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arXiv:1510.09116 · Physical Review A

Evidence of indistinguishability and entanglement determined by the energy-time uncertainty principle in a system of two strongly coupled bosonic modes

Smail B. Bougouffa, Z. Ficek

Published Jun 27, 2016• 12 citations
arXivHTMLPDF

Abstract

The link of two concepts, indistinguishability and entanglement, with the energy-time uncertainty principle is demonstrated in a system composed of two strongly coupled bosonic modes. Working in the limit of a short interaction time, we find that the inclusion of the antiresonant terms to the coupling Hamiltonian leads the system to relax to a state which is not the ground state of the system. This effect occurs passively by just presence of the antiresonant terms and is explained in terms of the time-energy uncertainty principle for the simple reason that at a very short interaction time, the uncertainty in the energy is of order of the energy of a single excitation, thereby leading to a distribution of the population among the zero, singly and doubly excited states. The population distribution, correlations, and entanglement are shown to substantially dependent on whether the modes decay independently or collectively to an exterior reservoir. In particular, when the modes decay independently with equal rates, entanglement with the complete distinguishability of the modes is observed. The modes can be made mutually coherent if they decay with unequal rates. However, the visibility in the single-photon interference cannot exceed $50%$. When the modes experience collective damping, they are indistinguishable even if decay with equal rates and the visibility can, in principle, be as large as unity. We find that this feature derives from the decay of the system to a pure entangled state rather than the expected mixed state. When the modes decay with equal rates, the steady-state values of the density matrix elements are found dependent on their initial values.

