitive detection of force, mass, and displacement. \n \nQuantum control over a mechanical resonator, or, conversely, the prospect of using resonator's motion for probing quantum states, both involve some tight requirements. First of all, the interaction between the mechanics and its quantum partner has to be large on the scale of the decoherence rates of the coupled systems. In most cases, the coupling mechanism has to be activated by engineering the resonator with electrodes, magnets, or mirrors, or by using tailored laser fields. For this reason, the search for a strong coupling typically competes with the requirement of overcoming decoherence effects. In addition, for quantum effects to be observable, strong coupling has to be accompanied by the preparation of zero entropy initial states, for instance by cooling the resonator into its ground state of motion. \n \nThe motivation pursued by this thesis is to contribute to the inspiring field of hybrid systems by walking through each of the aforementioned directions. We in fact demonstrate a promising system in which optically active quantum dots, embedded in fully self-assembled core-shell nanowires, are coupled to the nanowire motion. Mechanical vibrations of the nanowire modulate the quantum dot emission energy over a broad range exceeding 14 meV, by means of deformation potential coupling. In our system, therefore, both the coupling mechanism and the quantum states themselves are intrinsic to the resonator's structure. Besides revealing unusually strong, such a built-in opto-mechanical interaction produces a hybrid system whose inherent coherence is unspoiled by any functionalization or external field and whose fabrication is simpler than top-down techniques. \n \nWe further demonstrate the use of a quantum point contact as a displacement transducer to measure and control the low-temperature thermal motion of a nearby micromechanical cantilever. We show that by including the QPC in a suitable feedback loop, we are able to cool the cantilever's fundamental mechanical mode down to the level of the measurement noise, achieving a squashing of the QPC noise at high gain. Due to its off-board design, our system is particularly versatile and suitable to force-sensing applications. Since the QPC transducer is sensitive to local modifications of the nearby electric field, our approach is in principle compatible with any nanoscale resonator, without requiring any functionalization to activate the coupling. By improving the performance of the QPC as a one-dimensional conductor and the cantilever-QPC capacitive coupling, our system has the potential to achieve quantum-limited displacement resolution and ground state cooling. We then report on some ongoing attempts to overcome the current limitations of our system and couple mechanical motion to different mesoscopic transport devices. \n \nWe remark that our demonstration of an as-grown quantum-dot-in-nanowire hybrid system opens up bright prospects on future experiments, as also testified by the very recent ferment of the scientific community around this topic. We find that the opto-mechanical coupling rate is not far from the nanowire mechanical frequency. This fact makes our system particularly promising for the quantum non-demolition readout of a quantum dot state through a measurement of the nanowire position. On the other hand, we show that the coupling can be further optimized, and the nanowire mechanical heating rate reduced, thus disclosing the captivating perspective of using quantum dots to probe and control the mechanical state of a nanowire. In this context, it would be important to investigate a possible spin-oscillator coupling in our system, given the long coherence time offered by a spin state in a quantum dot. The wide range of control over the quantum dots emission energy and the ability to tune two neighboring dots into resonance pave the way to mechanically induced emitter-emitter coupling. In addition, our monolithic opto-mechanical system constitutes a good candidate for recent proposals of a tripartite hybrid system, which would integrate an optical cavity, a quantum two-level system and a mechanical resonator. The intrinsically strong coupling between the quantum dots and the nanowire motion would enhance the interaction between the mechanics and the cavity field, leading for instance to efficient cooling of the resonator to the ground state. Finally, the quantum dot sensitivity to the nanowire resonant vibration could also support the use of our system as an integrated force probe or as a nanomechanical mass sensor. In other words, the results reported in this dissertation constitute not only a relevant proof-of-principle, moreover they open up intriguing challenges for future research.
