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arXiv:1501.03495 · Physical Review Letters

Constraining Quantum Critical Dynamics: (2+1)D Ising Model and Beyond

William Witczak‐Krempa

Published Apr 28, 2015• 26 citations
arXivHTMLPDF

Abstract

Quantum critical (QC) phase transitions generally lead to the absence of quasiparticles. The resulting correlated quantum fluid, when thermally excited, displays rich universal dynamics. We establish nonperturbative constraints on the linear-response dynamics of conformal QC systems at finite temperature, in spatial dimensions above 1. Specifically, we analyze the large frequency or momentum asymptotics of observables, which we use to derive powerful sum rules and inequalities. The general results are applied to the O(N) Wilson-Fisher fixed point, describing the QC Ising model when N=1. We focus on the order parameter and scalar susceptibilities, and the dynamical shear viscosity. Connections to simulations, experiments, and gauge theories are made.

DOI
10.1103/physrevlett.114.177201

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Quantum critical (QC) phase transitions generally lead to the absence of quasiparticles. The resulting correlated quantum fluid, when thermally excited, displays rich universal dynamics. We establish nonperturbative constraints on the linear-response dynamics of conformal QC systems at finite temperature, in spatial dimensions above 1. Specifically, we analyze the large frequency or momentum asymptotics of observables, which we use to derive powerful sum rules and inequalities. The general results are applied to the O(N) Wilson-Fisher fixed point, describing the QC Ising model when N=1. We focus on the order parameter and scalar susceptibilities, and the dynamical shear viscosity. Connections to simulations, experiments, and gauge theories are made.
The perturbative approach to the description of long-wavelength excitations at high temperature breaks down near the critical point of a second order phase transition. We study the dynamics of these excitations in a relativistic scalar field theory at and near the critical point via a renormalization group approach at high temperature and an $\ensuremath{\epsilon}$ expansion in $d=5\ensuremath{-}\ensuremath{\epsilon}$ space-time dimensions. The long-wavelength physics is determined by a nontrivial fixed point of the renormalization group. At the critical point we find that the dispersion relation and width of quasiparticles of momentum p are ${\ensuremath{\omega}}_{p}\ensuremath{\sim}{p}^{z}$ and ${\ensuremath{\Gamma}}_{p}\ensuremath{\sim}(z\ensuremath{-}1){\ensuremath{\omega}}_{p},$ respectively, and the group velocity of quasiparticles ${v}_{g}\ensuremath{\sim}{p}^{z\ensuremath{-}1}$ vanishes in the long-wavelength limit at the critical point. Away from the critical point for $T\ensuremath{\gtrsim}{T}_{c}$ we find ${\ensuremath{\omega}}_{p}\ensuremath{\sim}{\ensuremath{\xi}}^{\ensuremath{-}z}[1+(p\ensuremath{\xi}{)}^{2z}{]}^{1/2}$ and ${\ensuremath{\Gamma}}_{p}\ensuremath{\sim}(z\ensuremath{-}1){\ensuremath{\omega}}_{p}(p\ensuremath{\xi}{)}^{2z}/[1+(p\ensuremath{\xi}{)}^{2z}]$ with $\ensuremath{\xi}$ the finite temperature correlation length $\ensuremath{\xi}\ensuremath{\propto}|T\ensuremath{-}{T}_{c}{|}^{\ensuremath{-}\ensuremath{\nu}}.$ The new dynamical exponent z results from anisotropic renormalization in the spatial and time directions. For a theory with O(N)O(N)O(N) symmetry we find $z=1+\ensuremath{\epsilon}{(N+2)/(N+8)}^{2}+\mathcal{O}({\ensuremath{\epsilon}}^{2}).$ This dynamical critical exponent describes a new universality class for dynamical critical phenomena in quantum field theory. Critical slowing down, i.e., a vanishing width in the long-wavelength limit, and the validity of the quasiparticle picture emerge naturally from this analysis.
We study high-frequency response functions, notably the optical conductivity, in the vicinity of quantum critical points (QCPs) by allowing for both detuning from the critical coupling and finite temperature. We consider general dimensions and dynamical exponents. This leads to a unified understanding of sum rules. In systems with emergent Lorentz invariance, powerful methods from quantum field theory allow us to fix the high-frequency response in terms of universal coefficients. We test our predictions analytically in the large-N O(N) model and using the gauge-gravity duality and numerically via quantum Monte Carlo simulations on a lattice model hosting the interacting superfluid-insulator QCP. In superfluid phases, interacting Goldstone bosons qualitatively change the high-frequency optical conductivity and the corresponding sum rule.
