Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1510.02665 · Physical Review Letters

Demonstration of Light-Matter Micro-Macro Quantum Correlations

Alexey Tiranov, Jonathan Lavoie, Peter C. Strassmann, Nicolas Sangouard, Mikael Afzelius, Félix Bussières, Nicolas Gisin

Published May 11, 2016• 11 citations
arXivHTMLPDF

Abstract

Quantum mechanics predicts microscopic phenomena with undeniable success. Nevertheless, current theoretical and experimental efforts still do not yield conclusive evidence that there is or is not a fundamental limitation on the possibility to observe quantum phenomena at the macroscopic scale. This question prompted several experimental efforts producing quantum superpositions of large quantum states in light or matter. We report on the observation of quantum correlations, revealed using an entanglement witness, between a single photon and an atomic ensemble of billions of ions frozen in a crystal. The matter part of the state involves the superposition of two macroscopically distinguishable solid-state components composed of several tens of atomic excitations. Assuming the insignificance of the time ordering our experiment indirectly shows light-matter micro-macro entanglement. Our approach leverages from quantum memory techniques and could be used in other systems to expand the size of quantum superpositions in matter.

DOI
10.1103/physrevlett.116.190502

Related papers

Strict experimental test of macroscopic realism in a light-matter-interfaced system

Xiao Liu, Zong‐Quan Zhou, Yong‐Jian Han +10 more

Macroscopic realism is a classical worldview that a macroscopic system is always determinately in one of the two or more macroscopically distinguishable states available to it and so is never in a superposition of these states. The question of whether there is a fundamental limitation on the possibility to observe quantum phenomena at the macroscopic scale remains unclear. Here we implement a strict and simple protocol to test macroscopic realism in a light-matter-interfaced system. We create a micro-macro entanglement with two macroscopically distinguishable solid-state components and rule out those theories which would deny coherent superpositions of up to 76 atomic excitations shared by ${10}^{10}$ ions in two separated solids. These results provide a general method to enhance the size of superposition states of atoms by utilizing quantum memory techniques and to push the envelope of macroscopicity at higher levels.

arXiv:1910.10865•Physical Review A•Sep 5, 2019•5 citations

Entanglement between more than two hundred macroscopic atomic ensembles in a solid

Parisa Zarkeshian, Chetan Deshmukh, Neil E. Sinclair +12 more

There are both fundamental and practical motivations for studying whether quantum entanglement can exist in macroscopic systems. However, multiparty entanglement is generally fragile and difficult to quantify. Dicke states are multiparty entangled states where a single excitation is delocalized over many systems. Building on previous work on quantum memories for photons, we create a Dicke state in a solid by storing a single photon in a crystal that contains many large atomic ensembles with distinct resonance frequencies. The photon is re-emitted at a well-defined time due to an interference effect analogous to multi-slit diffraction. We derive a lower bound for the number of entangled ensembles based on the contrast of the interference and the single-photon character of the input, and we experimentally demonstrate entanglement between over two hundred ensembles, each containing a billion atoms. We also illustrate the fact that each individual ensemble contains further entanglement.Multipartite entanglement is of both fundamental and practical interest, but is notoriously difficult to witness and characterise. Here, Zarkeshian et al. demonstrate multipartite entanglement in an atomic frequency comb storing a single photon in a Dicke state spread over a macroscopic ensemble.

arXiv:1703.04709•Nature Communications•Oct 9, 2017•28 citations

Solid-state optical quantum memory: from large entanglement to telecom wavelengths

