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arXiv:1505.04900 · Physical Review A

Eigenvalue decomposition method for photon statistics of frequency-filtered fields and its application to quantum dot emitters

Kenji Kamide, Satoshi Iwamoto, Yasuhiko Arakawa

Published Sep 18, 2015• 13 citations
arXivHTMLPDF

Abstract

A simple calculation method for photon statistics of frequency-filtered fields is proposed. This method, based on eigenvalue decompositions of superoperators, allows us to study effects on the photon statistics of spectral filtering by various types of filters, such as Gaussian and rectangular filters as well as Lorentzian filters, which is not possible by conventional approaches. As an example, this method is applied to a simulation of quantum dot single-photon emitters, where we found that the efficient choice of the filter types to have pure single photons depends on the excitation conditions, i.e., incoherent or coherent (and resonant) excitations.

DOI
10.1103/physreva.92.033833

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A simple calculation method for photon statistics of frequency-filtered fields is proposed. This method, based on eigenvalue decompositions of superoperators, allows us to study effects on the photon statistics of spectral filtering by various types of filters, such as Gaussian and rectangular filters as well as Lorentzian filters, which is not possible by conventional approaches. As an example, this method is applied to a simulation of quantum dot single-photon emitters, where we found that the efficient choice of the filter types to have pure single photons depends on the excitation conditions, i.e., incoherent or coherent (and resonant) excitations.
Frequency-filtered photon correlations have been proven to be extremely useful in grasping how the detection process alters photon statistics. Harnessing the spectral correlations also permits refinement of the emission and unraveling of previously hidden strong correlations in a plethora of quantum-optical systems under continuous-wave excitation. In this work, we investigate such correlations for time-dependent excitation and develop a methodology to compute efficiently time-integrated correlations, which are at the heart of the photon-counting theory, and subsequently apply it to analyze the photon emission of pulsed systems. By combining this formalism with the —which facilitates frequency-resolved correlations—we demonstrate how spectral filtering enhances single-photon purity and suppresses multiphoton noise in time-bin-encoded quantum states. Specifically, filtering the central spectral peak of a dynamically driven two-level system boosts temporal coherence and improves the fidelity of time-bin entanglement preparation, even under conditions favoring multiphoton emission. These results establish spectral filtering as a critical tool for tailoring photon statistics in pulsed quantum light sources.
We develop a formalism based on a time-dependent wave-function ansatz to study correlations of photons emitted from a collection of two-level quantum emitters. We show how to simulate the system dynamics and evaluate the intensity of the scattered photons and the second-order correlation function g(2)g^{(2)}g(2) in terms of the amplitudes of the different components of the wave function. Our approach is efficient for considering systems that contain up to two excitations. To demonstrate this we first consider the example of spectral filtering of photons emitted from a single quantum emitter. We show how our formalism can be used to study spectral filtering of the two-photon component of the emitted light from a single quantum emitter for various kinds of filters. Furthermore, as a general application of our formalism, we show how it can be used to study photon-photon correlations in an optically dense ensemble of two-level quantum emitters. In particular we lay out the details of simulating correlated photon transport in such ensembles reported recently by S. Mahmoodian {\it et.al.} [Phys. Rev. Lett. {\bf 121}, 143601 (2018)]. Compared to other existing techniques, the advantage of our formalism is that it is applicable to any generic spectral filter and quantum many-body systems involving a large number of quantum emitters while requiring only a modest computational resource.
One of the most common approaches for coupling optical single-photon sources and photonic integrated circuits is to use a cavity. The cavity acts as a spectral filter that distorts the light spectrum and changes its statistical properties. But in the general case one should take into account not only spectral filtering of light but also the spectral filter influence on the single-photon source dynamics. We build an effective analytical model for description of the cavity influence on the photon statistics of light emitted by the single-photon source as spectral filtering only. We show that this model correctly describes the photon statistics even in a strong-coupling regime between the single-photon source and the spectral filter. Our results can be useful for analytical modeling of photon statistics of quantum emitters strongly coupled to various electromagnetic interfaces.
Spectral filtering of resonance fluorescence is widely employed to improve single photon purity and indistinguishability by removing unwanted backgrounds. For filter bandwidths approaching the emitter linewidth, complex behavior is predicted due to preferential transmission of components with differing photon statistics. We probe this regime using a Purcell-enhanced quantum dot in both weak and strong excitation limits, finding excellent agreement with an extended sensor theory model. By changing only the filter width, the photon statistics can be transformed between antibunched, bunched, or Poissonian. Our results verify that strong antibunching and a subnatural linewidth cannot simultaneously be observed, providing new insight into the nature of coherent scattering.
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Abstract. We apply our recently developed theory of frequency-filtered and time-resolved N-photon correlations [1] to study the two-photon spectra of a variety of systems of increasing complexity: single mode emitters with two limiting statistics (one harmonic oscillator or a two-level system) and the various combinations that arise from their coupling. We consider both the linear and nonlinear regimes under incoherent excitation. We find that even the simplest systems display a rich dynamics of emission, not accessible by simple single photon spectroscopy. In the strong coupling regime, novel two-photon emission processes involving virtual states are revealed. Furthermore, two general results are unraveled by two-photon correlations with narrow linewidth detectors: i) filtering induced bunching and ii) breakdown of the semi-classical theory. We show how to overcome this shortcoming in a fully-quantized picture. PACS numbers: 42.50.Ar,42.50.Lc,05.10.Gg,42.25.Kb,42.79.Pw ar X iv