In this thesis I investigate several aspects of local quantum criticality, a concept of key importance in a number of physical contexts ranging from critical heavy fermion compounds to quantum dot systems. Quantum critical points are associated with second order phase transitions at zero temperature. In contrast to their finite-temperature counterparts, the zero-point motion cannot be neglected near a quantum critical point. As a result, the incorporation of quantum dynamics leads to an effective dimension larger than the spatial dimension of the system for the order parameter fluctuations within the Ginzburg-Landau-Wilson treatment of criticality. This so-called quantum-to-classical mapping works well for the critical properties in insulating systems but apparently fails in systems containing gapless fermions. This has been experimentally most clearly been demonstrated within a particular class of intermetallic compounds called heavy fermions. A particular way in which the Ginzburg-Landau-Wilson paradigm fails is for critical Kondo destruction that seems to underlie the unconventional quantum criticality seen in the heavy fermions. I focus on studying the properties of critical Kondo destruction and the emergence of energy-over-temperature-scaling in systems without spatial degrees of freedom, i.e., so-called quantum impurity systems. In particular, I employ large-N techniques to address critical properties of this class of quantum phase transitions in and out of equilibrium. As quantum critical systems are characterized by a scale-invariant spectrum with many low-lying excitations, it may appear that any perturbation can lead to a response beyond the linear response regime. Understanding what governs the non-linear response regime near quantum criticality is an interesting area. Here, I first present a path integral version of the Schrieffer-Wolff transformation which relates the functional integral form of the partition function of the Anderson model to that of its effective low-energy model. The equivalence between the low-energy sector of the Anderson model in the Kondo regime and the spin-isotropic Kondo model is usually established via a canonical transformation performed on the Hamiltonian, followed by a projection. The resulting functional integral assumes the form of a spin path integral and includes a geometric phase factor, i.e. a Berry phase. The approach stresses the underlying symmetries of the model and allows for a straightforward generalization of the transformation to more involved models. As an example of the efficiency of the approach I apply it to a single electron transistor attached to ferromagnetic leads and derive the effective low-energy model of such a magnetic transistor. As Kondo screening is a local phenomenon, it and its criticality can be studied using the appropriate impurity model. A general impurity model to study critical Kondo destruction is the pseudogap Bose-Fermi Kondo model. Here, I concentrate on the multi-channel version of the model using the dynamical large-N study. This model allows to study the non-trivial interplay between two different mechanisms of critical Kondo destruction. The interplay of two processes that can each by itself lead to critical Kondo destruction. The zero-temperature residual entropy at various fixed points for the model is also discussed. The two channel Anderson model exhibits several continuous quantum phase transitions between weak- and strong-coupling phases. The non-crossing approximation (NCA) is believed to give reliable results for the standard two-channel Anderson model of a magnetic impurity in a metal. I revisit the reliability of the NCA for the standard two channel Anderson model (constant conduction electron density of states) and investigate its reliability for the two-channel pseudogap Anderson model. This is done by comparing finite-temperature, finite-frequency solutions of the NCA equations and asymptotically exact zero-temperature NCA solutions with numerical renormalization-group calculations. The phase diagram of this model is well established. The focus here will be on the dynamical scaling properties obtained within the NCA. Finally, I study the thermal and non-thermal steady state scaling functions and the steady-state dynamics of the pseudogap Kondo model. This model allows us to study the concept of effective temperatures near fully interacting as well as weak-coupling fixed points and compare the out-of-equilibrium scaling properties of critical Kondo destruction to those of the traditional spin-density wave (SDW) scenario. The differences I identify can be experimentally probed. This may be helpful in identifying the nature of the quantum critical points observed in certain heavy fermion compounds.
