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arXiv:1503.01828 · Physical Review A

Localizing spin dynamics in a spin-1 Bose-Einstein condensate via magnetic pulses

Huanbin Li, Zhengguo Pu, Michael Chapman, Wenxian Zhang

Published Jul 27, 2015• 2 citations
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Abstract

Spin-exchange interaction between atoms in a spin-1 Bose-Einstein condensate causes atomic spin evolving periodically under the single-spatial-mode approximation in the mean-field theory. By applying fast magnetic pulses according to a two-step or a four-step control protocol, we find analytically that the spin dynamics is significantly suppressed for an arbitrary initial state. Numerical calculations under single-mode approximation are carried out to confirm the validity and robustness of these protocols. This localization method can be readily utilized to improve the sensitivity of a magnetometer based on spin-1 Bose-Einstein condensates.

DOI
10.1103/physreva.92.013630

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Spin-exchange interaction between atoms in a spin-1 Bose-Einstein condensate causes atomic spin evolving periodically under the single-spatial-mode approximation in the mean-field theory. By applying fast magnetic pulses according to a two-step or a four-step control protocol, we find analytically that the spin dynamics is significantly suppressed for an arbitrary initial state. Numerical calculations under single-mode approximation are carried out to confirm the validity and robustness of these protocols. This localization method can be readily utilized to improve the sensitivity of a magnetometer based on spin-1 Bose-Einstein condensates.
It remains a challenge to independently manipulate the magnetic dipolar and the spin-exchange interactions, which are entangled in many spin systems, particularly in spin-1 Bose-Einstein condensates. For this purpose, we put forward a sequence of rf pulses and the periodic dynamical decoupling sequence of optical Feshbach resonance pulses to control the dipolar and the spin-exchange interactions, respectively. Our analytic results and the numerical simulations demonstrate that either of the two interactions can be suppressed to make the other dominate the spin dynamics; furthermore, both of the interactions can be simultaneously suppressed to realize spinor-condensate--based magnetometers with a higher sensitivity. This manipulation method may find its wide applications in magnetic resonance and spintronics.
Compared to single-component Bose-Einstein condensates, spinor Bose-Einstein condensates display much richer dynamics. In addition to density oscillations, spinor Bose-Einstein condensates exhibit intriguing spin dynamics that is associated with population transfer between different hyperfine components. This paper analyzes the validity of the widely employed single-mode approximation when describing the spin dynamics in response to a quench of the system Hamiltonian. The single-mode approximation assumes that the different hyperfine states all share the same time-independent spatial mode. This implies that the resulting spin Hamiltonian only depends on the spin interaction strength and not on the density interaction strength. Taking the spinor sodium Bose-Einstein condensate in the f=1f=1f=1 hyperfine manifold as an example and working within the mean-field theory framework, it is found numerically that the single-mode approximation misses, in some parameter regimes, intricate details of the spin and spatial dynamics. We develop a physical picture that explains the observed phenomenon. Moreover, using that the population oscillations described by the single-mode approximation enter into the effective potential felt by the mean-field spinor, we derive a semiquantitative condition for when dynamical mean-field induced corrections to the single-mode approximation are relevant. Our mean-field results have implications for a variety of published and planned experimental studies.
With current magnetic-field shielding and high-precision detection in dipolar spinor Bose-Einstein condensates, it is possible to experimentally detect the low- or zero-field nonsecular dipolar dynamics. Here we analytically investigate the zero-field nonsecular magnetic dipolar interaction effect, with an emphasis on magnetization dynamics in a spin-1 Bose-Einstein condensate under the single spatial mode approximation within the mean-field theory. Due to the biaxial nature of the dipolar interaction, a novel resonance occurs in the condensate magnetization oscillation, in contrast to the previous assumption of a conserved magnetization in strong magnetic fields. Furthermore, we propose a dynamical-decoupling detection method for such a resonance, which cancels the stray magnetic fields in experiment but restores the magnetization dynamics. Our results shed light on the dipolar systems and may find potential applications beyond cold atoms.
The spin mixing dynamics of spin-1 Bose–Einstein condensates with zero magnetization and under an external magnetic field is investigated in a systematic way. Beyond the mean field theory, the time-dependent solutions of the Hamiltonian under the single mode approximation are obtained via a procedure of diagonalization. Thereby the time-dependent populations of spin-0 component starting from various initial states are obtained and analyzed. The features of evolution are compared in detail with those with the field removed so as to emphasize the effect of the field. Since the solutions are exact for the Hamiltonian, we can study the long-term behavior of the evolution, where periodicity and inherent symmetry emerge. In particular, some special cases are found in which the evolution is highly sensitive to the field, very strong oscillation in population can be thereby induced. A new mode of oscillation of the population characterized by having two frequencies, one is high and one is low, is found when the field is sufficiently strong.
We propose to localize spin mixing dynamics in a spin-1 Bose-Einstein condensate by a temporal modulation of spin exchange interaction, which is tunable with optical Feshbach resonance. Adopting techniques from coherent control, we demonstrate the localization and freezing of spin mixing dynamics, and the suppression of the intrinsic dynamic instability and spontaneous spin domain formation in a ferromagnetically interacting condensate of 87Rb^{87}\mathrm{Rb}87Rb atoms. This work points to a promising scheme for investigating the weak magnetic spin dipole interaction, which is usually masked by the more dominant spin exchange interaction.
23Na^{23}\mathrm{Na}23Na spin-1 Bose-Einstein condensates are used to experimentally demonstrate that mean-field physics beyond the single-mode approximation can be relevant during the nonequilibrium dynamics. The experimentally observed spin oscillation dynamics and associated dynamical spatial structure formation confirm theoretical predictions that are derived by solving a set of coupled mean-field Gross-Pitaevskii equations [J. Jie et al., Phys. Rev. A 102, 023324 (2020)]. The experiments rely on microwave dressing of the f=1f=1f=1 hyperfine states, where fff denotes the total angular momentum of the 23Na^{23}\mathrm{Na}23Na atom. The fact that physics beyond the single-mode approximation at the mean-field level, i.e., spatial mean-field dynamics that distinguishes the spatial density profiles associated with different Zeeman levels, can, in certain parameter regimes, have a pronounced effect on the dynamics when the spin healing length is comparable to or larger than the size of the Bose-Einstein condensate has implications for using Bose-Einstein condensates as models for quantum phase transitions and spin squeezing studies as well as for nonlinear SU(1,1) interferometers.