Clean carbon nanotubes coupled to superconducting impedance-matching circuits
V. Ranjan, Gabriel Puebla‐Hellmann, Minkyung Jung, T. Hasler, Andreas Nunnenkamp, Matthias Muoth, Christofer Hierold, Andreas J. Wallraff, Christian Schönenberger
Coupling carbon nanotube devices to microwave circuits offers a significant increase in bandwidth (BW) and signal-to-noise ratio. These facilitate fast non-invasive readouts important for quantum information processing, shot noise and correlation measurements. However, creation of a device that unites a low-disorder nanotube with a low-loss microwave resonator has so far remained a challenge, due to fabrication incompatibility of one with the other. Employing a mechanical transfer method, we successfully couple a nanotube to a gigahertz superconducting matching circuit and thereby retain pristine transport characteristics such as the control over formation of, and coupling strengths between, the quantum dots. Resonance response to changes in conductance and susceptance further enables quantitative parameter extraction. The achieved near matching is a step forward promising high-BW noise correlation measurements on high impedance devices such as quantum dot circuits. Radio-frequency circuits offer fast low-noise detection of signals in carbon nanotubes, but incompatibilities in fabrication degrade the performance of the hybrid device. Here, the authors use a deterministic mechanical transfer to couple pristine nanotubes to a gigahertz superconducting matching circuit.
Coupling carbon nanotube devices to microwave circuits offers a significant increase in bandwidth (BW) and signal-to-noise ratio. These facilitate fast non-invasive readouts important for quantum information processing, shot noise and correlation measurements. However, creation of a device that unites a low-disorder nanotube with a low-loss microwave resonator has so far remained a challenge, due to fabrication incompatibility of one with the other. Employing a mechanical transfer method, we successfully couple a nanotube to a gigahertz superconducting matching circuit and thereby retain pristine transport characteristics such as the control over formation of, and coupling strengths between, the quantum dots. Resonance response to changes in conductance and susceptance further enables quantitative parameter extraction. The achieved near matching is a step forward promising high-BW noise correlation measurements on high impedance devices such as quantum dot circuits. Radio-frequency circuits offer fast low-noise detection of signals in carbon nanotubes, but incompatibilities in fabrication degrade the performance of the hybrid device. Here, the authors use a deterministic mechanical transfer to couple pristine nanotubes to a gigahertz superconducting matching circuit.
Modern experiments using high-speed, high-impedance devices such as quantum dots can suffer from strong suppression of signal power, if components are not carefully impedance-matched. To overcome this problem, the authors show that a resonant impedance-matching circuit based on superconducting transmission lines can improve the signal to noise ratio by nearly three orders of magnitude. This technology is particularly important to noise studies of electron transport in quantum systems, which can provide information that is unattainable by other means.
Fast measurement of small currents and even smaller fluctuations in devices with large impedance is not trivial. Standard low frequency lock-in measurements suffer from stray capacitance of the order of nF reducing the bandwidth to merely kHz and a time resolution of ms. One approach of increasing the bandwidth is to connect the high-impedance device next to a low input impedance amplifier, though, the signal is decreased by the ratio of the impedances of the device and the amplifier, easily a factor of a thousand. Therefore, long averaging times are required to detect the small signal. Moreover, 1/f noise still affects the measurements. The issues of small bandwidth, impedance mismatch and 1/f noise can be simultaneously addressed using resonant LC circuits. The success of this impedance transformer lies in replacing the slow operation of applying voltages and measuring currents by applying fast radio frequency signals and measuring the reflectance. LC circuits remain appealing because of a rather simple assembly. Nonetheless, the challenge to reproducibly achieve the resonance frequencies in gigahertz (GHz) range while matching to high impedance still remains due to the large parallel stray capacitance of the measurement setup. Resonance frequency in GHz range is desirable for two reasons. Firstly, measurements are faster and 1/f noise smaller. Yet more importantly, one can profit from the wide range of measurement techniques developed in the context of circuit quantum electrodynamics, such as FPGA based hardware and quantum limited Josephson parametric amplifiers. \n \nIn this thesis, a matching circuit namely stub tuner based on coplanar transmission lines is designed, fabricated and integrated with mesoscopic devices. Owing to the simple