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arXiv:1509.00854 · Physical Review Letters

Formation and Dynamics of Antiferromagnetic Correlations in Tunable Optical Lattices

Daniel Greif, Gregor Jotzu, Michael Messer, Rémi Desbuquois, Tilman Esslinger

Published Dec 23, 2015• 86 citations
arXivHTMLPDF

Abstract

We report on the observation of antiferromagnetic correlations of ultracold fermions in a variety of optical lattice geometries that are well described by the Hubbard model, including dimers, 1D chains, ladders, isolated and coupled honeycomb planes, as well as square and cubic lattices. The dependence of the strength of spin correlations on the specific geometry is experimentally studied by measuring the correlations along different lattice tunneling links, where a redistribution of correlations between the different lattice links is observed. By measuring the correlations in a crossover between distinct geometries, we demonstrate an effective reduction of the dimensionality for our atom numbers and temperatures. We also investigate the formation and redistribution time of spin correlations by dynamically changing the lattice geometry and studying the time evolution of the system. Time scales ranging from a sudden quench of the lattice geometry to an adiabatic evolution are probed.

DOI
10.1103/physrevlett.115.260401

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We report on the observation of antiferromagnetic correlations of ultracold fermions in a variety of optical lattice geometries that are well described by the Hubbard model, including dimers, 1D chains, ladders, isolated and coupled honeycomb planes, as well as square and cubic lattices. The dependence of the strength of spin correlations on the specific geometry is experimentally studied by measuring the correlations along different lattice tunneling links, where a redistribution of correlations between the different lattice links is observed. By measuring the correlations in a crossover between distinct geometries, we demonstrate an effective reduction of the dimensionality for our atom numbers and temperatures. We also investigate the formation and redistribution time of spin correlations by dynamically changing the lattice geometry and studying the time evolution of the system. Time scales ranging from a sudden quench of the lattice geometry to an adiabatic evolution are probed.
The exchange coupling between quantum mechanical spins lies at the origin of quantum magnetism. We report on the observation of nearest-neighbor magnetic spin correlations emerging in the many-body state of a thermalized Fermi gas in an optical lattice. The key to obtaining short-range magnetic order is a local redistribution of entropy within the lattice structure. This is achieved in a tunable-geometry optical lattice, which also enables the detection of the magnetic correlations. We load a low-temperature two-component Fermi gas with repulsive interactions into either a dimerized or an anisotropic simple cubic lattice. For both systems the correlations manifest as an excess number of singlets as compared to triplets consisting of two atoms with opposite spins. For the anisotropic lattice, we determine the transverse spin correlator from the singlet-triplet imbalance and observe antiferromagnetic correlations along one spatial axis. Our work paves the way for addressing open problems in quantum magnetism using ultracold fermions in optical lattices as quantum simulators.
Quantum magnetism originates from the exchange coupling between quantum mechanical spins. Here, we report on the observation of nearest-neighbor magnetic correlations emerging in the many-body state of a thermalized Fermi gas in an optical lattice. The key to obtaining short-range magnetic order is a local redistribution of entropy, which allows temperatures below the exchange energy for a subset of lattice bonds. When loading a repulsively interacting gas into either dimerized or anisotropic simple cubic configurations of a tunable-geometry lattice, we observe an excess of singlets as compared with triplets consisting of two opposite spins. For the anisotropic lattice, the transverse spin correlator reveals antiferromagnetic correlations along one spatial axis. Our work facilitates addressing open problems in quantum magnetism through the use of quantum simulation.
We study the effects of anisotropic hopping amplitudes on quantum phases of ultracold fermions in optical lattices described by the repulsive Fermi-Hubbard model. In particular, using dynamical mean-field theory (DMFT) we investigate the dimensional crossover between the isotropic square and the isotropic cubic lattice. We analyze the phase transition from the antiferromagnetic to the paramagnetic state and observe a significant change in the critical temperature: depending on the interaction strength, the anisotropy can lead to both a suppression or increase. We also investigate the localization properties of the system, such as the compressibility and double occupancy. Using the local-density approximation in combination with DMFT we conclude that density profiles can be used to detect the mentioned anisotropy-driven transitions.