DOI
10.1103/physreva.93.063848

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The Journal of Chemical Physics•Feb 1, 1979•124 citations
The link of two concepts, indistinguishability and entanglement, with the energy-time uncertainty principle is demonstrated in a system composed of two strongly coupled bosonic modes. Working in the limit of a short interaction time, we find that the inclusion of the antiresonant terms to the coupling Hamiltonian leads the system to relax to a state which is not the ground state of the system. This effect occurs passively by just presence of the antiresonant terms and is explained in terms of the time-energy uncertainty principle for the simple reason that at a very short interaction time, the uncertainty in the energy is of order of the energy of a single excitation, thereby leading to a distribution of the population among the zero, singly and doubly excited states. The population distribution, correlations, and entanglement are shown to substantially dependent on whether the modes decay independently or collectively to an exterior reservoir. In particular, when the modes decay independently with equal rates, entanglement with the complete distinguishability of the modes is observed. The modes can be made mutually coherent if they decay with unequal rates. However, the visibility in the single-photon interference cannot exceed 5050%50. When the modes experience collective damping, they are indistinguishable even if decay with equal rates and the visibility can, in principle, be as large as unity. We find that this feature derives from the decay of the system to a pure entangled state rather than the expected mixed state. When the modes decay with equal rates, the steady-state values of the density matrix elements are found dependent on their initial values.
Interesting coherence and correlations appear between superpositions of two bosonic modes when the modes are parametrically coupled to a third intermediate mode and are also coupled to external modes which are in thermal states of unequal mean photon numbers. Under such conditions, it is found that one of linear superpositions of the modes, which is effectively decoupled from the other modes, can be perfectly coherent with the other orthogonal superposition of the modes and can simultaneously exhibit anticoherence with the intermediate mode, which can give rise to entanglement between the modes. It is shown that the coherence effects have a substantial effect on the population distribution between the modes, which may result in lowering the population of the intermediate mode. This shows that the system can be employed to cool modes to lower temperatures. Furthermore, for appropriate thermal photon numbers and coupling strengths between the modes, it is found that entanglement between the directly coupled superposition and the intermediate modes may occur in a less restricted range of the number of the thermal photons such that the modes could be strongly entangled, even at large numbers of the thermal photons.
We study the entanglement dynamics in the system of coupled boson fields. We demonstrate that there are different natural notions of locality in this context leading to inequivalent notions of entanglement. We concentrate on the particle picture, when entanglement of one particle is determined by one-particle density matrix. We study, in detail, the effect of interaction preserving populations of individual one-particle states. We show that if the system is initially in a disentangled state with the definite total number of particles and the dimension of the one-particle Hilbert space is more than two, then only potentials of the special form admit complete entanglement, which is shown to be reached at NOON states. If the system is initially in Glauber’s coherent state, complete entanglement is not reached despite the presence of two entangling channels in this case. We conclude with studying the time evolution of entanglement of photons in a cavity with multiple quantum dots in the limit of large number of photons. We show that in a relatively short time scale the completely entangled states belong to the class of graph states and are formed due to the interaction with dots in resonance with the cavity modes.
Dynamics of entangled states of two independent single-mode cavities in squeezed reservoirs is investigated in the context of matching of the correlations contained in the entangled states to those contained in the squeezed reservoir. We illustrate our considerations by examining the time evolution of entanglement of single and double excitation NOON and EPR states. A comparison is made when each cavity is coupled to own reservoir or both cavities are coupled to a common reservoir. It is shown that the evolution of the initial entanglement and transfer of entanglement from the squeezed reservoir to the cavity modes depend crucially on the matching of the initial correlations to that contained in the squeezed reservoir. In particular, it is found that initially entangled modes with correlations different from the reservoir correlations prevent the transfer of the correlations from the squeezed field to the modes. In addition, we find that the transient entanglement exhibits several features unique to quantum nature of squeezing. In particular, we show that in the case of separate squeezed reservoirs a variation of the decay time of the initial entanglement with the squeezing phase is unique to quantum squeezing. In the case of a common reservoir a recurrence of entanglement occurs and we find that this feature also results from the reservoir correlations unique to quantum squeezing. There is no revival of entanglement when the modes interact with a classically squeezed field.
Entanglement is a fundamental feature of quantum physics and a key resource for quantum communication, computing, and sensing. Entangled states are fragile and maintaining coherence is a central challenge in quantum information processing. Nevertheless, entanglement can be generated and stabilized through dissipative processes. In fact, entanglement has been shown to exist in the steady state of certain interacting quantum systems subject solely to incoherent coupling to thermal baths. This has been demonstrated in a range of bi- and multipartite settings using systems of finite dimension. Here we focus on the steady state of infinite-dimensional bosonic systems. Specifically, we consider any set of bosonic modes undergoing excitation-number-preserving interactions of arbitrary strength and divided between an arbitrary number of parties that each couple weakly to thermal baths at different temperatures. We show that a unique steady state is always separable.
