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arXiv:1509.02519 · Physical review. B./Physical review. B

Heat diffusion in the disordered electron gas

Georg Schwiete, Alexander M. Finkel’stein

Published Mar 11, 2016• 13 citations
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Abstract

We study the thermal conductivity of the disordered two-dimensional electron gas. To this end, we analyze the heat density--heat density correlation function concentrating on the scattering processes induced by the Coulomb interaction in the subtemperature energy range. These scattering processes are at the origin of logarithmic corrections violating the Wiedemann-Franz law. Special care is devoted to the definition of the heat density in the presence of the long-range Coulomb interaction. To clarify the structure of the correlation function, we present details of a perturbative calculation. While the conservation of energy strongly constrains the general form of the heat density--heat density correlation function, the balance of various terms turns out to be rather different from that for the correlation functions of other conserved quantities such as the density-density or spin density--spin density correlation function.

DOI
10.1103/physrevb.93.115121

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We study the thermal conductivity of the disordered two-dimensional electron gas. To this end, we analyze the heat density--heat density correlation function concentrating on the scattering processes induced by the Coulomb interaction in the subtemperature energy range. These scattering processes are at the origin of logarithmic corrections violating the Wiedemann-Franz law. Special care is devoted to the definition of the heat density in the presence of the long-range Coulomb interaction. To clarify the structure of the correlation function, we present details of a perturbative calculation. While the conservation of energy strongly constrains the general form of the heat density--heat density correlation function, the balance of various terms turns out to be rather different from that for the correlation functions of other conserved quantities such as the density-density or spin density--spin density correlation function.
We present a detailed study of thermal transport in the disordered Fermi liquid with short-range interactions. At temperatures smaller than the impurity scattering rate, i.e., in the diffusive regime, thermal conductivity acquires nonanalytic quantum corrections. When these quantum corrections become large at low temperatures, the calculation of thermal conductivity demands a theoretical approach that treats disorder and interactions on an equal footing. In this paper, we develop such an approach by merging Luttinger's idea of using gravitational potentials for the analysis of thermal phenomena with a renormalization group calculation based on the Keldysh nonlinear sigma model. The gravitational potentials are introduced in the action as auxiliary sources that couple to the heat density. These sources are a convenient tool for generating expressions for the heat density and its correlation function from the partition function. Already in the absence of the gravitational potentials, the nonlinear sigma model contains several temperature-dependent renormalization group charges. When the gravitational potentials are introduced into the model, they acquire an independent renormalization group flow. We show that this flow preserves the phenomenological form of the correlation function, reflecting its relation to the specific heat and the constraints imposed by energy conservation. The main result of our analysis is that the Wiedemann-Franz law holds down to the lowest temperatures even in the presence of disorder and interactions and despite the quantum corrections that arise for both the electric and thermal conductivities.
We study the heat conductivity in Anderson insulators in the presence of a power-law interaction. Particle-hole excitations built on localized electron states are viewed as two-level systems randomly distributed in space and energy and coupled due to electron-electron interaction. A small fraction of these states form resonant pairs that in turn build a complex network allowing for energy propagation. We identify the character of energy transport through this network and evaluate the thermal conductivity. For physically relevant cases of two-dimensional and three-dimensional spin systems with 1/r31/{r}^{3}1/r3 dipole-dipole interaction (originating from the conventional 1/r1/r1/r Coulomb interaction between electrons), the found thermal conductivity $\ensuremath{\kappa}$ scales with temperature as $\ensuremath{\kappa}\ensuremath{\propto}{T}^{3}$ and $\ensuremath{\kappa}\ensuremath{\propto}{T}^{4/3}$, respectively. Our results may be of relevance also to other realizations of random spin Hamiltonians with long-range interactions.
We consider heat transport in a Luttinger liquid (LL) with weak disorder and study the Lorenz number for this system. We start at a high- T regime, and calculate both the electrical and thermal conductivities using a memory function approach. The resulting Lorenz number L is independent of T but depends explicitly on the LL exponents. Lowering T , however, allows for a renormalization of the LL exponents from their bare values by disorder, causing a violation of the Wiedemann-Franz law. Finally, we extend the discussion to quantum wire systems and study the wire size dependence of the Lorenz number.