Peter C. Strassmann

Quantum mechanics is leading to many modern technologies, e.g. based on laser physics. Emerging fields are for example nonlinear optics, hybrid systems, or quantum communication. Despite these applications, there are still limitations of our understanding of quantum mechanics. Even though it is broadly accepted that decoherence limits the size of entangled states, we currently do not know how to overcome these limitations. How large can commonly entangled states be? Can we observe macroscopic quantum phenomena with coarse-grained detectors or even with our bare eyes? This thesis contributes towards answering these fundamental questions and to technological advances. The experiments are based on a light-matter platform of quantum optical states and atomic ensembles. The ensembles consist of rare-earth ion-doped crystals. Additionally, the atomic frequency comb protocol turns the ensemble into a quantum memory. In the scope of quantum communication we work on a quantum repeater. First, we investigate fundamental quantum mechanical states and their validity at macroscopic scales. We show that the detection of a collectively emitted excitation can be used to measure the size of the entangled ensemble. The entangled ensemble shared this excitation in a coherent superposition. This superposition of an atomic excitation in an ensemble is called W-state. We certify a new lower bound to the possible size of an entangled W-state between at least 16 million atoms. The proof of entanglement of this size relies on two measures: one determines the number of atoms involved in the storage process. The other one determines the state "quantumness" by examining the re-emitted light. Another experiment studies a macroscopically distinguishable superposition state. The superposition survives the storage in an atomic ensemble. Second, we perform two more experiments that contribute to a quantum repeater. One experiment probes the quantum states simultaneously stored in a multi-mode quantum memory. In this work we also develop the concept of indirect entanglement witness. For the other experiment, a frequency down-conversion platform is set up. The conversion overcomes the wavelength compatibility issue between some quantum memories and the telecommunication C-band. The narrow spectral filtering of the conversion performs better than expected. In summary, our work analyzes large entangled states and building blocks for a quantum repeater. The presented quantum memories are capable of temporal multi-mode storage. Its temporally precise re-emission is due to the re-phasing of the atoms of the W-state. We also show a good way to set up frequency down-conversion for the sake of quantum repeaters. This work emphasizes the atomic frequency comb protocol as a viable and reliable platform for quantum repeaters.

•Jan 1, 2019•0 citations

Experimental certification of millions of genuinely entangled atoms in a solid

Florian Fröwis, Peter C. Strassmann, Alexey Tiranov +6 more

Quantum theory predicts that entanglement can also persist in macroscopic physical systems, albeit difficulties to demonstrate it experimentally remain. Recently, significant progress has been achieved and genuine entanglement between up to 2900 atoms was reported. Here, we demonstrate 16 million genuinely entangled atoms in a solid-state quantum memory prepared by the heralded absorption of a single photon. We develop an entanglement witness for quantifying the number of genuinely entangled particles based on the collective effect of directed emission combined with the non-classical nature of the emitted light. The method is applicable to a wide range of physical systems and is effective even in situations with significant losses. Our results clarify the role of multipartite entanglement in ensemble-based quantum memories and demonstrate the accessibility to certain classes of multipartite entanglement with limited experimental control.The presence of entanglement in macroscopic systems is notoriously difficult to observe. Here, the authors develop a witness which allow them to demonstrate entanglement between millions of atoms in a solid-state quantum memory prepared by the heralded absorption of a single photon.

arXiv:1703.04704•Nature Communications•Oct 9, 2017•34 citations

Macroscopic quantum coherence and entanglement in mechanical systems

Benjamin Yadin, Matteo Fadel

The notion of a macroscopic quantum state must be pinned down in order to assess how well experiments probe the large-scale limits of quantum mechanics. However, the issue of quantifying so-called quantum macroscopicity is fraught with multiple approaches having varying interpretations and levels of computability and measurability. Here, we introduce two measures that capture independent macroscopic properties: i) extensive size, measuring the degree of coherence in position or momentum observables relative to atomic-scale units, and ii) entangled size, quantifying the number of entangled subsystems. These measures unify many desirable features of past proposals while having rigorously justified interpretations from quantum information theory in terms of coherence and multipartite entanglement. We demonstrate how to estimate them and obtain lower-bounds using experimental data from micro-mechanical oscillators and diffracting molecules. Notably, we find evidence for genuine multipartite entanglement of 10 5 to 10 7 atoms in recent mechanical superposition states.