Recently, it has become possible to tune optical lattices continuously between square and triangular geometries. We compute thermodynamics and spin correlations in the corresponding Hubbard model using a determinant quantum Monte Carlo technique and show that the frustration effects induced by the variable hopping terms can be clearly separated from concomitant bandwidth changes by a proper rescaling of the interaction. An enhancement of the double occupancy by geometric frustration signals the destruction of nontrivial antiferromagnetic correlations at weak coupling and entropy $s\ensuremath{\lesssim}\mathrm{ln}(2)$ (and restores Pomeranchuk cooling at strong frustration), paving the way to the long-sought experimental detection of antiferromagnetism in ultracold fermions on optical lattices.
Simulating the real-time evolution of quantum spin systems far out of equilibrium poses a major theoretical challenge, especially in more than one dimension.We experimentally explore quench dynamics in a two-dimensional Ising spin system with transverse and longitudinal fields.We realize the system with a near unit-occupancy atomic array of over 200 atoms obtained by loading a spin-polarized band insulator of fermionic lithium into an optical lattice and induce short-range interactions by direct excitation to a lowlying Rydberg state.Using site-resolved microscopy, we probe antiferromagnetic correlations in the system after a sudden quench from a paramagnetic state and compare our measurements to numerical calculations using state-of-the-art techniques.We achieve many-body states with longer-range antiferromagnetic correlations by implementing a near-adiabatic quench of the longitudinal field and study the buildup of correlations as we vary the rate with which we change the field.
This thesis reports on the microscopic investigation of antiferromagnetic order in Hubbard chains, realized with ultracold repulsively interacting fermions in an optical lattice. Extending a quantum gas microscope on spin resolution opened the possibility to Access the full charge and spin statistics of a strongly correlated fermionic many body system. Using this technique, we measured antiferromagnetic correlations over distances up to three lattice sites. Starting with a repulsive degenerate two component mixture of 6Li atoms trapped in a single plane of a vertical lattice, we loaded the Atoms into one-dimensional tubes of a transverse optical superlattice. By adiabatically ramping up the lattice potential along the tubes, we isentropically entered the strongly correlated regime of the one-dimensional Fermi-Hubbard Hamiltonian. We spatially separated the two spin states into opposite sites of local double wells orthogonal to the direction of the lattice before single atom and site sensitive imaging. In this way we extracted the spin information of every single lattice site and were able to evaluate spin-spin correlations. The two component degenerate gases were produced with sub-Poissonian atom number fluctuations by magnetically driven evaporative cooling in vicinity of a Feshbach resonance, used to set the scattering length. The dependence of antiferromagnetic correlations on the driving superexchange coupling was experimentally investigated by varying the interparticle scattering length before loading the atoms into the optical lattice. Taking advantage of the underlying trapping potential of the optical lattice, which shaped the filling and the entropy of the gases, the influence of density excitations and different entropies on spin correlations was observed. By post-selecting the Hubbard chains based on their average filling and local atom number fluctuations, spin correlations corresponding to 58% of the zero temperature predictions in the Heisenberg regime were measured. By comparing the obtained antiferromagnetic correlations to Quantum-Monte-Carlo predictions for our System the lowest measured entropy per particle could be stated as s = 0.51(4)kB, clearly below the critical value of s = ln(2)kB, which is required to form longer ranged correlations. Below this critical entropy, in contrast to local density fluctuations, these spin correlations strongly depend on the entropy of the system. In the future, such a spin thermometer can be used to benchmark novel cooling techniques, which are required to enter the temperature regime of d-wave superconducting states. The access to the full particle and spin statistics will enable us to read out multi-point correlation functions, which characterize such exotic states of matter.