design, we could predict the frequency response of a stub tuner in terms of the standard circuit model (Chapter 3). We initiated certain necessary fabrication adaptations to achieve integration of niobium circuits with devices. In particular, a reliable stamping of carbon nanotubes from the growth substrate to the target substrate was accomplished, improving both the device quality and yield (Chapter 4). RF reflectometry is employed to perform admittance measurements on CNT quantum dots. We could reliably deduce all circuit and device properties using the resonance response. The measurement bandwidth is shown to be in MHz range which is three orders of magnitude larger than that for DC measurements. In particular, using the phase response of the circuit, double-dot qubit energy and dephasing rate are studied (Chapter 5). We could even get rid of conventional contacts that could degrade the device properties, and still extract quantum capacitance and dissipation in graphene p-n junctions. The residual doping is shown to affect not only the mean free path but also the Fermi velocity. We further see that at small doping, electron-electron interactions could modify the Fermi velocity and that the dispersion relation could deviate from linearity (Chapter 6). \n \nIn the second half of the scientific results, real strength of stub tuner is tested in transmission measurements. The large bandwidth and signal to noise ratio is utilized to measure extremely clean noise power densities at high speed and draw comparisons with the corresponding average current. Clear changes in the shot noise spectrum are seen when a transport channel is added or removed from the bias window of the quantum dot. We especially observe noise enhancement outside the Coulomb diamonds due to blocking states (Chapter 7). Finally, we investigate noise properties of quantum dots when leads are superconducting. Distinct charge transfers due to multiple Andreev reflections are visible in the shot noise. The main finding, however, was the thermal noise at zero bias. We observed its periodic suppression and emergence across the quantum dot resonance. In another device, shot noise due to the Kondo effect is found to be enhanced in the superconducting state when the Kondo temperature exceeds the value of the superconducting gap (Chapter 8). Simple design and reliable calibration of the GHz matching circuit in both reflectance and transmission pave a way for fast and non-invasive measurements of mesoscopic conductors. \n \n \n \n \n
Circuit quantum electrodynamics has received an increasing amount of attention over the last decade in light of its potential use in quantum information processing. The underlying principle of this architecture is the coherent coupling between microwave photons stored in superconducting resonators and superconducting qubits made from non-linear, non-dissipative electrical circuits. This architecture can be extended to other solid-state systems with transition frequencies in the microwave regime, such as nuclear and electron spins or Andreev bound states. These hybrid devices would allow the coherent exchange of information between such systems and superconducting qubits mediated by a microwave resonator. This could lead to advances in quantum information processing and new insights in the physics governing these interacting systems. In this dissertation experimental work with different types of hybrid quantum circuits is presented. A first experiment investigates the coherent coupling of microwave photons with a spin ensemble in a correlated and uncorrelated state. The coupling strength and magnetic resonance is studied as a function of temperature and magnetic field direction. A pronounced temperature dependent anisotropy of the magnetic resonance is observed, which can be attributed to the onset of antiferromagnetic correlations in the spin ensemble when cooled below T=4 K. A simple one-dimensional model gives a good description of this anisotropy. A next experiment studies the transport characteristics of carbon nanotubes electrically accessed with normal and superconducting contacts. These devices were characterised using both DC and RF reflectometry techniques. The carbon nanotube devices with superconducting contacts exhibit transport characteristics of Josephson junctions with critical currents of up to Ic~18 nA, as well as multiple Andreev reflections. These semiconductor-superconductor hybrid Josephson junctions are then used to realise a carbon-nanotube-based superconducting qubit with voltage tunable transition frequency using a local electrostatic gate. Strong coupling (g~100 MHz) to a coplanar waveguide resonator is demonstrated via a resonator frequency shift dependent on applied gate voltage. Qubit parameters are extracted from spectroscopy and correspond well to the DC measurements of the carbon nanotube Josephson junctions. Qubit relaxation and coherence times in the range 10-100 ns are observed. The hybrid devices investigated in this work present potential building blocks for more extensive hybrid architectures for quantum information processing.
