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arXiv:1509.08633 · Physical Review A

Green's-function formalism for waveguide QED applications

Michael P. Schneider, Tobias Sproll, Christina Stawiarski, Peter Schmitteckert, Kurt Busch

Published Jan 14, 2016• 38 citations
arXivHTMLPDF

Abstract

We present a quantum-field-theoretical framework based on path integrals and Feynman diagrams for the investigation of the quantum-optical properties of one-dimensional waveguiding structures with embedded quantum impurities. In particular, we obtain the Green's functions for a waveguide with an embedded two-level system in the single- and two-excitation sector for arbitrary dispersion relations both in the time and the frequency domains. In the single-excitation sector, we show how to sum the diagrammatic perturbation series to all orders and thus obtain explicit expressions for physical quantities such as the spectral density and the scattering matrix. In the two-excitation sector, we show that strictly linear dispersion relations exhibit the special property that the corresponding diagrammatic perturbation series terminates after two terms, again allowing for closed-form expressions for physical quantities. In the case of general dispersion relations, notably those exhibiting a band edge or waveguide cutoff frequencies, the perturbation series cannot be summed explicitly. Instead, we derive a self-consistent $T\text{-matrix}$ equation that reduces the computational effort to that of a single-excitation computation. This analysis allows us to identify a Fano resonance between the occupied quantum impurity and a free photon in the waveguide as a unique signature of the few-photon nonlinearity inherent in such systems. In addition, our diagrammatic approach allows for the classification of different physical processes such as the creation of photon-photon correlations and interaction-induced radiation trapping, the latter being absent for strictly linear dispersion relations. Our framework can serve as the basis for further studies that involve more complex scenarios such as several and many-level quantum impurities, networks of coupled waveguides, disordered systems, and nonequilibrium effects.

