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arXiv:1506.09058 · Nano Letters

Dark High Density Dipolar Liquid of Excitons

Kobi J. Cohen, Yehiel Shilo, K. W. West, Loren N. Pfeiffer, Ronen Rapaport

Published May 16, 2016• 47 citations
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Abstract

The possible phases and the nanoscale particle correlations of two-dimensional interacting dipolar particles is a long-sought problem in many-body physics. Here we observe a spontaneous condensation of trapped two-dimensional dipolar excitons with internal spin degrees of freedom from an interacting gas into a high density, closely packed liquid state made mostly of dark dipoles. Another phase transition, into a bright, highly repulsive plasma, is observed at even higher excitation powers. The dark liquid state is formed below a critical temperature Tc ≈ 4.8 K, and it is manifested by a clear spontaneous spatial condensation to a smaller and denser cloud, suggesting an attractive part to the interaction which goes beyond the purely repulsive dipole-dipole forces. Contributions from quantum mechanical fluctuations are expected to be significant in this strongly correlated, long living dark liquid. This is a new example of a two-dimensional atomic-like interacting dipolar liquid, but where the coupling of light to its internal spin degrees of freedom plays a crucial role in the dynamical formation and the nature of resulting condensed dark ground state.

DOI
10.1021/acs.nanolett.6b01061

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The possible phases and the nanoscale particle correlations of two-dimensional interacting dipolar particles is a long-sought problem in many-body physics. Here we observe a spontaneous condensation of trapped two-dimensional dipolar excitons with internal spin degrees of freedom from an interacting gas into a high density, closely packed liquid state made mostly of dark dipoles. Another phase transition, into a bright, highly repulsive plasma, is observed at even higher excitation powers. The dark liquid state is formed below a critical temperature Tc ≈ 4.8 K, and it is manifested by a clear spontaneous spatial condensation to a smaller and denser cloud, suggesting an attractive part to the interaction which goes beyond the purely repulsive dipole-dipole forces. Contributions from quantum mechanical fluctuations are expected to be significant in this strongly correlated, long living dark liquid. This is a new example of a two-dimensional atomic-like interacting dipolar liquid, but where the coupling of light to its internal spin degrees of freedom plays a crucial role in the dynamical formation and the nature of resulting condensed dark ground state.
The formation of a dense Bose-Einstein condensate in dark spin states of two-dimensional dipolar excitons is shown to be driven by a dynamical transition to the long-lived dark states. The condensate is stabilized by strong dipole-dipole interactions up to densities high enough for a dark quantum liquid to form. The persistence of dark condensation was observed in recent experiments. A model describing the non-equilibrium dynamics of externally driven coupled dark and bright condensates reproduces the step-like dependence of the exciton density on the pump power or on temperature. This unique condensate dynamics demonstrates the possibility of observing new unexpected collective phenomena in coupled condensed Bose systems, where the particle number is not conserved.
Strongly interacting bosons display a rich variety of quantum phases, the study of which has so far been focused in the dilute regime, at a fixed number of particles. Here we demonstrate the formation of a dense Bose-Einstein condensate in a long-lived dark spin state of 2D dipolar excitons. A dark condensate of weakly interacting excitons is very fragile, being unstable against a coherent coupling of dark and bright spin states. Remarkably, we find that strong dipole-dipole interactions stabilize the dark condensate. As a result, the dark phase persists up to densities high enough for a dark quantum liquid to form. The striking experimental observation of a step-like dependence of the exciton density on the pump power is reproduced quantitatively by a model describing the nonequilibrium dynamics of driven coupled dark and bright condensates. This unique behavior marks a dynamical condensation to dark states with lifetimes as long as a millisecond, followed by a brightening transition at high densities.
A dramatic stabilization of a Bose-Einstein condensate in dark spin states of two-dimensional dipolar excitons is predicted, driven by strong particle correlations which are induced by dipole-dipole interactions. This stability persists up to densities high enough to support the formation of a dark quantum liquid, where the transition to a mixed phase of dark and bright states, becomes robust against variations of system parameters and local conditions. This stabilized behavior is in accordance with puzzling recent observations of a stable dark quantum liquid. In a remarkable similarity to these observations, a model describing the dynamics of such coupled dark and bright condensates with external pumping and variable particle occupation numbers predicts a dynamical step-like dependence of the exciton density on the external pump power or on temperature. The two turning points mark the onsets of the dark and the mixed dark-bright condensates. This unique condensate dynamics demonstrates the possibility of observing new unexpected collective phenomena in coupled condensed Bose systems, where the particle number is not a conserved quantity.
We investigate the phases of a Bose-Einstein condensate of dipolar atoms restricted to move in a two-dimensional plane. The dipole moments are all aligned in a direction tilted with respect to the plane normal. As a result of the attractive and repulsive components of the dipole-dipole interaction, the dipolar gas has a self-bound phase, which is stabilized by quantum fluctuations. Tilting the dipoles tunes the anisotropy of the dipole-dipole interaction, which can trigger a spatial density modulation. In this work we study these two aspects and investigate the conditions for the formation of a self-bound and striped phase, which has been realized in experiments with dipolar droplets. We use a variational method based on the hypernetted-chain Euler-Lagrange optimization of a Jastrow-Feenberg ansatz for the many-body wave function to study the ground-state properties. This method takes into account quantum fluctuations in a nonperturbative way and thus can be used also for strongly correlated systems.
Two-dimensional (2D) dipolar atomic gases present unique opportunities for exploring novel quantum phases due to their anisotropic and long-range interactions. However, the behavior of strongly dipolar Bose gases in 2D remains unclear, especially when dipoles are tilted. Here, we demonstrate the creation and characterization of strongly dipolar 2D condensates in a quasi-2D harmonic trap with tunable dipole orientation. By investigating scale invariance properties through breathing collective mode measurements, we observe significant breaking of scale invariance when dipoles are tilted in-plane indicating the dominance of the nonlocal dipole-dipole interactions (DDIs) in this regime. Interestingly, the breaking of the scale invariant dynamics is accompanied by an increase in quantum fluctuations, as shown by comparison with mean-field and beyond mean-field theoretical studies. Our experiments also reveal that at critical tilt angles around 70°, stripe-type density modulations emerge, suggesting the presence of a roton spectrum in 2D, while the system still shows hydrodynamic nature with the phase-locking breathing behavior. This observation elucidates the many-body effect induced by DDIs in 2D, thus marking a crucial step toward realizing 2D supersolids and other exotic quantum phases.
We consider quantum phase transitions in a system of bright dipolar excitons which can form bound pairs (dipolar biexcitons). The biexciton energy is tuned from negative to positive values through the scattering threshold. At sufficiently large density an exciton superfluid transforms into a superfluid of biexcitons. With the average relative momenta of excitons in the pairs being beyond the light cone, the transition is accompanied by a reduction of the photoluminescence intensity. Effective magnetic fields due to the long-range exchange splitting of exciton states shift the position of the gap in the elementary excitation spectrum to a circle of degenerate minima in the $\mathbit{k}$ space. Closing the gap results in the formation of exciton stripes polarized linearly along the direction of their translational symmetry. In the biexciton energy vs density phase diagram the novel phase intervenes between the dark biexciton and radiative exciton superfluids. We conclude that formation of a BCS-like biexciton condensate induces correlated alignment of the effective magnetic fields and excitonic spins. We outline important differences in the predicted mechanism from the phenomenon of spin-orbit-coupled Bose-Einstein condensation.