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arXiv:1501.06278 · Physical Review Letters

Operating Spin Echo in the Quantum Regime for an Atomic-Ensemble Quantum Memory

Jun Rui, Yan Jiang, Sheng-Jun Yang, Bo Zhao, Xiao‐Hui Bao, Jian-Wei Pan

Published Sep 24, 2015• 35 citations
arXivHTMLPDF

Abstract

Spin echo is a powerful technique to extend atomic or nuclear coherence times by overcoming the dephasing due to inhomogeneous broadenings. However, there are disputes about the feasibility of applying this technique to an ensemble-based quantum memory at the single-quanta level. In this experimental study, we find that noise due to imperfections of the rephasing pulses has both intense superradiant and weak isotropic parts. By properly arranging the beam directions and optimizing the pulse fidelities, we successfully manage to operate the spin echo technique in the quantum regime by observing nonclassical photon-photon correlations as well as the quantum behavior of retrieved photons. Our work for the first time demonstrates the feasibility of harnessing the spin echo method to extend the lifetime of ensemble-based quantum memories at the single-quanta level.

DOI
10.1103/physrevlett.115.133002

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Spin echo is a powerful technique to extend atomic or nuclear coherence times by overcoming the dephasing due to inhomogeneous broadenings. However, there are disputes about the feasibility of applying this technique to an ensemble-based quantum memory at the single-quanta level. In this experimental study, we find that noise due to imperfections of the rephasing pulses has both intense superradiant and weak isotropic parts. By properly arranging the beam directions and optimizing the pulse fidelities, we successfully manage to operate the spin echo technique in the quantum regime by observing nonclassical photon-photon correlations as well as the quantum behavior of retrieved photons. Our work for the first time demonstrates the feasibility of harnessing the spin echo method to extend the lifetime of ensemble-based quantum memories at the single-quanta level.
A major challenge in quantum technologies is to build an efficient and long-lived quantum memory, particularly using solid-state devices. I will here report on an experiment where we combine the AFC optical memory with spin-echo techniques to extend the memory time from a few microseconds to about 1 ms, using an Europium-doped crystal. In general the spin-echo technique allows one to control the inhomogeneous spin dephasing which often sets the storage-time limit both in solid-state systems and laser-cooled gases. However, theoretically it is has been argued that spin-echo techniques would be extremely difficult to apply without creating noise in the case of a single quanta stored in a large spin ensemble. We here show how this noise can be limited and demonstrate high signal-to-noise ratio in the output mode when storing pulses at the single-photon level. Furthermore we stored polarization qubits encoded onto weak coherent , with fidelities surpassing a classical storage scheme.
Spin-echo techniques are essential for achieving long coherence times in solid-state quantum memories for light because of inhomogeneous broadening of the spin transitions. It has been suggested that unrealistic levels of precision for the radio-frequency control pulses would be necessary for successful decoherence control at the quantum level. Here we study the effects of pulse imperfections in detail, using both a semiclassical and a fully quantum-mechanical approach. Our results show that high efficiencies and low noise-to-signal ratios can be achieved for the quantum memories in the single-photon regime for realistic levels of control pulse precision. We also analyze errors due to imperfect initial-state preparation (optical pumping), showing that they are likely to be more important than control pulse errors in many practical circumstances. These results are crucial for future developments of solid-state quantum memories.
Spin echo techniques are essential for achieving long coherence times in solid state quantum memories for light because of inhomogeneous broadening of the spin transitions. Here we study the effects of radio frequency decoherence control pulse imperfections in detail, using both a semi-classical and a fully quantum-mechanical approach. Our results show that high efficiencies and low noise-to-signal ratios can be achieved for the quantum memories in the single-photon regime for realistic levels of control pulse precision. We also analyze errors due to imperfect initial state preparation (optical pumping), showing that they are likely to be more important than control pulse errors in many practical circumstances. These results are crucial for future developments of solid state quantum memories.
Rephasing in photon echoes is a fundamental mechanism of retrieving optical information stored in a collective ensemble of atoms or ions. With an extremely weak quantum optical data, population inversion by the rephasing process is inevitable resulting in serious quantum noise. Here, an inversion-free rephasing method in photon echoes is presented by using deshelving-based atom phase control. The present method makes photon echoes directly applicable to quantum memories with benefits of extended photon storage time and nearly perfect retrieval efficiency. In this revised version only the rephasing pulse propagation direction is corrected to make a silent echo of E1 in Fig. 1.
Long-lived quantum memories are essential components of a long-standing goal of remote distribution of entanglement in quantum networks. These can be realized by storing the quantum states of light as single-spin excitations in atomic ensembles. However, spin states are often subjected to different dephasing processes that limit the storage time, which in principle could be overcome using spin-echo techniques. Theoretical studies suggest this to be challenging due to unavoidable spontaneous emission noise in ensemble-based quantum memories. Here, we demonstrate spin-echo manipulation of a mean spin excitation of 1 in a large solid-state ensemble, generated through storage of a weak optical pulse. After a storage time of about 1 ms we optically read-out the spin excitation with a high signal-to-noise ratio. Our results pave the way for long-duration optical quantum storage using spin-echo techniques for any ensemble-based memory.
Quantum memories for quantum communication need to be able to store photons for an extended time and then to release them on demand. This can be achieved in atomic frequency comb ensemble-based quantum memories by control pulses that transfer the excitation to and from long-lived spin states. However, such pulses can give rise to coherent and incoherent noise due to their interaction with the memory ensemble. In this paper, we experimentally demonstrate the ability to switch off the coherent noise from such control pulses during the echo emission in a spin-wave quantum memory, using the linear Stark effect in rare-earth-ion doped crystals. By applying an electric-field pulse, the echo emission was coherently switched off prior to the first spin transfer pulse, and the stored data pulse was restored only when both an optical recall pulse and a rephasing electrical pulse were applied, giving a high degree of control of both desired and undesired emissions. We estimate the effectiveness of this technique by turning off the free-induction decay of a narrow ensemble of ions. This technique can thus improve the noise performance of spin-wave storage at the single-photon level by quenching coherent optical radiation created by strong control pulses. The method demonstrated here represents a proof of principle that the spin-wave storage scheme can be combined with Stark control. The combined scheme serves as an addition to the toolbox of techniques that can be used to realize a full version of a quantum repeater. Published by the American Physical Society 2024