It is well established that an entanglement encoded in the Bell states of a two-qubit system with correlated spins exhibits completely different evolution properties from that encoded in states with the anticorrelated spins. A complete and abrupt loss of the entanglement, called the entanglement sudden death, can be found to occur for the spin-correlated states, but the entanglement evolves without any discontinuity or decays asymptotically for the spin-anticorrelated states. We consider the evolution of an initial entanglement encoded in the spin-anticorrelated states and demonstrate that the asymptotic behavior predicted before occurs only in the weak-coupling limit or equivalently when the rotating-wave approximation (RWA) is made on the interaction Hamiltonian of the qubits with the field. If we do not restrict ourselves to the RWA, we find that the entanglement undergoes a discontinuity, the sudden-death phenomenon. We illustrate this behavior by employing an efficient scheme for entanglement evolution between two cold-trapped atoms located inside a single-mode cavity. Although only a single excitation is initially present in the system, we find that the two-photon excited state, which plays the key role for the discontinuity in the behavior of the entanglement, gains a population over a short time of the evolution. When the RWA is made on the interaction, the two-photon excited state remains unpopulated for all times and the discontinuity is absent. We attribute this phenomenon to the principle of complementarity between the evolution time and energy, and the presence of the counter-rotating terms in the interaction Hamiltonian.
One purpose of this paper is to present new studies on the effect of bandwidth and the coherence properties of the excitation source on the decay and the dephasing of isolated large molecules. A detailed study of the system pentacene in a p-terphenyl matrix is presented utilizing three different excitation sources, a single mode dye laser (60 KHz–6 MHz bandwidth depending on the time scale of the experiment) a multimode dye laser (240 GHz bandwidth), and an incoherent N2 flash lamp. Optical T1 (the longitudinal relaxation time) and T2 (the transverse relaxation time) are measured from the coherent and incoherent transients observed either in the forward direction of the laser or at right angles to the exciting beam. At 1.8 °K, the optical transition (1A1g→1B2u) of pentacene in p-terphenyl exhibits four sites, the lowest of which at 16 887 cm−1 has the following parameters: T2=44±2 nsec; T1=24.9±2 nsec, and μ=0.7±0.1 D. The transition moment μ, is obtained directly from the optical nutation, which exhibits a Rabi nutation time (h//μ⋅ε) of 27.3 nsec, and is corrected for the effect of the Lorentz local field inside the terphenyl crystal. The experiments presented here are categorized into two time regimes for theoretical analysis; a transient coherence regime where the observed decay is comparable with (h//μ⋅ε) and T2, and a steady-state coherence regime where transient dephasing is complete and the off-diagonal elements of the density matrix have decayed to their steady-state values in the presence of the field of amplitude ε. Using the Wilcox–Lamb method, rate equations (with T2 expressions) describing the population flow in the ’’complete’’ level structure of pentacene (ground‖0〉, singlet ‖p〉, and triplet {‖l}) are derived from the density matrix equations of motion. When these equations are averaged over the inhomogeneous width of the optical transition and the measured Gaussian transverse profile of our laser we obtain T1p0=24.9±2 nsec and T1pl=15.7 μsec, the time constants by which pentacene spontaneously decays to ‖0〉 or crosses over into l, as well as the averaged population at time t. In an effort to be complete, attention is placed upon the relationship between theory and the experimental findings. First, expressions for the OFID and nutation in the solid are presented for the pentacene case in order to relate T1, T2, and μ to the level structure. Second, at low temperatures (1.8 °K), the origin of dephasing is identified as spontaneous emission from p→0 since experimentally T2?2T1, in agreement with other work. At higher temperature, however, a strongly temperature dependent dephasing process with an onset at 3.7 °K takes place. Armed with these observations we present a theoretical treatment of these distinct dephasing channels and their temperature dependences. A discussion regarding the influence of ’’accepting’’ phonon modes (either optical or acoustic) on optical dephasing is also given. The results indicate that the treatment of Jones et al. can (1) explain the observed temperature dependence of T2 in pentacene; (2) distinguish dephasing as a result of scattering by acoustic phonons from that due to resonance or quasilocalized phonons with clear connections to gas and liquid state theories, but without invoking more than two approximation levels. (3) explain both the level shift and line width changes as a result of ’’conventional’’ dephasing or dephasing by exchange mechanisms; and (4) relate the pure dephasing term to an anisotropy in the scattering amplitudes (between the ground and excited states in the system) which contribute largely to the homogeneous width of the transition. Optical site selection of these transitions is also reported and discussed in relation to vibrational relaxation and to both homogeneous and inhomogeneous broadenings. The studies of the homogeneous broadening of the vibronic origin (267 cm−1) indicate that vibrational relaxation is fast (psec) in the excited singlet manifold of pentacene. Finally from more than ten independent experiments including single and multimode excitation, on- and off-resonance scattering, Zeeman effect and the transient decay as a function of excess energy in the molecule, a more complete picture of the pentacene level structure {‖l〉} is given. With this in mind, the influence of the laser bandwidth and coherence properties on state preparation and subsequent dephasing and decay is concluded. It is proposed that the slow decay, (∼15 μsec) observed during narrow-band excitation represents intersystem crossing to nearby triple manifolds after the transient coherence of the 0↔p subsystem is decayed. In addition, the decay of the primary state prepared in these experiments is not sensitive to the bandwidth or the correlation time of our excitation sources.