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arXiv:1506.02775 · Journal of the Physical Society of Japan

Ground State Phase Diagram of Twisted Three-Leg Spin Tube in Magnetic Field

Kouki Yonaga, Naokazu Shibata

Published Aug 10, 2015• 15 citations
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Abstract

We study the ground state phase diagram of the twisted three-leg spin tube in magnetic fields by the density matrix renormalization group (DMRG) method. The twisted spin tube is composed of triangular unit cells and possesses strong quantum fluctuations under geometrical frustration. We apply the sine square deformation method to remove the strong boundary effects and obtain smooth magnetization curves without steps of finite systems. With the analysis of the magnetization curves and correlation functions we determine the ground state phase diagram consisting of (a) a Tomonaga-Luttinger (TL) liquid characterized by spin-$\frac{3}{2}$ Heisenberg model, (b) 3-sublattice state named UUD with 1/3 magnetization and (c) TL-liquid of massless chirality with 1/3 magnetization plateau, (d) TL-liquid of massless spin mode with or without chirality quasi long-range order.

DOI
10.7566/jpsj.84.094706

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We study the ground state phase diagram of the twisted three-leg spin tube in magnetic fields by the density matrix renormalization group (DMRG) method. The twisted spin tube is composed of triangular unit cells and possesses strong quantum fluctuations under geometrical frustration. We apply the sine square deformation method to remove the strong boundary effects and obtain smooth magnetization curves without steps of finite systems. With the analysis of the magnetization curves and correlation functions we determine the ground state phase diagram consisting of (a) a Tomonaga-Luttinger (TL) liquid characterized by spin-32\frac{3}{2}23​ Heisenberg model, (b) 3-sublattice state named UUD with 1/3 magnetization and (c) TL-liquid of massless chirality with 1/3 magnetization plateau, (d) TL-liquid of massless spin mode with or without chirality quasi long-range order.
We use a combination of numerical density matrix renormalization group calculations and several analytical approaches to comprehensively study a simplified model for a spatially anisotropic spin-12\frac{1}{2}21​ triangular lattice Heisenberg antiferromagnet: the three-leg triangular spin tube (TST). The model is described by three Heisenberg chains, with exchange constant JJJ, coupled antiferromagnetically with exchange constant ${J}^{\ensuremath{'}}$ along the diagonals of the ladder system, with periodic boundary conditions in the shorter direction. Here, we determine the full phase diagram of this model as a function of both spatial anisotropy (between the isotropic and decoupled chain limits) and magnetic field. We find a rich phase diagram, which is remarkably dominated by quantum states: the phase corresponding to the classical ground state appears only in an exceedingly small region. Among the dominant phases generated by quantum effects are commensurate and incommensurate coplanar quasiordered states, which appear in the vicinity of the isotropic region for most fields, and in the high-field region for most anisotropies. The coplanar states, while not classical ground states, can at least be understood semiclassically. Even more strikingly, the largest region of phase space is occupied by a spin density wave phase, which has incommensurate collinear correlations along the field. This phase has no semiclassical analog, and may be ascribed to enhanced one-dimensional fluctuations due to frustration. Cutting across the phase diagram is a magnetization plateau, with a gap to all excitations and ``up-up-down'' spin order, with a quantized magnetization equal to 13\frac{1}{3}31​ of the saturation value. In the TST, this plateau extends almost but not quite to the decoupled chains limit. Most of the above features are expected to carry over to the two-dimensional system, which we also discuss. At low field, a dimerized phase appears, which is particular to the one-dimensional nature of the TST, and which can be understood from quantum Berry phase arguments.
We study the ground-state phase diagram of a frustrated spin-1/2 four-leg tube. Using a variety of complementary techniques, namely, density matrix renormalization group, exact diagonalization, Schwinger boson mean-field theory, quantum Monte Carlo, and series expansion, we explore the parameter space of this model in the regime of all-antiferromagnetic exchange. In contrast to unfrustrated four-leg tubes, we uncover a rich phase diagram. Apart from the Luttinger liquid fixed point in the limit of decoupled legs, this comprises several gapped ground states, namely, a plaquette, an incommensurate, and an antiferromagnetic quasispin-2 chain phase. The transitions between these phases are analyzed in terms of total energy and static structure factor calculations and are found to be of (weak) first order. Despite the absence of long-range order in the quantum case, remarkable similarities to the classical phase diagram are uncovered, with the exception of the icommensurate regime, which is strongly renormalized by quantum fluctuations. In the limit of large leg exchange, the tube exhibits a deconfinement crossover from gapped magnon-like excitations to spinons.
Thermodynamic properties of the twisted three-leg spin tube under magnetic field are studied by the finite-TTT density-matrix renormalization group method. The specific heat, spin, and chiral susceptibilities of the infinite system are calculated for both the original and its low-energy effective models. The obtained results show that the presence of the chirality is observed as a clear peak in the specific heat at low temperature and the contribution of the chirality dominates the low-temperature part of the specific heat as the exchange coupling along the spin tube decreases. The peak structures in the specific heat, spin, and chiral susceptibilities are strongly modified near the quantum phase transition where the critical behaviors of the spin and chirality correlations change. These results confirm that the chirality plays a major role in characteristic low-energy behaviors of the frustrated spin systems.
Recent developments of theoretical studies on spin nanotubes are reviewed, especially focusing on the S = 1/2 three-leg spin tube. In contrast to the three-leg spin ladder, the tube has a spin gap in the case of the regular-triangle unit cell when the rung interaction is sufficiently large. The effective theory based on the Hubbard Hamiltonian indicates a quantum phase transition to a gapless spin liquid due to the lattice distortion to an isosceles triangle. This is also supported by the numerical diagonalization and the density matrix renormalization group analyses. Furthermore, combining analytical and numerical approaches, we reveal several novel magnetic-field-induced phenomena: Néel, dimer, chiral and/or inhomogeneous orders, a new mechanism for the magnetization plateau formation, and others. The recently synthesized spin tube materials are also briefly introduced.
The frustrated three-leg antiferromagnetic spin-12\frac{1}{2}21​ tube with a weak interchain coupling in a magnetic field is investigated by means of Abelian bosonization techniques. It is clearly shown that a vector chiral long-range order and a one-component Tomonaga-Luttinger liquid coexist in a wide magnetic-field region from a state with a small magnetization to a nearly saturated one. The chiral order is predicted to still survive in the intermediate plateau state. We further predict that (even) when the strength of one bond in the three rung couplings is decreased (increased), an Ising-type quantum phase transition takes place and the chirality vanishes (no singular phenomena occur and the chiral order is maintained). Even without magnetic fields, the chiral order would also be present if the spin tube possesses easy-plane anisotropy.
Using the density matrix renormalization group method we have studied the ground-state phase diagram of a spin-1/2 frustrated three-leg antiferromagnetic Heisenberg ladder, and identified two phases corresponding to the spin-3/2 chain and the standard spin ladder. Varying the diagonal coupling ${J}_{\ifmmode\times\else\texttimes\fi{}}$ leads to a quantum phase transition from one ground state to the other, but does not alter the gapless nature of the excitation spectra. On the phase boundary, the degenerate ground states form a chiral spin liquid with a central charge c=2.c=2.c=2. The critical value of ${J}_{\ifmmode\times\else\texttimes\fi{}}$ is insensitive to the number of legs in the ladder, suggesting that a quantum phase transition may occur at ${J}_{\ifmmode\times\else\texttimes\fi{}}=0.6$ for the isotropic spin-1/2 antiferromagnetic Heisenberg model on the square lattice.