arXiv:2503.08324•Quantum•Oct 30, 2026•0 citations

Quantum correlations in mesoscopic systems

Run Yan Teh

Quantum correlations are correlations that arise from a unique feature in quantum mechanics: quantum superposition. The most famous example of quantum superposition is the Schrodinger’s cat state, where a cat is in a state of neither dead nor alive before an observer determines the cat’s status. This is not what we expect. Nevertheless, quantum superposition and correlations are routinely created in the laboratories with microscopic systems involving atoms and light particles. Can this counterintuitive notion be realised in the macroscopic world? This thesis investigates this question by devising criteria that certify the existence of quantum correlations in mesoscopic/macroscopic systems. Powerful mathematical tools are used to simulate two quantum protocols in a mesoscopic system which have applications in quantum communication and computation.

•Jan 1, 2024•1 citation
Quantum mechanics predicts microscopic phenomena with undeniable success. Nevertheless, current theoretical and experimental efforts still do not yield conclusive evidence that there is or is not a fundamental limitation on the possibility to observe quantum phenomena at the macroscopic scale. This question prompted several experimental efforts producing quantum superpositions of large quantum states in light or matter. We report on the observation of quantum correlations, revealed using an entanglement witness, between a single photon and an atomic ensemble of billions of ions frozen in a crystal. The matter part of the state involves the superposition of two macroscopically distinguishable solid-state components composed of several tens of atomic excitations. Assuming the insignificance of the time ordering our experiment indirectly shows light-matter micro-macro entanglement. Our approach leverages from quantum memory techniques and could be used in other systems to expand the size of quantum superpositions in matter.
Macroscopic realism is a classical worldview that a macroscopic system is always determinately in one of the two or more macroscopically distinguishable states available to it and so is never in a superposition of these states. The question of whether there is a fundamental limitation on the possibility to observe quantum phenomena at the macroscopic scale remains unclear. Here we implement a strict and simple protocol to test macroscopic realism in a light-matter-interfaced system. We create a micro-macro entanglement with two macroscopically distinguishable solid-state components and rule out those theories which would deny coherent superpositions of up to 76 atomic excitations shared by 1010{10}^{10}1010 ions in two separated solids. These results provide a general method to enhance the size of superposition states of atoms by utilizing quantum memory techniques and to push the envelope of macroscopicity at higher levels.
There are both fundamental and practical motivations for studying whether quantum entanglement can exist in macroscopic systems. However, multiparty entanglement is generally fragile and difficult to quantify. Dicke states are multiparty entangled states where a single excitation is delocalized over many systems. Building on previous work on quantum memories for photons, we create a Dicke state in a solid by storing a single photon in a crystal that contains many large atomic ensembles with distinct resonance frequencies. The photon is re-emitted at a well-defined time due to an interference effect analogous to multi-slit diffraction. We derive a lower bound for the number of entangled ensembles based on the contrast of the interference and the single-photon character of the input, and we experimentally demonstrate entanglement between over two hundred ensembles, each containing a billion atoms. We also illustrate the fact that each individual ensemble contains further entanglement.Multipartite entanglement is of both fundamental and practical interest, but is notoriously difficult to witness and characterise. Here, Zarkeshian et al. demonstrate multipartite entanglement in an atomic frequency comb storing a single photon in a Dicke state spread over a macroscopic ensemble.
Quantum mechanics is leading to many modern technologies, e.g. based on laser physics. Emerging fields are for example nonlinear optics, hybrid systems, or quantum communication. Despite these applications, there are still limitations of our understanding of quantum mechanics. Even though it is broadly accepted that decoherence limits the size of entangled states, we currently do not know how to overcome these limitations. How large can commonly entangled states be? Can we observe macroscopic quantum phenomena with coarse-grained detectors or even with our bare eyes? This thesis contributes towards answering these fundamental questions and to technological advances. The experiments are based on a light-matter platform of quantum optical states and atomic ensembles. The ensembles consist of rare-earth ion-doped crystals. Additionally, the atomic frequency comb