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arXiv:1507.06973 · Physica Scripta

Why the laser linewidth is so narrow: a modern perspective

Alexander Cerjan, A. Douglas Stone

Published Dec 8, 2015• 15 citations
arXivHTMLPDF

Abstract

Abstract We review and interpret a modern approach to laser theory, steady-state ab initio laser theory (SALT), which treats lasing and amplification in a unified manner as a non-unitary scattering problem described by a nonlinear scattering matrix. Within the semiclassical version of the theory the laser line has zero width as the lasing mode corresponds to the existence of an eigenvector of the S -matrix with diverging eigenvalue due to the occurrence of a pole of the scattering matrix on the real axis. In this approach the system is infinite from the outset and no distinction is made between cavity modes and modes of the Universe; lasing modes exist both in the cavity and in the external region as solutions satisfying Sommerfeld radiation boundary conditions. We discuss how such solutions can be obtained by a limiting procedure in a finite box with damping according to the limiting absorption principle. When the electromagnetic and matter fields are treated as operators, quantum fluctuations enter the relevant correlation functions and a finite linewidth is obtained, via a generalization of SALT to include noise (N-SALT). N-SALT leads to an analytic formula for the linewidth that is more general than all previous corrected versions of the Schawlow–Townes formula, and can be evaluated simply from knowledge of the semiclassical SALT modes. We derive a simpler version of this formula which emphasizes that the noise is dominated by the fluctuations in the polarization of the gain medium and is controlled by the rate of spontaneous emission.