This thesis presents an effort towards integration of superconductor-contacted carbon nanotubes into microwave circuits, as a new tool for building quantum circuits. Carbon nanotubes show a wealth of quantum phenomena demonstrated in transport experiments by different groups in the last two decades. With the development of circuit QED, one can study these phenomena using on-chip microwave circuits. Moreover, in superconductor-contacted nanotubes, Andreev reflection of the particles at the interfaces leads to the formation of Andreev bound states. A pair of such states can potentially serve as a new type of a qubit. Here, fabrication and measurement techniques of superconductor contacted carbon nanotubes and superconductor/normal metal bilayer microwave circuits is developed, and their behaviour is studied. In superconductor-contacted nanotubes the full range of contact transparencies is investigated, showing different transport phenomena such as Coulomb blockade, Kondo effect and Fabry-Pérot interference. In addition, the interplay of these effects with multiple Andreev reflection phenomena and the superconducting proximityinduced non-dissipative current transport through the nanotube is studied. The proximity effect is studied using microwave resonators made of superconductor/ normal metal bilayers. Characteristic parameters of the bilayers, such as the critical temperature and the magnetic penetration depth are reliably extracted from the measurements. Finally, the two experiments are brought together in the first step towards using superconductor-contacted nanotubes in quantum microwave circuits. The successful realization of such circuit is achieved, where the Coulomb blockade in a nanotube quantum dot is probed with a microwave field.
This thesis deals with the implementation and demonstration of an optomechanical system that is composed of a superconducting microwave resonator and a suspended carbon nanotube (CNT). This is of particular interest, as CNTS - being macromolecules - have outstanding electronic and mechanical properties. Single electron effects combined with large mechanical resonance frequencies, quality factors, and zero-point motion amplitudes make possible promising applications in the field of quantum information processing or fundamental research, e.g. the synthesis of arbitrary quantum states. Besides the assembly of a high frequency measurement setup for cryogenic temperatures in the millikelvin range, introductory chapters discuss electronic and mechanical characteristics of carbon nanotubes. Here, two different fabrication techniques are described, the overgrowth and the fork transfer process. The physics of superconducting microwave resonators in coplanar waveguide geometry is introduced. Their high frequency behaviour at low temperatures is described by a transition from Mattis-Bardeen to two-level system theory. This serves as a means to investigate the high frequency material properties of a molybdenum/rhenium alloy, which is particularly suitable for the overgrowth process. Device design adjustments and considerations are described that were necessary for the integration of CNTs into hybrid geometries using the fork transfer process. Through this, the (previously demonstrated) electronic coupling of a carbon nanotube to a microwave resonator could be successfully experimentally demonstrated. There, the transmission of the resonator is sensitive to single electron tunneling processes in the CNT. The central point of this thesis is the introduction to the field of dispersive optomechanics. Here, the interaction of a vibrating carbon nanotube and a microwave field is investigated. A mechanism based on the quantum capacitance enhances this otherwise negligible coupling by orders of magnitude. Through an optomechanically induced transparency experiment, this coupling was experimentally quantified. A comparison to the beforehand deduced theory shows a very good agreement. In conclusion, subsequent prospective experiments towards optomechanical cooling and motion manipulation are explained and preliminary experimental data are discussed.
Hybrid circuit quantum electrodynamics (QED) involves the study of coherent quantum physics in solid state systems via their interactions with superconducting microwave circuits.Here we present a crucial step in the implementation of a hybrid superconducting qubit that employs a carbon nanotube as a Josephson junction.We realise the junction by contacting a carbon nanotube with a superconducting Pd/Al bi-layer, and implement voltage tunability of the quantum circuit's frequency using a local electrostatic gate.We demonstrate a strong dispersive coupling to a coplanar waveguide resonator by investigating the gate-tunable resonator frequency.We extract qubit parameters from spectroscopy using dispersive readout and find qubit relaxation and coherence times in the range of 10 -200 ns.