We study nonperturbative interaction corrections to the thermodynamic quantities of multichannel disordered wires in the presence of the Coulomb interactions. Within the replica nonlinear $\ensuremath{\sigma}$-model $(\mathrm{NL}\ensuremath{\sigma}\mathrm{M})$ formalism, they arise from nonperturbative soliton saddle points of the $\mathrm{NL}\ensuremath{\sigma}\mathrm{M}$ action. The problem is reduced to evaluating the partition function of a replicated classical one-dimensional Coulomb gas. The state of the latter depends on two parameters: the number of transverse channels in the wire Nch{N}_{\mathit{ch}}Nch​ and the dimensionless conductance G(LT)G({L}_{T})G(LT​) of a wire segment of length equal to the thermal diffusion length LT{L}_{T}LT​. At relatively high temperatures, $G({L}_{T})\ensuremath{\gtrsim}\mathrm{ln}\phantom{\rule{0.2em}{0ex}}{N}_{\mathit{ch}}$, the gas is dimerized, i.e., consists of bound neutral pairs. At lower temperatures, $\mathrm{ln}\phantom{\rule{0.2em}{0ex}}{N}_{\mathit{ch}}\ensuremath{\gtrsim}G({L}_{T})\ensuremath{\gtrsim}1$, the pairs overlap and form a Coulomb plasma. The crossover between the two regimes occurs at a parametrically large conductance $G({L}_{T})\ensuremath{\sim}\mathrm{ln}\phantom{\rule{0.2em}{0ex}}{N}_{\mathit{ch}}$ and may be studied independently from the perturbative effects. Specializing on the high-temperature regime, we obtain the leading nonperturbative correction to the wire heat capacity. Its ratio to the heat capacity for noninteracting electrons, C0{C}_{0}C0​, is $\ensuremath{\delta}C∕{C}_{0}\ensuremath{\sim}{N}_{\mathit{ch}}{G}^{2}({L}_{T}){e}^{\ensuremath{-}2G({L}_{T})}$.
The fluctuation-dissipation theorem is applied to the study of the pair correlation functions of the system containing charged particles which is not invariant under spatial translation. The results are expressed in terms of the longitudinal response functions and involve correlation functions which depend only on screened short-range Coulomb interactions S0{S}_{0}S0​. In the case of the electron gas, the density-density correlation function is $S(\mathbf{r}{\mathbf{r}}^{\ensuremath{'}};\ensuremath{\omega})=[\ensuremath{\delta}(\mathbf{r}\ensuremath{-}\mathbf{R})\ensuremath{-}K(r{\mathbf{R}}^{\ensuremath{'}\ensuremath{'}};\ensuremath{\omega})v({\mathbf{R}}^{\ensuremath{'}\ensuremath{'}}\mathbf{R})]{S}_{0}(\mathbf{R}{\mathbf{R}}^{\ensuremath{'}};\ensuremath{\omega})[\ensuremath{\delta}({\mathbf{R}}^{\ensuremath{'}}\ensuremath{-}{\mathbf{r}}^{\ensuremath{'}})\ensuremath{-}v({\mathbf{R}}^{\ensuremath{'}}{\mathbf{R}}^{\ensuremath{'}\ensuremath{'}\ensuremath{'}})\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{K}({\mathbf{R}}^{\ensuremath{'}\ensuremath{'}\ensuremath{'}}{\mathbf{r}}^{\ensuremath{'}};\ensuremath{-}\ensuremath{\omega})]$where KKK is the response function of the electron density to an external potential field, and $\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{K}$ its conjugate; vvv represents the Coulomb interaction; and the repeated spatial coordinates are integrated over the volume. It is shown that this expression implies the principle of superposition of dressed particles (the bare particles plus their associated screening clouds); for the calculations of the correlation functions, the dressed particles may be superposed without further consideration of the long-range parts of Coulomb interactions. Similar reductions are carried out for the various correlation functions in the electron-ion system, and the superposition principle is confirned. A possible extension of the results to a nonequilibrium stationarysystem is suggested and discussed. The interrelationship among various longitudinal response functions, which is characteristic of the inhomogeneous system, is discussed and clarified. Simplifications arising from the homogeneity and discussions from diagrammatic considerations are given in Appendices.
We derive analytical expressions for the spectral moments of the dynamical response functions of the Hubbard model using the high-temperature series expansion. We consider generic dimension ddd as well as the infinite-ddd limit, arbitrary electron density nnn, and both finite and infinite repulsion UUU. We use moment-reconstruction methods to obtain the one-electron spectral function, the self-energy, and the optical conductivity. They are all smooth functions at high temperature and, at large UUU, they are featureless with characteristic widths of the order of the lattice hopping parameter ttt. In the infinite-ddd limit, we compare the series expansion results with accurate numerical renormalization group and interaction expansion quantum Monte Carlo results. We find excellent agreement down to surprisingly low temperatures, throughout most of the bad-metal regime, which applies for $T\ensuremath{\gtrsim}(1\ensuremath{-}n)D$, the Brinkman-Rice scale. The resistivity increases linearly in TTT at high temperature without saturation. This results from the 1/T1/T1/T behavior of the compressibility or kinetic energy, which play the role of the effective carrier number. In contrast, the scattering time (or diffusion constant) saturates at high TTT. We find that $\ensuremath{\sigma}(n,T)\ensuremath{\approx}(1\ensuremath{-}n)\ensuremath{\sigma}(n=0,T)$ to a very good approximation for all nnn, with $\ensuremath{\sigma}(n=0,T)\ensuremath{\propto}t/T$ at high temperatures. The saturation at small nnn occurs due to a compensation between the density dependence of the effective number of carriers and that of the scattering time. The TTT dependence of the resistivity displays a kneelike feature which signals a crossover to the intermediate-temperature regime where the diffusion constant (or scattering time) starts increasing with decreasing TTT. At high temperatures, the thermopower obeys the Heikes formula, while the Wiedemann-Franz law is violated with the Lorenz number vanishing as 1/T21/{T}^{2}1/T2. The relevance of our calculations to experiments probing high-temperature transport in materials with strong electronic correlations or ultracold atomic gases in an optical lattice is briefly discussed.