DOI
10.1103/physreva.93.013828

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We present a quantum-field-theoretical framework based on path integrals and Feynman diagrams for the investigation of the quantum-optical properties of one-dimensional waveguiding structures with embedded quantum impurities. In particular, we obtain the Green's functions for a waveguide with an embedded two-level system in the single- and two-excitation sector for arbitrary dispersion relations both in the time and the frequency domains. In the single-excitation sector, we show how to sum the diagrammatic perturbation series to all orders and thus obtain explicit expressions for physical quantities such as the spectral density and the scattering matrix. In the two-excitation sector, we show that strictly linear dispersion relations exhibit the special property that the corresponding diagrammatic perturbation series terminates after two terms, again allowing for closed-form expressions for physical quantities. In the case of general dispersion relations, notably those exhibiting a band edge or waveguide cutoff frequencies, the perturbation series cannot be summed explicitly. Instead, we derive a self-consistent T-matrixT\text{-matrix}T-matrix equation that reduces the computational effort to that of a single-excitation computation. This analysis allows us to identify a Fano resonance between the occupied quantum impurity and a free photon in the waveguide as a unique signature of the few-photon nonlinearity inherent in such systems. In addition, our diagrammatic approach allows for the classification of different physical processes such as the creation of photon-photon correlations and interaction-induced radiation trapping, the latter being absent for strictly linear dispersion relations. Our framework can serve as the basis for further studies that involve more complex scenarios such as several and many-level quantum impurities, networks of coupled waveguides, disordered systems, and nonequilibrium effects.
We study one- and two-photon scattering from a qubit embedded in a one-dimensional waveguide in the presence of modal dispersion. We use a resolvent based analysis and utilize techniques borrowed from the Lee model studies. Modal dispersion leads to atom-photon bound states which necessitate the use of multichannel scattering theory. We present multichannel scattering matrix elements in terms of the solution of a Fredholm integral equation of the second kind. Through the use of the Lippmann-Schwinger equation, we derive an infinite series of Feynman diagrams that represent the solution to the integral equation. We use the Feynman diagrams as vertex correction terms to come up with closed-form formulas that successfully predict the trapping rate of a photon in the atom-photon bound state. We verify our formalism through Krylov-subspace based numerical studies with pulsed excitations. Our results provide the tools to calculate the complex correlations between scattered photons in a dispersive environment.
We present a detailed quantum theory and simulations of few-photon Fock state pulses interacting with a two-level system (TLS) in an open waveguide-QED system. For a rectangular pulse shape, we present an exact temporal scattering theory to derive analytical expressions for the TLS population, using one-photon and two-photon pulses, for both chiral and symmetric emitters. We also derive the stationary (long-time) and time-dependent spectra for one-photon excitation, and show how these differ at a fundamental level when considering TLS population effects. Numerically, we also present matrix product state (MPS) simulations, which allow us to compute more general photon correlation functions for arbitrary quantum pulses, and we use this approach to also show results for Gaussian quantum pulses and to confirm the accuracy of our analytical solutions. In the case of a chiral TLS, we show how a one-photon pulse, of any temporal shape, yields a transmitted long-time spectrum that is identical to the input pulse, despite significant TLS population effects. However, the dynamical spectra and spectral intensity show rich population effects, allowing for their detection in spectroscopic experiments. We also show the striking differences between one-photon and two-photon excitation, where the latter shows clear signatures of nonlinear saturation effects. In addition, we demonstrate how significant population TLS dynamics also occur for pulses that are relatively long compared to the radiative decay time (showing that a weak excitation approximation, which neglects finite TLS population effects, cannot be made) and investigate the population signatures, nonlinear features and dynamical behavior as a function of quantum pulse length.
We present a method to systematically study multiphoton transmission in one-dimensional systems comprised of correlated quantum emitters coupled to input and output waveguides. Within the Green's function approach of the scattering matrix (S(S(S matrix), we develop a diagrammatic technique to analytically obtain the system's scattering amplitudes while at the same time visualize all the possible absorption and emission processes. Our method helps to reduce the significant effort in finding the general response of a many-body bosonic system, particularly the nonlinear response embedded in the Green's functions. We demonstrate our proposal through physically relevant examples involving scattering of multiphoton states from two-level emitters as well as from arrays of correlated Kerr nonlinear resonators in the Bose-Hubbard model.
Strong coupling between light and matter has been demonstrated both in classical cavity quantum electrodynamics (QED) systems and in more recent circuit-QED experiments. This enables the generation of strong nonlinear photon-photon interactions at the single-photon level, which is of great interest for the observation of quantum nonlinear optical phenomena, the control of light quanta in quantum information protocols such as quantum networking, as well as the study of strongly correlated quantum many-body systems using light. Recently, strong coupling has also been realized in a variety of one-dimensional (1D) waveguide- QED experimental systems, which in turn makes them promising candidates for quantum information processing. Compared to cavity-QED systems, there are two new features in waveguide-QED: the existence of a continuum of states and the restricted 1D phase space, which together bring in new physical effects, such as the bound-state effects. This thesis consists of two parts: 1) understanding the fundamental interaction between local quantum objects, such as two-level systems and four-level systems, and photons confined in the waveguide; 2) exploring its implications in quantum information processing, in particular photonic quantum computation and quantum key distribution. First, we demonstrate that by coupling a two-level system (TLS) or three/fourlevel system to a 1D continuum, strongly-correlated photons can be generated inside the waveguide. Photon-photon bound states, which decay exponentially as a function of the relative coordinates of photons, appear in multiphoton scattering processes. As a result, photon bunching and antibunching can be observed in the photon-photon correlation function, and nonclassical light source can be generated on demand. In the case of an N-type four-level system, we show that the effective photon-photon interaction mediated by the four-level system, gives rise to a variety of nonlinear optical phenomena, including photon blockade, photon-induced tunneling, and creation of single-photon states and photon pairs with a high degree of spectral entanglement, all in the absence of a cavity. However, to enable greater quantum networking potential using waveguide- QED, it is important to study systems having more than just one TLS/qubit. We develop a numerical Green function method to study cooperative effects in a system of two qubits coupled to a 1D waveguide. Quantum beats emerge in photon-photon correlations, and persist to much longer time scales because of non-Markovian processes. In addition, this system can be used to generate a high-degree of long-distance entanglement when one of the two qubits is driven by an on-resonance laser, further paving the way toward waveguide-QED-based quantum networks. Furthermore, based on our study of light-matter interactions in waveguide- QED, we investigate its implications in quantum information processing. First, we study quantum key distribution using the sub-Possonian single photon source obtained by scattering a coherent state off a two-level system. The rate for key generation is found to be twice as large as for other sources. Second, we propose a new scheme for scalable quantum computation using flying qubits--propagating photons in a one-dimensional waveguide--interacting with matter qubits. Photonphoton interactions are mediated by the coupling to a three- or four-level system, based on which photon-photon -phase gates (Controlled-NOT) can be implemented for universal quantum computation. We show that high gate fidelity is possible given recent dramatic experimental progress in superconducting circuits and photonic-crystal waveguides. The proposed system can be an important building block for future on-chip quantum networks.
We provide a theoretical and computational framework for fully quantum mechanical studies of few-photon transport phenomena in arbitrary waveguiding structures in the presence of coherent interaction with optically active emitters. The reduced dimensionality of such systems leads to pronounced quantum interference effects that may be exploited for a number of applications and we apply our framework to the case of single-photon transport through a two-level atom. In this system, the atom's emission dynamics leads to strong interference effects that can be used for the realization of nanomirrors.
This work presents a full-wave Green's function framework for modeling collective and coherent single-photon emission from multiple quantum emitters embedded in complex electromagnetic structures. Starting from a transverse modal completeness relation of modified Langevin noise formalism, we derive a closed set of coupled equations for population dynamics and frequency-resolved field amplitudes in the single-excitation regime. Since the electromagnetic reservoir is not traced out at the level of the dynamical amplitudes, the emitted single-photon dynamics can be modeled within the same closed set of equations without Markovian approximation in open and dissipative environments. We demonstrate that finite-bandwidth truncation of the spectral density leads to systematic deviations in coherent dispersive interactions, even when dissipative rates appear converged. To restore causal consistency, we introduce a counter-term compensation scheme that restores the missing dispersive contributions without modifying the retained non-Markovian memory kernel. To validate the scheme and demonstrate the practicality of the proposed framework, we present numerical examples ranging from benchmark configurations to a three-dimensional dispersive ring-resonator structure via finite element method. These capabilities provide a practical route for rigorously incorporating full-wave electromagnetic simulations into non-Markovian multi-emitter quantum electrodynamics, enabling predictive modeling of collective emission, coherent energy exchange, and single-photon radiation in realistic open structures.