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arXiv:1509.03159 · Physical Review A

Simultaneous generation of two spin-wave–photon entangled states in an atomic ensemble

Yuelong Wu, Long Tian, Zhongxiao Xu, Wei Ge, Lirong Chen, Shujing Li, Haoxiang Yuan, Yafei Wen, Hai Wang, Changde Xie, Kunchi Peng

Published May 19, 2016• 14 citations
arXivHTMLPDF

Abstract

Spontaneous Raman scattering (SRS) in atomic ensembles provides a promising method to generate spin-wave--photon entangled states. In the past experiments, a spin-wave--photon entangled state was produced via SRS from an atomic ensemble. Here, we report a scheme of simultaneously generating two spin-wave--photon (atom-photon) entangled states in a cold Rb ensemble via SRS. Based on joint Bell-state measurements on the two photons coming from the two atom-photon entangled sources, respectively, we projected the two stored spin waves into a Bell state and then mapped the quantum memory into a polarization-entangled photon pair. Such a polarization-entangled photon pair can be released on demand and thus the presented scheme has potential application in the preparation of large-size photonic entangled states.

DOI
10.1103/physreva.93.052327

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Spontaneous Raman scattering (SRS) in atomic ensembles provides a promising method to generate spin-wave--photon entangled states. In the past experiments, a spin-wave--photon entangled state was produced via SRS from an atomic ensemble. Here, we report a scheme of simultaneously generating two spin-wave--photon (atom-photon) entangled states in a cold Rb ensemble via SRS. Based on joint Bell-state measurements on the two photons coming from the two atom-photon entangled sources, respectively, we projected the two stored spin waves into a Bell state and then mapped the quantum memory into a polarization-entangled photon pair. Such a polarization-entangled photon pair can be released on demand and thus the presented scheme has potential application in the preparation of large-size photonic entangled states.
Entanglement swapping (ES) between memory repeater links is critical for establishing quantum networks via quantum repeaters. So far, ES with atomic-ensemble-based memories has not been achieved. Here, we experimentally demonstrated ES between two entangled pairs of spin-wave memories via Duan-Lukin-Cirac-Zoller scheme. With a cloud of cold atoms inserted in a cavity, we produce non-classically-correlated spin-wave-photon pairs in 12 spatial modes and then prepare two entangled pairs of spin-wave memories via a multiplexed scheme. Via single-photon Bell measurement on retrieved fields from two memories, we project the two remaining memories never entangled previously into an entangled state with the measured concurrence of C = 0.0124(0.003). The successful probability of ES in our scheme is increased by three times, compared with that in non-multiplexed scheme. Our presented work shows that the generation of entanglement (C>0) between the remaining memory ensembles requires the average cross-correlation function of the spin-wave-photon pairs to be >30 .
We report a polarization-entangled photon-pair source obtained via spontaneous four-wave mixing (SFWM) in a Doppler-broadened atomic ensemble of ^{87}Rb atoms using a Sagnac interferometer. Collective two-photon coherence occurs in the Doppler-broadened ladder-type atomic system with bidirectional counterpropagating two-photon resonant pump and coupling fields; hence, polarization-entangled photon pairs are collectively radiated in the phase-matched direction. Without phase stabilization of the interferometry for polarization entanglement, we robustly produce all four Bell states via a polarization Sagnac configuration. The brightness, stability, and temporal purity advantages provided by our polarization-entangled SFWM photon-pair source have very important applications in the context of a practical scalable quantum network.
In spontaneous Raman scattering in an atomic ensemble, a collective atomic spin wave is created in correlation with the Stokes field. When the Stokes photons from two or more such atomic ensembles are made indistinguishable, a 'which-way' collective atomic spin excitation is generated among the independent atomic ensembles. We demonstrate this phenomenon experimentally by reading out the atomic spin excitations and observing interference between the read-out beams. When a single-photon projective measurement is made on the indistinguishable Stokes photons, this simple scheme can be used to entangle independent atomic ensembles. Compared to other currently used methods, this scheme can be easily scaled up and has greater efficiency.
We propose a scheme of heralded storages of single photons via spontaneous Raman scattering (SRS) enhanced by a chiral standing-wave cavity, which creates a non-classically correlated pair of a spin wave and a Stokes photon (heralded photon) when a single-photon “write” pulse is applied to an atomic ensemble. In this scheme, to decrease the power of the write pulse for SRS, the write laser and the Stokes fields are aligned to propagate near-collinearly through the atoms. The short storage lifetime remains a challenge in standing-wave cavity-enhanced SRS. To prolong the storage lifetime, we achieve a long-wavelength spin-wave memory by removing the backward-scattering Stokes field from the cavity, which is realized by using non-reciprocal couplings between the Stokes fields and the atoms. In the experiment, the memory lifetime is demonstrated up to ∼100 μs, which is beyond the limitation (∼350 ns) of the storage in the atomic ensembles coupled to standing-wave cavities. We achieve a spin-wave memory for the write pulse containing a mean photon number of ∼4. The quantum correlation of the Stokes-spin-wave pairs is beyond 2, which gives strong evidence of non-classical behavior.
In this paper we consider the optical coupling of two four-level atoms via cooperative Raman scattering of correlated photons of the nondegenerate spontaneous parametric radiation. The Raman scattering of twin photons incident on the atoms is additionally stimulated by coherent classical radiation in such a way that it is slightly off resonant for each atom considered independently but resonant for the joint system. We discuss the special excitation conditions when the amplitude of the cooperative stimulated Raman scattering from quantum to classical modes becomes greater than the normal transition rates associated with independent Raman scattering. In certain conditions weak entanglement between the Zeeman sublevels in the ground states of these atoms can appear. The small admixture of entanglement in the system of two atoms leads to strong entanglement between transverse macroscopic spin fluctuations of two spatially separated atomic ensembles coupled by such quantum light. The proposed mechanism of entanglement is relevant to the ground state spin subsystem of two distant macroscopic and optically thin atomic ensembles. Such an entangled state can be stored for a long time and used as a basic Einstein-Podolsky-Rosen system in different applications pursuing the goal of spreading quantum information schemes in atomic subsystems.
A source that can generate atom-photon quantum correlations or entanglement based on a quantum memory is a basic building block of quantum repeaters (QRs). To achieve high entanglement generation rates in ensemble-based QRs, spatial-, temporal-, and spectral-multimode memories are needed. Previous temporal-multimode memories are based on rephasing mechanisms in inhomogeneously broadened media. Here, by applying a train of write pulses in time, with each pulse coming from a different direction, to a homogeneously broadened atomic ensemble to induce Duan-Lukin-Cirac-Zoller-like Raman processes, we prepare up to 19 pairs of modes, namely, one spin-wave mode and one photonic time bin. Spin-wave-photon (i.e., atom-photon) entanglement is probabilistically produced in these mode pairs. Based on the stored spin-wave modes together with feedforward-controlled readout, we build a temporally multiplexed source and then demonstrate an 18.8-fold increase in the probability of the generation of spin-wave-photon entanglement compared to the sources that use individual modes. The measured Bell parameter for the multiplexed source is $2.30\ifmmode\pm\else\textpm\fi{}0.02$, and the memory lifetime is 30 \ensuremath{\mu}s.