Quantum correlations between spatially separated parts of a d-dimensional bipartite system (d ≥ 2) have no classical analog. Such correlations, also called entanglements, are not only conceptually important, but also have a profound impact on information science. In theory the violation of Bell inequalities based on local realistic theories for d-dimensional systems provides evidence of quantum nonlocality. Experimental verification is required to confirm whether a quantum system of extremely large dimension can possess this feature, however it has never been performed for large dimension. Here, we report that Bell inequalities are experimentally violated for bipartite quantum systems of dimensionality d = 16 with the usual ensembles of polarization-entangled photon pairs. We also estimate that our entanglement source violates Bell inequalities for extremely high dimensionality of d > 4000. The designed scenario offers a possible new method to investigate the entanglement of multipartite systems of large dimensionality and their application in quantum information processing.
Quantum correlations between spatially separated parts of a d-dimensional bipartite system (d ≥ 2) have no classical analog. Such correlations, also called entanglements, are not only conceptually important, but also have a profound impact on information science. In theory the violation of Bell inequalities based on local realistic theories for d-dimensional systems provides evidence of quantum nonlocality. Experimental verification is required to confirm whether a quantum system of extremely large dimension can possess this feature, however it has never been performed for large dimension. Here, we report that Bell inequalities are experimentally violated for bipartite quantum systems of dimensionality d = 16 with the usual ensembles of polarization-entangled photon pairs. We also estimate that our entanglement source violates Bell inequalities for extremely high dimensionality of d > 4000. The designed scenario offers a possible new method to investigate the entanglement of multipartite systems of large dimensionality and their application in quantum information processing.
Quantum correlations between spatially separated parts of a d-dimensional bipartite system (d≥2) have no classical analog. Such correlations, also called entanglements, are not only conceptually important, but also have a profound impact on information science. In theory the violation of Bell inequalities based on local realistic theories for d-dimensional systems provides evidence of quantum nonlocality. Experimental verification is required to confirm whether a quantum system of extremely large dimension can possess this feature, however it has never been performed for large dimension (e.g., d≥1000). Here, we report that Bell inequalities are experimentally violated for bipartite quantum systems of extremely high dimensionality with the usual ensembles of polarization-entangled photon pairs. Our entanglement source violates Bell inequalities for extremely high dimensionality of d>4000. The designed scenario offers a possible new method to investigate the entanglement of multipartite systems of large dimensionality and their application in quantum information processing.
Quantum correlations resulting in violations of Bell inequalities have generated a lot of interest in quantum information science and fundamental physics. In this paper, we address some questions that become relevant in Bell-type tests involving systems with local dimension greater than 2. For CHSH-Bell tests within 2D subspaces of such high-dimensional systems, it has been suggested that experimental violation of Tsirelson's bound indicates that more than 2D entanglement was present. We explain that the overstepping of Tsirelson's bound is due to violation of fair sampling, and can in general be reproduced by a separable state, if fair sampling is violated. For a class of Bell-type inequalities generalized to d-dimensional systems, we then consider what level of violation is required to guarantee d-dimensional entanglement of the tested state, when fair sampling is satisfied. We find that this can be used as an experimentally feasible test of d-dimensional entanglement for up to quite high values of d.
It is theoretically and experimentally shown that photons emitted by statistically independent incoherent classical light sources and measured in the far field in spatially separated modes may display spatial correlations akin to path-entanglement of photons produced by quantum sources. By measuring higher order photon-correlations at different locations, i.e., m photons in one mode and one photon in another mode, we experimentally demonstrate for m≥6 a violation of Bell-type inequalities for spatial degrees of freedom. The spatial correlations among the photons can be understood from state projection where the detection of the first m photons projects the sources onto a state which emits the subsequent photon in a strongly correlated manner. From this perspective the entanglement and violation of Bell's inequalities appears as a consequence of nonvanishing cross correlations between noncommuting quadrature phase components of the two spatially separated fields after m photons have been recorded. In this way we show that classical systems may produce spatial field correlations violating local realistic theories.