Quantum phase transition arises in general as second order phase transition at zero temperature, tuned by a non-thermal parameter such as pressure, doping or a magnetic field. The point in the phase diagram of the material in which different phases meet is called a quantum critical point (QCP). Physics around QCPs are of extensive current interest because the critical quantum fluctuations influence the physical properties in a wide temperature range (quantum criticality), and are believed to be responsible for many emergent physical properties such as non-Fermi liquids and unconventional superconductivity. In this research we explore dynamics and thermodynamics near QCPs via investigating three classes of models, which all have real material correspondence. Specifically first, we study local dynamics in a perturbed quantum critical Ising chain with E8 symmetry, where we show the local dynamical spin susceptibility has a singular dependence on frequency, but differs from the diffusion form. The nuclear magnetic resonance (NMR) relaxation rate at low temperatures depends exponentially on the inverse temperature, whose prefactor we also determine. We propose NMR experiments as a means to further test the applicability of the E8 description for CoNb2O6. Second, we investigate the thermodynamic properties of itinerant ferromagnets near quantum critical points, described by the quantum Landau-Ginzburg theory. We provide a regularized perturbative renormalization group procedure to calculate the free energy. We further carry out numerical calculations on thermodynamic quantities, capturing not only the leading critical behaviors, but also the subleading and nonsingular contributions. We demonstrate various thermodynamic signatures of quantum criticality, including the entropy accumulation effect and the divergence of the specific heat coefficient. A detailed comparison to the recent experimental results on an itinerant ferromagnet Sr3Ru2O7 is also presented. Third, we explore Ising-nematic and magnetic phases and their transitions in iso-electronically doped iron pnictides by carrying out a large-N study of an effective low-energy Ginzburg-Landau model for these systems. We demonstrate that the magnetic and Ising orders transitions are concurrent at zero temperature, and both transitions are weakly first-order, which is consistent with RG-based prediction and experimental observations.
We discuss the quench dynamics near a quantum critical point focusing on the sine-Gordon model as a primary example. We suggest a unified approach to sudden and slow quenches, where the tuning parameter $\ensuremath{\lambda}(t)$ changes in time as $\ensuremath{\lambda}(t)\ensuremath{\sim}\ensuremath{\upsilon}{t}^{r}$, based on the adiabatic expansion of the excitation probability in powers of $\ensuremath{\upsilon}$. We show that the universal scaling of the excitation probability can be understood through the singularity of the generalized adiabatic susceptibility ${\ensuremath{\chi}}_{2r+2}(\ensuremath{\lambda})$, which for sudden quenches (r=0)(r=0)(r=0) reduces to the fidelity susceptibility. In turn this class of susceptibilities is expressed through the moments of the connected correlation function of the quench operator. We analyze the excitations created after a sudden quench of the cosine potential using a combined approach of form-factors expansion and conformal perturbation theory for the low-energy and high-energy sector, respectively. We find the general scaling laws for the probability of exciting the system, the density of excited quasiparticles, the entropy and the heat generated after the quench. In the two limits where the sine-Gordon model maps to hard-core bosons and free massive fermions we provide the exact solutions for the quench dynamics and discuss the finite temperature generalizations.
We investigate two-dimensional spin models and begin with an introduction to critical phenomena with emphasis on classical systems with boundaries and conformal invariance. Then we introduce the antiferromagnetic quantum Heisenberg model with frustrating interactions. Conformal invariance of a statistical mechanical system at criticality has powerful implications in two dimensions. With the use of conformal field theory, we investigate finite-size and boundary effects for a class of N-critical models that describe the simplest type of multicritical behaviour. In Papers I and II, correlation functions for the order parameter and other operators of these multicritical Ising models are derived for restricted domains (semi-infinite plane, infinite strip, disc and rectangle) with free or fixed boundary conditions. These yield the corresponding universal surface exponents and allow for a detailed analysis of correlations lengths, structure factors and response functions. The interplay between duality and boundary conditions is also made explicit. In Paper III, we analyse structure factors at criticality and show how apparent power- law scaling at intermediate momenta - induced by finite size and boundaries - depends on the boundary conditions applied. The predictions are confirmed by using correlation functions calculated in Papers I and II. Two-dimensional Heisenberg antiferromagnets have attracted much attention because of their relation to high-Tc superconductors. The second part of the thesis (Papers IV and V) treats spin-1/2 antiferromagnets defined on square- and honeycomb lattices with frustrating interactions. By using a Schwinger-boson mean-field theory, we calculate low-temperature quantum corrections to thermodynamic parameters, such as spin-wave velocity and transverse susceptibility. Their dependence on frustration is explicated and used to estimate the stability of the Néel state via a mapping to the nonlinear .sigma. model that describes the low-energy limit of the antiferromagnet.