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arXiv:1504.06895 · Nature Communications

Single-photon non-linear optics with a quantum dot in a waveguide

Alisa Javadi, Immo Söllner, M. Arcari, Sofie Lindskov Hansen, Leonardo Midolo, Sahand Mahmoodian, Gabija Kiršanskė, Tommaso Pregnolato, E. H. Lee, Jin Dong Song, Søren Stobbe, Peter Lodahl

Published Oct 23, 2015• 277 citations
arXivHTMLPDF

Abstract

Strong non-linear interactions between photons enable logic operations for both classical and quantum-information technology. Unfortunately, non-linear interactions are usually feeble and therefore all-optical logic gates tend to be inefficient. A quantum emitter deterministically coupled to a propagating mode fundamentally changes the situation, since each photon inevitably interacts with the emitter, and highly correlated many-photon states may be created. Here we show that a single quantum dot in a photonic-crystal waveguide can be used as a giant non-linearity sensitive at the single-photon level. The non-linear response is revealed from the intensity and quantum statistics of the scattered photons, and contains contributions from an entangled photon-photon bound state. The quantum non-linearity will find immediate applications for deterministic Bell-state measurements and single-photon transistors and paves the way to scalable waveguide-based photonic quantum-computing architectures.

DOI
10.1038/ncomms9655

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Strong non-linear interactions between photons enable logic operations for both classical and quantum-information technology. Unfortunately, non-linear interactions are usually feeble and therefore all-optical logic gates tend to be inefficient. A quantum emitter deterministically coupled to a propagating mode fundamentally changes the situation, since each photon inevitably interacts with the emitter, and highly correlated many-photon states may be created. Here we show that a single quantum dot in a photonic-crystal waveguide can be used as a giant non-linearity sensitive at the single-photon level. The non-linear response is revealed from the intensity and quantum statistics of the scattered photons, and contains contributions from an entangled photon-photon bound state. The quantum non-linearity will find immediate applications for deterministic Bell-state measurements and single-photon transistors and paves the way to scalable waveguide-based photonic quantum-computing architectures.
Abstract Single-atom waveguide-QED systems have emerged as a leading platform for demonstrating non-linear optics in the few-photon regime. Devices with such non-linear behavior are necessary for developing deterministic gates for photonic quantum computing. Artificial atoms coupled to nanophotonic or superconducting waveguides can be used to engineer highly efficient light-matter interfaces for such non-linear interactions, where every photon in the system interacts with the quantum emitter. However, it has been a challenge to access the reflection port of the waveguide due to the inability of rejecting stray electromagnetic fields that do not interact with the artificial atom. Here, we show coherent reflection of single photons from a semiconductor quantum dot strongly coupled to the fundamental waveguide mode of a nanowire. We utilize the tapered end of the nanowire for ideal mode-matching in a vertical geometry, enabled by a novel extinction technique. This mode-matching allows for efficient transfer of photons from the input to the reflection port while having all interacted with the quantum dot. Such a high-efficiency scalable photonic platform opens up applications in few-photon quantum nonlinear optics and has been proposed for creating key resource states for universal photon-based quantum computing.
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A quantum emitter efficiently coupled to a nanophotonic waveguide constitutes a promising system for the realization of single-photon transistors, quantum-logic gates based on giant single-photon nonlinearities, and high bit-rate deterministic single-photon sources. The key figure of merit for such devices is the β factor, which is the probability for an emitted single photon to be channeled into a desired waveguide mode. We report on the experimental achievement of β=98.43%±0.04% for a quantum dot coupled to a photonic crystal waveguide, corresponding to a single-emitter cooperativity of η=62.7±1.5. This constitutes a nearly ideal photon-matter interface where the quantum dot acts effectively as a 1D "artificial" atom, since it interacts almost exclusively with just a single propagating optical mode. The β factor is found to be remarkably robust to variations in position and emission wavelength of the quantum dots. Our work demonstrates the extraordinary potential of photonic crystal waveguides for highly efficient single-photon generation and on-chip photon-photon interaction.