Quantum entanglement is the ability of joint quantum systems to possess global properties (correlation among systems) even when subsystems have no definite individual property. Whilst the 2-dimensional (qubit) case is well-understood, currently, tools to characterise entanglement in high dimensions are limited. We experimentally demonstrate a new procedure for entanglement certification that is suitable for large systems, based entirely on information-theoretics. It scales more efficiently than Bell's inequality and entanglement witness. The method we developed works for arbitrarily large system dimension d and employs only two local measurements of complementary properties. This procedure can also certify whether the system is maximally entangled. We illustrate the protocol for families of bipartite states of qudits with dimension up to 32 composed of polarisation-entangled photon pairs.
It is one of the most remarkable features of quantum physics that measurements on spatially separated systems cannot always be described by a locally causal theory. In such a theory, the outcomes of local measurements are determined in advance solely by some unknown (or hidden) variables and the choice of local measurements. Correlations that are allowed within the framework of a locally causal theory are termed classical. Typically, the fact that quantum mechanics does not always result in classical correlations is revealed by the violation of Bell inequalities, which are constraints that have to be satisfied by any classical correlations. It has been known for a long time that entanglement is necessary to demonstrate nonclassical correlations, and hence a Bell inequality violation. However, since some entangled quantum states are known to admit explicit locally causal models, the exact role of entanglement in Bell inequality violation has remained obscure. This thesis provides both a comprehensive review on these issues as well as a report on new discoveries made to clarify the relationship between entanglement and Bell inequality violation. In particular, within the framework of a standard Bell experiment, i.e., a Bell inequality test that is directly performed on a single copy of a quantum state r, we have derived two algorithms to determine, respectively, a lower bound and an upper bound on the strength of correlations that r can offer for any given Bell inequality. Both of these algorithms make use convex optimization techniques in the form of a semidefinite program. By examples, we show that these algorithms can often be used in tandem, in conjunction with convexity arguments, to determine if a quantum state can offer nonclassical correlations and hence violates a given Bell inequality. On the other hand, since a standard Bell experiment typically involves measurements over many copies of the quantum systems, we have also investigated the possibility of enhancing the strength of nonclassical correlation by, instead, performing collective measurements on multiple copies of the quantum systems. Our findings show that even without postselection, such joint measurements may also lead to stronger nonclassical correlations, and hence a better Bell inequality violation. Meanwhile, previous studies have indicated that entangled state admitting locally causal models may still lead to observable nonclassical correlations if, prior to a standard Bell experiment, the state is subjected to some appropriate local preprocessing. This phenomenon of hidden nonlocality was discovered more than a decade ago, but to date, it is still not known if all entangled states can demonstrate nonclassical correlations through these more sophisticated Bell experiments. A key result in this thesis then consists of showing that for all bipartite entangled states, observable nonclassical correlations, in the form of a Bell-CHSH inequality violation, can indeed be derived if we allow both local preprocessing and the usage of shared ancillary state which by itself does not violate the Bell-CHSH inequality. This establishes a kind of equivalence between bipartite entanglement and states that cannot be simulated by classical correlations. In summary, for a standard Bell experiment where no local preprocessing on a quantum state r is allowed, we have provided two algorithms that can be used in tandem to determine if r can be simulated by a locally causal theory, whereas in the scenario where local preprocessing is allowed, we have demonstrated that bipartite entangled states are precisely those which cannot always be simulated classically.
Bell inequality tests based on high-dimensional entanglement usually require measurements that can resolve multiple possible outcomes. However, the implementation of high-dimensional multi-outcome measurements is often only emulated via a collection of ``click or no-click'' measurements. This reduction of multi-outcome measurements to binary-outcome measurements opens a loophole in high-dimensional tests Bell inequalities which can be exploited by local hidden variable models [Tavakoli et al., Phys. Rev. A 111, 042433 (2025)]. Here, we close this loophole by using four-dimensional photonic path-mode entanglement and multi-outcome detection. We test both the well-known Collins-Gisin-Linden-Massar-Popescu inequality and a related Bell inequality tailored for maximally entangled states in high-dimension. We observe violations that are large enough to also rule out any quantum model based on entanglement of lower dimension, thereby demonstrating genuinely high-dimensional nonlocality free of the binarisation loophole.