DOI
10.1088/0031-8949/91/1/013003

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Abstract We review and interpret a modern approach to laser theory, steady-state ab initio laser theory (SALT), which treats lasing and amplification in a unified manner as a non-unitary scattering problem described by a nonlinear scattering matrix. Within the semiclassical version of the theory the laser line has zero width as the lasing mode corresponds to the existence of an eigenvector of the S -matrix with diverging eigenvalue due to the occurrence of a pole of the scattering matrix on the real axis. In this approach the system is infinite from the outset and no distinction is made between cavity modes and modes of the Universe; lasing modes exist both in the cavity and in the external region as solutions satisfying Sommerfeld radiation boundary conditions. We discuss how such solutions can be obtained by a limiting procedure in a finite box with damping according to the limiting absorption principle. When the electromagnetic and matter fields are treated as operators, quantum fluctuations enter the relevant correlation functions and a finite linewidth is obtained, via a generalization of SALT to include noise (N-SALT). N-SALT leads to an analytic formula for the linewidth that is more general than all previous corrected versions of the Schawlow–Townes formula, and can be evaluated simply from knowledge of the semiclassical SALT modes. We derive a simpler version of this formula which emphasizes that the noise is dominated by the fluctuations in the polarization of the gain medium and is controlled by the rate of spontaneous emission.
We perform a first-principles calculation of the quantum-limited laser linewidth, testing the predictions of recently developed theories of the laser linewidth based on fluctuations about the known steady-state laser solutions against traditional forms of the Schawlow-Townes linewidth. The numerical study is based on finite-difference time-domain simulations of the semiclassical Maxwell-Bloch lasing equations, augmented with Langevin force terms, and includes the effects of dispersion, losses due to the open boundary of the laser cavity, and non-linear coupling between the amplitude and phase fluctuations (α factor). We find quantitative agreement between the numerical results and the predictions of the noisy steady-state ab initio laser theory (N-SALT), both in the variation of the linewidth with output power, as well as the emergence of side-peaks due to relaxation oscillations.
A recent SSS-matrix-based theory of the quantum-limited linewidth, which is applicable to general lasers, including spatially nonuniform laser cavities operating above threshold, is analyzed in various limits. For broadband gain, a simple interpretation of the Petermann and bad-cavity factors is presented in terms of geometric relations between the zeros and poles of the SSS matrix. When there is substantial dispersion, on the frequency scale of the cavity lifetime, the theory yields a generalization of the bad-cavity factor, which was previously derived for spatially uniform one-dimensional lasers. This effect can lead to sub--Schawlow-Townes linewidths in lasers with very narrow gain widths. We derive a formula for the linewidth in terms of the lasing mode functions, which has accuracy comparable to the previous formula involving the residue of the lasing pole. These results for the quantum-limited linewidth are valid even in the regime of strong line pulling and spatial hole burning, where the linewidth cannot be factorized into independent Petermann and bad-cavity factors.
In this thesis we generalize and extend the steady-state ab initio laser theory (SALT), first developed by Türeci and Stone, and apply it problems in laser design. SALT as first formulated modeled the gain medium as identical two-level atoms, leading to the well-known Maxwell Bloch laser equations. The result is a set of coupled non-linear wave equations that treats the openness of the cavity exactly and the non-linear modal interactions to infinite order. Most gain media have more than two atomic levels, and in this thesis we generalize the SALT equations to treat realistic and complex gain media, specifically N-level atomic media with a single lasing transition, N-level atomic media with multiple lasing transitions and semiconductor gain media with particle-hole band excitations. The extension to multiple transitions requires fundamentally enlarging the set of SALT equations, by adding a set of population equations that must be solved self-consistently with the non-linear wave equations for the lasing modes in standard SALT. In addition, the population equation can be generalized to treat gain diffusion, an important problem in a number of laser systems, not treated in SALT or in most earlier laser theories. The semiconductor version (Semi-SALT) includes the continuum of particle-hole transitions and the effect of Pauli blocking of transitions, but is only developed and applied in the free-carrier approximation. The resulting theory is termed complex SALT (C-SALT). We also demonstrate how to incorporate amplification and injected signals naturally within the SALT framework, yielding injection SALT (I-SALT). The generalization to I-SALT leads to a larger set of self-consistent coupled non-linear wave equations, a set for the lasing modes and a set for the injected and amplified fields, coupled through cross gain saturation. It clearly distinguishes the lasing modes, which correspond to poles of the scattering matrix, from the injected fields, which do not; in this limit the locking of a lasing mode corresponds to the injected signal forcing the lasing pole off the real axis, reducing its amplitude to zero. I-SALT is shown to reduce to a version of the standard Adler theory of injection-locked lasing in a certain limit (the single pole approximation). We apply SALT to design a highly multimode cavity for use as a spatially incoherent light source for applications to imaging and microscopy. Laser illumination typically leads to coherent artifacts that degrade optical images; this can be alleviated by having a very large number of modes 500) which are spatially independent and average out such artifacts. We used SALT to model a D-shaped laser cavity with chaotic ray dynamics and showed that a certain shape greatly increases the number of lasing modes for the same cavity size and pump strength, due to a flat distribution of Q-values and reduced mode competition. An on-chip electrically-pumped semiconductor laser was realized using this cavity design and showed negligible coherent artifacts in imaging, as well as much better efficiency and power per mode than traditional incoherent light sources such as LEDs. The thesis also goes beyond semiclassical laser theory to treat quantum noise and the laser linewidth in a SALT-based approach. We demonstrate that SALT solutions can be used in conjunction with a temporal coupled mode theory (TCMT) to derive an analytic formula for the quantum limited laser linewidth in terms of integrals over SALT solutions. This linewidth formula is a substantial generalization of the well-known Schawlow-Townes result and includes all previously known corrections: the Petermann factor, Henry alpha factor, incomplete inversion factor and the "bad cavity factor". However, unlike previous theories these corrections are not simply multiplicative and are not separable in general. The predictions of TCMT linewidth theory are tested quantitatively by means of an FDTD algorithm that includes the Langevin noise as a source term.
Abstract The Schawlow–Townes limit established spontaneous emission as the fundamental quantum mechanism defining the minimum linewidth of an ideal laser oscillator. According to this description, random phase perturbations introduced by spontaneous photons become progressively less significant as the intracavity photon population increases, resulting in a continuous narrowing of the emission linewidth with increasing optical power. Although this relation remains a cornerstone of laser physics, it represents an ideal limit in which other sources of phase instability are absent. Practical laser systems frequently deviate from this behaviour: after an initial power-dependent narrowing regime, the linewidth often approaches a residual value that cannot be removed by further increasing the optical power. Such saturation suggests that linewidth should be treated not only as a photon-statistical quantity, but also as a property of the complete laser system, including the active medium. In this work, we develop a phenomenological framework in which laser linewidth is described as the combined result of spontaneous-emission noise, pump-induced fluctuations, and medium induced phase perturbations. The proposed approach preserves the Schawlow–Townes limit as the fundamental quantum contribution while introducing an active-medium-dependent term associated with the finite spectral response and microscopic fluctuations of the gain medium. The physical origin of this residual contribution is analysed using optical line-shape theory, considering homogeneous broadening, inhomogeneous broadening and the role of local environments in solid-state gain media. Er³+-doped systems are considered as representative rare earth active media, since their shielded 4f–4f transitions remain sufficiently narrow to support coherent emission while still retaining measurable signatures of crystal-field splitting, host disorder and spectral broadening. The model provides a physical interpretation for linewidth saturation and highlights that the ultimate optimisation of laser coherence requires not only improved cavity design and pump stabilisation but also control of the microscopic stability of the active medium. This viewpoint reframes the linewidth floor as a system-level property emerging from the interaction between quantum fluctuations, excitation dynamics and the gain medium.
Previous theories of laser radiation have described the electromagnetic field in terms of a discrete set of quasimodes (Fox and Li "modes") of the laser cavity. Each quasimode was assumed to have a finite quality factor Q. In steady state (when gain due to lasing atoms cancels the losses) and in the absence of noise sources, the semiclassical theory predicts a $\ensuremath{\delta}$-function line shape. In the present semiclassical analysis (fluctuations are ignored), this theory is generalized for a maser with a cavity having a semitransparent wall as one of the mirrors so that there are now many modes of the universe corresponding to each Fox-Li-type quasimode. It is demonstrated that the normal modes of the universe associated with a single Fox-Li "mode" may, under proper conditions, lock together and the $\ensuremath{\delta}$-function laser line shape may be regained. Specifically, we investigate the conditions under which the coupled multimode equations associated with laser oscillation can be reduced to an equation of the form found in the usual single-quasimode theory.
The problem of fundamental laser line broadening due to random spontaneous emission of radiation and amplification of thermal radiation noise is analyzed in terms of a classical fluctuating field phasor model. We derive a general expression for the intrinsic linewidth, given in terms of the spectral power of the radiation noise source, which can be classical or quantum mechanical in nature. In the case of a two-level atomic laser, we recover by the use of Einstein relations, the traditional linewidth formula of the Schalow-Townes form. In the case of the free-electron laser (FEL), using the explicit expression for the spontaneous emission, we present calculation of the laser linewidth by purely classical methods. The result agrees with the one obtained in the framework of a quantum-mechanical model. By using ``extended Einstein relations'' which are applicable to classical radiators, we show that a Schalow-Townes-type formula can also be obtained for the FEL. The theory predicts extremely narrow intrinsic linewidth ${(10}^{\mathrm{\ensuremath{-}}7}$ Hz) for cw FEL's with parameters similar to those of the FEL experiment of Elias et al.