This Thesis is focused on the study of quantum electrodynamics in photonic crystal waveguides. We investigate the interplay between a single quantum dot and the fundamental mode of the photonic crystal waveguide. We demonstrate experimental coupling eciencies for the spontaneous emission into the mode exceeding 98% for emitters spectrally close to the band-edge of the waveguide mode. In addition we illustrate the broadband nature of the underlying eects, by obtaining coupling eciencies above 90% for quantum dots detuned from the band edge by as far as 20nm. These values are in good agreement with numerical simulations. Such a high coupling eciency implies that the system can be considered an articial 1D-atom, and we theoretically show that this system can generate strong photon-photon interaction, which is an essential functionality for deterministic optical quantum information processing. We present the progress towards the experimental demonstration of such a strong photon-photon nonlinearity. We present the rst signatures of resonant transmission in photonic crystal waveguides and discuss some of the encountered diculties and future directions of the experiments. In the nal part of this Thesis we discuss a novel type of photonic crystal waveguide and show its applications for on-chip quantum information processing. This structure was designed for the ecient mapping of two orthogonal circular dipole transitions to dierent propagation paths of the emitted photon, i.e. exhibits chiral quantum-dot-waveguide coupling. Such a structure is ideally suited for a number of applications in quantum information processing and among others we propose an on-chip spin-photon interface, a single photon transistor, and a deterministic cNOT gate.
In this thesis we investigate few-photon non-linearities in all-optical, on-chip circuits, and we discuss their possible applications in devices of interest for quantum information technology, such as conditional two-photon gates and single-photon sources. In order to propose efficient devices, it is crucial to fully understand the non-equilibrium dynamics of strongly interacting photons. Employing both numerical and analytical approaches we map out the full scattering dynamics for two photons scattering on a two-level emitter in a one-dimensional waveguide. The strongest non-linear interaction arise when the emitter is excited the most, which occurs for incoming photon pulses with a spectral bandwidth comparable to the emitter linewidth. For two identical, counter-propagating photons, the emitter works as a non-linear beam splitter, as the emitter induces strong directional correlations between the scattered photons. Even though the non-linearity also alters the pulse spectrum due to a four-wave mixing process, we demonstrate that input pulses with a Gaussian spectrum can be mapped to the output with up to 80 % fidelity. Using two identical two-level emitters, we propose a setup for a deterministic controlled-phase gate, which preserves the properties of the two incoming photons with almost 80 %, limited by spectral changes induced by the non-linearity and phase modulations upon scattering. Another setup for a controlled-phase operation is suggested with two coupled ring resonators exploiting a strong second-order material non-linearity. By dynamically trapping the first of two temporally separated photons in the non-linear resonator, the scattering of the second photon is altered. Due to the trapping, the undesired aforementioned non-linear effects are avoided, but the gate performance is now limited by the capturing process. Semiconductor quantum dots (QDs) are promising for realizing few-photon non-linearities in solid-state implementations, although coupling to phonon modes in the surrounding lattice have significant influence on the dynamics. By accounting for the commonly neglected asymmetry between the electron and hole wavefunction in the QD, we show how the phonon-assisted transition rate to a slightly detuned optical mode may be suppressed. This is achieved by properly matching the electrical carrier confinement with the deformation potential interaction, where the suppression only occurs in materials where the deformation potential interaction shifts the electron and hole bands in the same direction. We demonstrate also how the phonon-induced effects may be altered by placing the QD inside an infinite slab, where the confinement of the phonons is modified instead. For a slab thickness below ∼ 70 nm, the bulk description of the phonon modes may be insufficient. The QD decay rate may be strongly increased or decreased, depending on how the detuning between the QD and the optical mode matches the phonon modes in the slab.
Realizing a sensitive photon-number-dependent phase shift on a light beam is required both in classical and quantum photonics. It may lead to new applications for classical and quantum photonics machine learning or pave the way for realizing photon-photon gate operations. Nonlinear phase-shifts require efficient light-matter interaction, and recently quantum dots coupled to nanophotonic devices have enabled near-deterministic single-photon coupling. We experimentally realize an optical phase shift of 0.19π ± 0.03 radians ( ≈ 34 degrees) using a weak coherent state interacting with a single quantum dot in a planar nanophotonic waveguide. The phase shift is probed by interferometric measurements of the light scattered from the quantum dot in the waveguide. The process is nonlinear in power, the saturation at the single-photon level and compatible with scalable photonic integrated circuitry. The work may open new prospects for realizing high-efficiency optical switching or be applied for proof-of-concept quantum machine learning or quantum simulation demonstrations.