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arXiv:1506.00364 · Physical Review A

Second-order response theory of radio-frequency spectroscopy for cold atoms

Christophe Berthod, Michael Köhl, Thierry Giamarchi

Published Jul 22, 2015• 2 citations
arXivHTMLPDF

Abstract

We present a theoretical description of the radio-frequency (rf) spectroscopy of fermionic atomic gases, based on the second-order response theory at finite temperature. This approach takes into account the energy resolution due to the envelope of the rf pulse. For a noninteracting final state, the momentum- and energy-resolved rf intensity depends on the fermion spectral function and pulse envelope. The contributions due to interactions in the final state can be classified by means of diagrams. Using this formalism, as well as the local density approximation in two and three dimensions, we study the interplay of inhomogeneities and Hartree energy in forming the line shape of the rf signal. We show that the effects of inhomogeneities can be minimized by taking advantage of interactions in the final state, and we discuss the most relevant final-state effects at low temperature and density, in particular the effect of a finite lifetime.

DOI
10.1103/physreva.92.013626

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We present a theoretical description of the radio-frequency (rf) spectroscopy of fermionic atomic gases, based on the second-order response theory at finite temperature. This approach takes into account the energy resolution due to the envelope of the rf pulse. For a noninteracting final state, the momentum- and energy-resolved rf intensity depends on the fermion spectral function and pulse envelope. The contributions due to interactions in the final state can be classified by means of diagrams. Using this formalism, as well as the local density approximation in two and three dimensions, we study the interplay of inhomogeneities and Hartree energy in forming the line shape of the rf signal. We show that the effects of inhomogeneities can be minimized by taking advantage of interactions in the final state, and we discuss the most relevant final-state effects at low temperature and density, in particular the effect of a finite lifetime.
We present a theory of radio-frequency spectroscopy of impurities interacting with a quantum gas at finite temperature. By working in the canonical ensemble of a single impurity, we show that the impurity spectral response is directly connected to the finite-temperature equation of state (free energy) of the impurity. We consider two different response protocols: injection, where the impurity is introduced into the medium from an initially noninteracting state, and ejection, where the impurity is ejected from an initially interacting state with the medium. We show that there is a simple mapping between injection and ejection spectra, which is connected to the detailed balance condition in thermal equilibrium. To illustrate the power of our approach, we specialize to the case of the Fermi polaron, corresponding to an impurity atom that is immersed in a noninteracting Fermi gas. For a mobile impurity with a mass equal to the fermion mass, we employ a finite-temperature variational approach to obtain the impurity spectral response. We find a striking nonmonotonic dependence on temperature in the impurity free energy, the contact, and the radio-frequency spectra. For the case of an infinitely heavy Fermi polaron, we derive exact results for the finite-temperature free energy, thus generalizing Fumi's theorem to arbitrary temperature. We also determine the exact dynamics of the contact after a quench of the impurity-fermion interactions. Finally, we show that the injection and ejection spectra obtained from the variational approach compare well with the exact spectra, thus demonstrating the accuracy of our approximation method.
In this paper we present an overview of radio frequency (RF) spectroscopy in the atomic Fermi superfluids. An ultimate goal is to suggest new directions in the cold gas research agenda from the condensed matter perspective.Our focus is on the experimental and theoretical literature of cold gases and photoemission spectroscopy of the cuprates particularly as it pertains to areas of overlap. This paper contains a systematic overview of the theory of RF spectroscopy, both momentum integrated and momentum resolved. We discuss the effects of traps, population imbalance, final state interactions over the entire range of temperatures and compare theory and experiment. We show that this broad range of phenomena can be accomodated within the BCS-Leggett description of BCS-BEC crossover and that this scheme also captures some of the central observations in photoemission experiments in the cuprates. In this last context, we note that the key themes which have emerged in cuprate photoemission studies involve characterization of the fermionic self energy, of the pseudogap and of the effects of superconducting coherence (in passing from above to below the superfluid transition temperature, TcT_cTc​).These issues have a counterpart in the cold Fermi gases and it would be most useful in future to use these atomic systems to address these and the more sweeping question of how to describe that anomalous superfluid phase which forms in the presence of a normal state excitation gap.
We theoretically investigate the momentum-resolved radio-frequency spectroscopy of a harmonically trapped atomic Fermi gas near a Feshbach resonance in the presence of equal Rashba and Dresselhaus spin-orbit coupling. The system is qualitatively modeled as an ideal gas mixture of atoms and molecules, in which the properties of molecules, such as the wave function, binding energy, and effective mass, are determined from the two-particle solution of two interacting atoms. We calculate separately the radio-frequency response from atoms and molecules at finite temperatures by using the standard Fermi golden rule and take into account the effect of harmonic traps within local density approximation. The total radio-frequency spectroscopy is discussed as functions of temperature and spin-orbit coupling strength. Our results give a qualitative picture of radio-frequency spectroscopy of a resonantly interacting spin-orbit-coupled Fermi gas and can be directly tested in atomic Fermi gases of 40{}^{40}40K atoms at Shanxi University and 6{}^{6}6Li atoms at the Massachusetts Institute of Technology.
We investigate theoretically momentum-resolved radio-frequency (rf) spectroscopy of a noninteracting atomic Fermi gas in a spin-orbit coupled lattice. This lattice configuration has been recently created at MIT [Cheuk et al., Phys. Rev. Lett. 109, 095302 (2012)] for 6{}^{6}6Li atoms, by coupling the two hyperfine spin states with a pair of Raman laser beams and additional rf coupling. Here, we show that momentum-resolved rf spectroscopy can measure single-particle energies and eigenstates and therefore resolve the band structure of the spin-orbit coupled lattice. In our calculations, we take into account the effects of temperatures and harmonic traps. Our predictions are to be confronted with future experiments on spin-orbit coupled Fermi gases of 40{}^{40}40K atoms in a lattice potential.
The radio-frequency spectrum of the fermions in the unitary limit at finite temperatures is characterized by the sum-rule relations. We consider a simple picture where the atoms are removed by radio-frequency excitations from the strongly interacting states into a state of negligible interaction. We calculate the moments of the response function in the range of temperature 0.08ϵF<T<0.8ϵF0.08{ϵ}_{F}<T<0.8{ϵ}_{F}0.08ϵF​<T<0.8ϵF​ using auxiliary field Monte Carlo technique in which continuum auxiliary fields with a density-dependent shift are used. We estimate the effects of superfluid pairing from the clock shift. We find a qualitative agreement with the pairing gap--pseudogap transition behavior. We also find within the quasiparticle picture that in order for the gap to come into quantitative agreement with the previously known value at T=0T=0T=0, the effective mass has to be ${m}^{\ensuremath{\ast}}\ensuremath{\sim}1.43m$. Finally, we discuss implications for the adiabatic sweep of the resonant magnetic field.
We present spatially resolved radio-frequency spectroscopy of a trapped Fermi gas with resonant interactions and observe a spectral gap at low temperatures. The spatial distribution of the spectral response of the trapped gas is obtained using in situ phase-contrast imaging and 3D image reconstruction. At the lowest temperature, the homogeneous rf spectrum shows an asymmetric excitation line shape with a peak at 0.48(4)epsilonF with respect to the free atomic line, where epsilonF is the local Fermi energy.