protocol turns the ensemble into a quantum memory. In the scope of quantum communication we work on a quantum repeater. First, we investigate fundamental quantum mechanical states and their validity at macroscopic scales. We show that the detection of a collectively emitted excitation can be used to measure the size of the entangled ensemble. The entangled ensemble shared this excitation in a coherent superposition. This superposition of an atomic excitation in an ensemble is called W-state. We certify a new lower bound to the possible size of an entangled W-state between at least 16 million atoms. The proof of entanglement of this size relies on two measures: one determines the number of atoms involved in the storage process. The other one determines the state "quantumness" by examining the re-emitted light. Another experiment studies a macroscopically distinguishable superposition state. The superposition survives the storage in an atomic ensemble. Second, we perform two more experiments that contribute to a quantum repeater. One experiment probes the quantum states simultaneously stored in a multi-mode quantum memory. In this work we also develop the concept of indirect entanglement witness. For the other experiment, a frequency down-conversion platform is set up. The conversion overcomes the wavelength compatibility issue between some quantum memories and the telecommunication C-band. The narrow spectral filtering of the conversion performs better than expected. In summary, our work analyzes large entangled states and building blocks for a quantum repeater. The presented quantum memories are capable of temporal multi-mode storage. Its temporally precise re-emission is due to the re-phasing of the atoms of the W-state. We also show a good way to set up frequency down-conversion for the sake of quantum repeaters. This work emphasizes the atomic frequency comb protocol as a viable and reliable platform for quantum repeaters.
Quantum theory predicts that entanglement can also persist in macroscopic physical systems, albeit difficulties to demonstrate it experimentally remain. Recently, significant progress has been achieved and genuine entanglement between up to 2900 atoms was reported. Here, we demonstrate 16 million genuinely entangled atoms in a solid-state quantum memory prepared by the heralded absorption of a single photon. We develop an entanglement witness for quantifying the number of genuinely entangled particles based on the collective effect of directed emission combined with the non-classical nature of the emitted light. The method is applicable to a wide range of physical systems and is effective even in situations with significant losses. Our results clarify the role of multipartite entanglement in ensemble-based quantum memories and demonstrate the accessibility to certain classes of multipartite entanglement with limited experimental control.The presence of entanglement in macroscopic systems is notoriously difficult to observe. Here, the authors develop a witness which allow them to demonstrate entanglement between millions of atoms in a solid-state quantum memory prepared by the heralded absorption of a single photon.
The notion of a macroscopic quantum state must be pinned down in order to assess how well experiments probe the large-scale limits of quantum mechanics. However, the issue of quantifying so-called quantum macroscopicity is fraught with multiple approaches having varying interpretations and levels of computability and measurability. Here, we introduce two measures that capture independent macroscopic properties: i) extensive size, measuring the degree of coherence in position or momentum observables relative to atomic-scale units, and ii) entangled size, quantifying the number of entangled subsystems. These measures unify many desirable features of past proposals while having rigorously justified interpretations from quantum information theory in terms of coherence and multipartite entanglement. We demonstrate how to estimate them and obtain lower-bounds using experimental data from micro-mechanical oscillators and diffracting molecules. Notably, we find evidence for genuine multipartite entanglement of 10 5 to 10 7 atoms in recent mechanical superposition states.
Quantum correlations are correlations that arise from a unique feature in quantum mechanics: quantum superposition. The most famous example of quantum superposition is the Schrodinger’s cat state, where a cat is in a state of neither dead nor alive before an observer determines the cat’s status. This is not what we expect. Nevertheless, quantum superposition and correlations are routinely created in the laboratories with microscopic systems involving atoms and light particles. Can this counterintuitive notion be realised in the macroscopic world? This thesis investigates this question by devising criteria that certify the existence of quantum correlations in mesoscopic/macroscopic systems. Powerful mathematical tools are used to simulate two quantum protocols in a mesoscopic system which have applications in quantum communication and computation.