Using state-selective field ionization, the state distributions of Rydberg atoms in cold Rydberg gases are measured for various initially excited Rydberg levels, populations, and evolution times. We provide direct experimental evidence for
l-changing collisions that we previously observed indirectly [S. K. Dutta, D. Feldbaum, A. Walz-Flannigan, J. R. Guest, and G. Raithel, Phys. Rev. Lett. 86, 3993 (2001)]. We also observe
n-mixing and find that its effects are largely in agreement with recent theoretical work on
n-changing collisions between electrons and Rydberg atoms, thus enabling an estimation of the electron temperature. Unexpectedly large populations of atoms are found in states with principal quantum numbers much lower than that of the initially excited atoms. We explain this observation by collisions between high-
l Rydberg atoms, which are highly polar and can collide due to static electric-dipole forces between them.
We present experimental results on the controlled deexcitation of Rydberg states in a cold gas of Rb atoms. The effect of the van der Waals interactions between the Rydberg atoms is clearly seen in the deexcitation spectrum and dynamics. Our observations are confirmed by numerical simulations. In particular, for off-resonant (facilitated) excitation we find that the deexcitation spectrum reflects the spatial arrangement of the atoms in the quasi-one-dimensional geometry of our experiment. We discuss future applications of this technique and implications for detection and controlled dissipation schemes.
In the last twenty years, Rydberg atoms have become a versatile and much studied system for implementing quantum many-body systems in the framework of quantum computation and quantum simulation. However, even in the absence of coherent evolution Rydberg systems exhibit interesting and non-trivial many-body phenomena such as kinetic constraints and non-equilibrium phase transitions that are relevant in a number of research fields. Here we review our recent work on such systems, where dissipation leads to incoherent dynamics and also to population decay. We show that those two effects, together with the strong interactions between Rydberg atoms, give rise to a number of intriguing phenomena that make cold Rydberg atoms an attractive test-bed for classical many-body processes and quantum generalizations thereof.
In the last twenty years, Rydberg atoms have become a versatile and much studied system for implementing quantum many-body systems in the framework of quantum computation and quantum simulation. However, even in the absence of coherent evolution Rydberg systems exhibit interesting and non-trivial many-body phenomena such as kinetic constraints and non-equilibrium phase transitions that are relevant in a number of research fields. Here we review our recent work on such systems, where dissipation leads to incoherent dynamics and also to population decay. We show that those two effects, together with the strong interactions between Rydberg atoms, give rise to a number of intriguing phenomena that make cold Rydberg atoms an attractive test-bed for classical many-body processes and quantum generalizations thereof.
We explore the relaxation dynamics of elementary spin clusters in a kinetically constrained spin system. Inspired by experiments with Rydberg lattice gases, we focus on the situation in which an excited spin leads to a "facilitated" excitation of a neighboring spin. We show that even weak interactions that extend beyond nearest neighbors can have a dramatic impact on the relaxation behavior: they generate a linear potential, which under certain conditions leads to the onset of Bloch oscillations of spin clusters. These hinder the expansion of a cluster and, more generally, the relaxation of many-body states toward equilibrium. This shows that nonergodic behavior in kinetically constrained systems may occur as a consequence of the interplay between reduced connectivity of many-body states and weak interparticle interactions. We furthermore show that the emergent Bloch oscillations identified here can be detected in experiment through measurements of the Rydberg atom density and discuss how spin-orbit coupling between internal and external degrees of freedom of spin clusters can be used to control their relaxation behavior.