Spontaneous macroscopic quantum synchronization is an emergent phenomenon where an ensemble of quantum oscillators achieves global phase coherence through the interplay of interaction and dissipation. To illuminate this phenomenon, we study an ensemble of two-level systems (TLS) and establish its associated nonlinear quantum master equation, for which self-consistent analytical solutions of quantum synchronization can be obtained. The trajectories on the Bloch sphere vividly illustrate how dissipation and interaction drive the system toward a synchronized state. We present a phase diagram for macroscopic synchronization as a function of interaction strength and the gain-to-damping ratio. Furthermore, we demonstrate full synchronization and partial synchronization between two groups of TLS with different natural frequencies. This work establishes ensemble of TLS as a remarkable system for understanding spontaneous quantum synchronization.
Synchronization is a collective phenomenon in which interacting nonlinear oscillators develop a persistent relation between their phases and frequencies. In quantum systems, its description requires connecting the classical dynamics of limit-cycle oscillators with quantum fluctuations, dissipation, and the notion of phase. In this tutorial review, we offer a systematic framework for analyzing synchronization in classical and quantum dynamical systems. Starting from amplitude-phase dynamics, we introduce successively topics of relevance, such as phase locking, the Adler equation, Arnold tongues, and the Kuramoto model, and use these concepts to analyze coupled oscillators and their stability. We then formulate the corresponding description for quantum limit-cycle oscillators using Lindblad master equations and phase-space methods, with explicit examples of two and many coupled oscillators. We further discuss noise, synchronization measures, and the extreme quantum regime, including synchronization in spin systems. The emphasis throughout is on analytical derivations and a practical methodology for identifying synchronized states, determining their stability, and characterizing synchronization in quantum systems. The review is designed as a self-contained guide from which we hope that students can learn the essential concepts and techniques, while researchers can readily find the analytical tools and methodological insights needed to approach new synchronization problems.
Recent advances in generating well controlled dense arrangements of individual atoms in free space have generated interest in understanding how the extended nature of these systems influences superradiance phenomena. Here, we provide an in-depth analysis on how space-dependent light shifts and decay rates induced by dipole-dipole interactions modify the steady-state properties of coherently driven arrays of quantum emitters. We characterize the steady-state phase diagram, with particular focus on the radiative properties in the steady state. Interestingly, we find that diverging from the well-established Dicke paradigm of equal all-to-all interactions significantly modifies the emission properties. In particular, the prominent quadratic scaling of the radiated light intensity with particle number in the steady state—a hallmark of steady-state Dicke superradiance—is entirely suppressed, resulting in only linear scaling with particle number. We show that this breakdown of steady-state superradiance occurs due to the emergence of additional dissipation channels that populate not only superradiant states but also subradiant ones. The additional contribution of subradiant dark states in the dynamics leads to a divergence in the time scales needed to achieve steady states. Building on this, we further show that measurements taken at finite times for extended atom ensembles reveal properties closely mirroring the idealized Dicke scenario. Published by the American Physical Society 2024
We theoretically describe macroscopic quantum synchronization effects occurring in a network of all-to-all coupled quantum limit-cycle oscillators. The coupling causes a transition to synchronization as indicated by the presence of global phase coherence. We demonstrate that the microscopic quantum properties of the oscillators qualitatively shape the synchronization behavior in a macroscopically large network. Specifically, they result in a blockade of collective synchronization that is not expected for classical oscillators. Additionally, the macroscopic ensemble shows emergent behavior not present at the level of two coupled quantum oscillators.
A nanophotonic waveguide coupled with an atomic array forms one of the strongly coupled quantum interfaces to showcase many fascinating collective features of quantum dynamics. In particular, for a dissimilar array of two different interparticle spacings with competing photon-mediated dipole-dipole interactions and directionality of couplings, we study the steady-state phases of atomic excitations under a weakly driven condition of laser field. We identify a partial set of steady-state phases of the driven system composed of combinations of steady-state solutions in a homogeneous array. We also reveal the intricate role of the atom at the interface of the dissimilar array in determining the steady-state phases and find an alteration in the dichotomy of the phases strongly associated with steady-state distributions with crystalline orders. We further investigate in detail the interaction-induced depletion in half of the dissimilar array, where the blockaded region results from two contrasting interparticle spacings near the reciprocal coupling regime. This can be further evidenced from the analytical solutions under the reciprocal coupling. Our results can provide insights in the driven-dissipative quantum phases of atomic excitations with nonreciprocal couplings and pave the avenues toward quantum simulations of exotic many-body states essential for quantum information applications. Published by the American Physical Society 2024
We study the decoherence dynamics of dipole-coupled two-level quantum systems in Ramsey-type experiments. We focus on large networks of two-level systems, confined to two spatial dimensions and with positional disorder giving rise to disordered dipolar couplings. This setting is relevant for modeling the decoherence dynamics of the rotational excitations of polar molecules confined to deep optical lattices, where disorder arises from the random filling of lattice sites with occupation probability
p. We show that the decoherence dynamics exhibits a phase transition at a critical filling ${p}_{c}\ensuremath{\simeq}0.15$. For
p<pc the dynamics is disorder dominated and the Ramsey interference signal decays on a time scale ${T}_{2}\ensuremath{\propto}{p}^{\ensuremath{-}3/2}$. For
p>pc the dipolar interactions dominate the disorder, and the system behaves as a collective spin-ordered phase, representing synchronization of the two-level systems and persistent Ramsey oscillations with divergent
T2 for large systems. For a finite number of two-level systems
N, the spin-ordered phase at
p>pc undergoes a crossover to a collective spin-squeezed state on a time scale ${\ensuremath{\tau}}_{\mathrm{sq}}\ensuremath{\propto}\sqrt{N}$. We develop a self-consistent mean-field theory that is capable of capturing the synchronization transition at
pc, and provide an intuitive theoretical picture that describes the phase transition in the long-time dynamics. We also show that the decoherence dynamics appear to be ergodic in the vicinity of
pc, the long-time behavior being well described by the predictions of equilibrium thermodynamics. The results are supported by the results of exact diagonalization studies of small systems.