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arXiv:1507.03697 · Physical Review A

Role of interspecies interactions in the preparation of a low-entropy gas of polar molecules in a lattice

Arghavan Safavi-Naini, Michael L. Wall, Ana María Rey

Published Dec 18, 2015• 8 citations
arXivHTMLPDF

Abstract

The preparation of a quantum degenerate gas of heteronuclear molecules has been an outstanding challenge. We use path-integral quantum Monte Carlo simulations to understand the role of interactions and finite temperature effects in the protocol currently employed to adiabatically prepare a low-entropy gas of polar molecules in a lattice starting from an ultracold Bose-Fermi mixture. We find that interspecies interactions affect the final temperature of the mixture after the adiabatic loading procedure and detrimentally limit the molecular peak filling. Our conclusions are in agreement with recent experimental measurements [Moses et al., Science 350, 659 (2015)] and therefore are of immediate relevance for the myriad experiments that aim to form molecules from dual-species atomic gases.

DOI
10.1103/physreva.92.063416

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The preparation of a quantum degenerate gas of heteronuclear molecules has been an outstanding challenge. We use path-integral quantum Monte Carlo simulations to understand the role of interactions and finite temperature effects in the protocol currently employed to adiabatically prepare a low-entropy gas of polar molecules in a lattice starting from an ultracold Bose-Fermi mixture. We find that interspecies interactions affect the final temperature of the mixture after the adiabatic loading procedure and detrimentally limit the molecular peak filling. Our conclusions are in agreement with recent experimental measurements [Moses et al., Science 350, 659 (2015)] and therefore are of immediate relevance for the myriad experiments that aim to form molecules from dual-species atomic gases.
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The entropy-temperature curves are calculated for noninteracting Bose and Fermi gases in a 3D optical lattice. These curves facilitate understanding of how adiabatic changes in the lattice depth affect the temperature, and we demonstrate regimes where the atomic sample can be significantly heated or cooled by the loading process. We assess the effects of interactions on a Bose gas in a deep optical lattice and show that interactions ultimately limit the extent of cooling that can occur during lattic loading.
Ultracold polar molecules, because of their long-range, spatially anisotropic interactions, are a new quantum system in which to study novel many-body phenomena. In our lab, we have produced the first quantum gas of 40K87Rb polar molecules. These molecules were found to undergo exothermic chemical reactions, and this led to interesting studies of chemistry near absolute zero. By creating the molecules at individual sites of a 3D optical lattice, we completely suppress these chemical reactions, and the polar molecule gas becomes stable and lives for tens of seconds. This thesis documents our efforts to explore coherent, many-body phenomena resulting from long-range dipolar interactions in the lattice. By encoding a spin-1=2 system in the rotational states of the molecules, we were able to realize spin-exchange interactions based on a spin Hamiltonian, which is one of the first steps in studying quantum magnetism with polar molecules. While this study was the first realization of such coherent dipolar interactions with polar molecules in a lattice, its full potential was limited by the low lattice filling fractions. Using our ability to exquisitely control the initial atomic gas mixture, we loaded a Mott insulator of Rb and a band insulator of K into the lattice. This quantum synthesis approach led to significantly higher molecular filling fractions and represents the first fully connected system of polar molecules in an optical lattice. This low-entropy quantum gas of polar molecules opens the door to interesting quantum simulations, which should be attainable in the next generation of the experiment.
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We present a quantitative finite temperature analysis of a recent experiment with Bose-Fermi mixtures in optical lattices, in which the dependence of the coherence of bosons on the interspecies interaction was analyzed. Our theory reproduces the characteristics of this dependence and suggests that intrinsic temperature effects play an important role in these systems. Namely, under the assumption that the ramping up of the optical lattice is an isentropic process, adiabatic temperature changes of the mixture occur that depend on the interaction between bosons and fermions. Matching the entropy of two regimes-no lattice on the one hand and deep lattices on the other-allows us to compute the temperature in the lattice and the visibility of the quasimomentum distribution of the bosonic atoms, which we compare to the experiment.