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arXiv:1503.08629 · Physical Review Letters

Measurement and Shaping of Biphoton Spectral Wave Functions

Nora Tischler, Alexander Büse, L. G. Helt, Mathieu L. Juan, Nicolás Piro, Joyee Ghosh, Michael J. Steel, Gabriel Molina‐Terriza

Published Nov 3, 2015• 31 citations
arXivHTMLPDF

Abstract

In this work we present a simple method to reconstruct the complex spectral wave function of a biphoton, and hence gain complete information about the spectral and temporal properties of a photon pair. The technique, which relies on quantum interference, is applicable to biphoton states produced with a monochromatic pump when a shift of the pump frequency produces a shift in the relative frequencies contributing to the biphoton. We demonstrate an example of such a situation in type-II parametric down conversion allowing arbitrary paraxial spatial pump and detection modes. Moreover, our test cases demonstrate the possibility to shape the spectral wave function. This is achieved by choosing the spatial mode of the pump and of the detection modes, and takes advantage of spatiotemporal correlations.

DOI
10.1103/physrevlett.115.193602

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In this work we present a simple method to reconstruct the complex spectral wave function of a biphoton, and hence gain complete information about the spectral and temporal properties of a photon pair. The technique, which relies on quantum interference, is applicable to biphoton states produced with a monochromatic pump when a shift of the pump frequency produces a shift in the relative frequencies contributing to the biphoton. We demonstrate an example of such a situation in type-II parametric down conversion allowing arbitrary paraxial spatial pump and detection modes. Moreover, our test cases demonstrate the possibility to shape the spectral wave function. This is achieved by choosing the spatial mode of the pump and of the detection modes, and takes advantage of spatiotemporal correlations.
The complete measurement of the quantum state of two correlated photons requires reconstructing the amplitude and phase of the biphoton wavefunction. We show how, by means of spatially resolved single photon detection, one can infer the spatial structure of biphotons generated by spontaneous parametric down conversion. In particular, a spatially resolved analysis of the second-order correlations allows us to isolate the moduli of the pump and phase-matching contributions to the two-photon states. When carrying this analysis on different propagation planes, the free-space propagation of pump and phase-matching is observed. This result allows us, in principle, to gain enough information to also reconstruct the phase of the pump and the phase-matching and thus the full biphoton wavefunction. We show this in different examples where the pump is shaped as a superposition of orbital angular momentum modes or as a smooth amplitude with a phase structure with no singularities. The corresponding phase structure is retrieved employing maximum likelihood or genetic algorithms. These findings have potential applications in fast, efficient quantum state characterization that does not require phase locking of the unknown source with a reference biphoton.
We present an experimental implementation of spectral properties engineering on biphoton light, emitted via ultrafast type II spontaneous parametric down conversion (SPDC), based on the shaping of the pump pulse spectrum and propagation of the emitted correlated photons through dispersive media. Spectral properties of a biphoton state are fully characterized by the two-photon spectral amplitude (TPSA). Exploiting the group velocity dispersion (GVD) induced by the passage of optical fields through dispersive media, an energy to time two dimensional Fourier transform of the TPSA is operated: this returns a technique to reconstruct TPSA by means of a temporal measurement among the delay between the laser pulse emission (trigger) and the detection times of the two correlated photons. Exploiting this kind of measurement it is possible to deeply resolve the interference pattern in the shape of TPSA. In this research we report on the conditions under which subtle structure on TPSA spectra can be deliberately engineered via modulation of the pump beam spectrum.
In spontaneous parametric down-conversion, the spectral correlations between the signal and the idler are expressed by the joint spectral amplitude (JSA) function. However, in the standard coincidence measurements, the phase information of the JSA is lost, and only the square of the absolute value of the JSA is recorded, thus preventing full characterization of the biphoton state. Here, we present an experimental technique to investigate the interference of biphoton joint spectral amplitudes, unlocking new avenues in quantum photonics research. Our method explores phase-dependent phenomena within entangled biphoton spectra. This is achieved by simultaneously pumping two structured nonlinear photonic crystals and observing their interference, which reveals previously inaccessible effects with direct intensity measurements. We demonstrate the versatility of our technique by analyzing two types of joint spectra: one exhibiting a two-lobe shape and the other a three-lobe shape. Additionally, we reconstruct the joint spectral amplitudes for both scenarios and observe good agreement with theoretical predictions. These results pave the way for developing advanced quantum communication and information processing technologies using biphoton spectra.
This work is focused on the engineering and characterization of the frequency-time properties of photon pairs generated with a semiconductor source. This device emits photons propagating in opposite directions at telecom wavelengths using spontaneous parametric down-conversion at room temperature. A microcavity integrated in the source allows the resonance of the transverse pump beam, enhancing the efficiency of the nonlinear interaction. We give a theoretical description of the down-conversion process in the source and we show how the spatial and spectral properties of the pump beam impact the properties of the photons, in particular their degree of entanglement in frequency allowing a versatile engineering. The variety of states that can be produced is illustrated using the Joint Spectral Amplitude. Two techniques allowing the characterization of the Joint Spectral Intensity have been implemented. The first one is a single photon spectrograph. The second one, based on the stimulation of the down-conversion process showed a dramatic improvement in terms of resolution and integration time. Both techniques allowed the demonstration of the frequency correlation engineering by varying the waist and curvature radius of the pump beam. Examples of more exotic states and a technique to characterize their chronocyclic Wigner function are theoretically investigated. The relationship between time-frequency properties and degree of entanglement in polarization of the biphoton is also explored.
We investigate spectral and temporal features and entanglement of biphoton wave packets formed in spontaneous parametric down-conversion with a pulsed laser pump. The degree of entanglement is characterized by the experimentally measurable parameter RRR defined as the ratio of the coincidence and single-particle spectral widths. In the frequency representation, this parameter is found as a function of the pump-pulse duration $\ensuremath{\tau}$. The function $R(\ensuremath{\tau})$ is shown to have a minimum and even in the minimum, at rather natural conditions, the degree of entanglement is found to be very high (Rmin=73)({R}_{\mathrm{min}}=73)(Rmin​=73). The Schmidt number KKK is found analytically for both short and long pump pulses and interpolated for arbitrary pulse durations. All functional dependences of RRR and KKK are found to be identical and numerical coefficients are found to be rather close. Two-time temporal wave function of a biphoton state is investigated in detail, and a rather significant difference between the cases of short and long pump pulses is found to occur. In the case of long pulses, the temporal parameter Rt{R}_{t}Rt​ (defined as the ratio of durations of the single-particle and coincidence signals) is shown to be very close to the Schmidt number KKK.
The ability to manipulate and measure the time-frequency structure of quantum light is useful for information processing and metrology. Measuring this structure is also important when developing quantum light sources with high modal purity that can interfere with other independent sources. Here, we present and experimentally demonstrate a scheme based on intensity interferometry to measure the joint spectral mode of photon pairs produced by spontaneous parametric down-conversion. We observe correlations in the spectral phase of the photons due to chirp in the pump. We show that our scheme can be combined with stimulated emission tomography to quickly measure their mode using bright classical light. Our scheme does not require phase stability, nonlinearities, or spectral shaping and thus is an experimentally simple way of measuring the modal structure of quantum light.