Why are classical theories often sufficient to describe the physics of our world even though everything around us is entirely composed of microscopic quantum systems? The boundary between these two fundamentally dissimilar theories remains an unsolved problem in modern physics. Position measurements of small objects allow us to probe the area where the classical approximation breaks down. In quantum mechanics, Heisenbergâ s uncertainty principle dictates that any measurement of the position must be accompanied by measurement induced back-action---in this case manifested as an uncertainty in the momentum. In recent years, cavity optomechanics has become a powerful tool to perform precise position measurements and investigate their fundamental limitations. The utilization of optical micro-cavities greatly enhances the interaction between light and state-of-the-art nanomechanical oscillators. Therefore, quantum mechanical phenomena have been successfully observed in systems far beyond the microscopic world. In such a cavity optomechanical system, the fluctuations in the position of the oscillator are transduced onto the phase of the light, while fluctuations in the amplitude of the light disturb the momentum of the oscillator during the measurement. As a consequence, correlations are established between the amplitude and phase quadrature of the probe light. However, so far, observation of quantum effects has been limited exclusively to cryogenic experiments, and access to the quantum regime at room temperature has remained an elusive goal because the overwhelming amount of thermal motion masks the weak quantum effects. This thesis describes the engineering of a high-performance cavity optomechanical device and presents experimental results showing, for the first time, the broadband effects of quantum back-action at room temperature. The device strongly couples mechanical and optical modes of exceptionally high quality factors to provide a measurement sensitivity ∼104 times below the requirement to resolve the zero-point fluctuations of the mechanical oscillator. The quantum back-action is then observed through the correlations created between the probe light and the motion of the nanomechanical oscillator. A so-called â variational measurementâ , which detects the transmitted light in a homodyne detector tuned close to the amplitude quadrature, resolves the quantum noise due to these correlations at the level of 10\% of the thermal noise over more than an octave of Fourier frequencies around mechanical resonance. Moreover, building on this result, an additional experiment demonstrates the ability to achieve quantum enhanced metrology. In this case, the generated quantum correlations are used to cancel quantum noise in the measurement record, which then leads to an improved relative signal-to-noise ratio in measurements of an external force. In conclusion, the successful observation of broadband quantum behavior on a macroscopic object at room temperature is an important milestone in the field of cavity optomechanics. Specifically, this result heralds the rise of optomechanical systems as a platform for quantum physics at room temperature and shows promise for generation of ponderomotive squeezing in room-temperature interferometers.
The conventional Quantum 1/f (Q1/f) Effect is present in any scattering cross section or process rate involving charged particles or current carriers. The present paper shows how bremsstrahlung and decoherence at all frequencies yield macroscopic quantum interference, resulting in probability density fluctuations at all frequencies in the outgoing scattered beam, that are observed as fundamental base-band 1/f noise and as 1/f frequency fluctuations, or phase noise close to carrier, in materials, devices, and resonant or non-resonant systems. We emphasize the role of the phenomenon of quantum decoherence showing that the fundamental, universal 1/f noise is both a phenomenon of decoherence and of the infrared divergence of quantum electrodynamics. This eliminates the last persisting misunderstandings of the Q1/f Theory and of this new field of Infra-quantum Physics. On this basis we give the first universal engineering formulas, applicable for the ultra-low noise optimization of all Hi-Tech applications, of the materials, devices and systems of modern industry, microelectronics, nanotechnology, highest stability resonators, oscillators and clocks, MEMS, and any resonant and non-resonant sensors. Q1/f noise, i.e, the coherent and conventional Q1/f Effects, is a new fundamental aspect of quantum physics, as basic as space and time. In resonators and oscillators, fundamental frequency fluctuations come usually from 1/f fluctuations in the dissipation.
We investigate a system composed of two coupled oscillators subject to stochastic fluctuations in its internal parameters. In particular, we answer the question whether the well-known classical analogy of the quantum dynamics of two-level systems (TLSs), i.e., qubits, provided by two coupled oscillators can be extended to simulate the dynamics of dissipative quantum systems. In the context of nanomechanics, the analogy in the dissipation-free case has already been tested in multiple experimental setups, e.g., doubly clamped or cantilever string resonators and optically levitated particles. A well-known result of this classical analogy is that the relaxation and decoherence times of the analog quantum system must be equal, i.e., T1=T2 , in contrast to the general case of quantum TLSs. We show that this fundamentally quantum feature, i.e., T1≠T2 , can be implemented as well in the aforementioned classical systems by adding stochastic fluctuations in their internal parameters. Moreover, we show that these stochastic contributions can be engineered in the control apparatus of those systems, discussing, in particular, the application of this theory to levitated nanoparticles and to nanostring resonators. Published by the American Physical Society 2024
One central theme in quantum photonics is tailoring the interactions between atoms/spins and their electromagnetic (EM) environments. Considerable effort has focused on engineering spontaneous emission by shaping EM environments, known as the Purcell effect. However, photonic environment control of pure dephasing, which is a complementary paradigm of non-unitary atom/spin couplings with EM environments, remains largely unexplored. Here, we introduce a nanophotonic approach to modify qubit pure dephasing dynamics. Unlike Purcell engineering that tailors photonic environments at qubit resonance frequencies (typically optical/near-infrared), we develop ultra-subwavelength spin noise metasurfaces for efficient broadband control of low-frequency (e.g., ∼MHz) photonic environments far off-resonant with atoms/spins for dephasing engineering. We experimentally demonstrate our approach using lithographically defined CoFeB metasurfaces and shallow nitrogen-vacancy (NV) centers in diamond. Instead of modified spontaneous emission, we observe modified NV pure dephasing dynamics near different spin noise metasurfaces. We further isolate metasurface-controlled dephasing from other dephasing mechanisms (e.g., spin bath) by measuring the NV ensemble dephasing noise spectrum with dynamical decoupling spectral decomposition techniques. Our results establish a new frontier in engineering quantum light-matter interactions with nanophotonic structures.