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arXiv:1412.8472 · New Journal of Physics

Exotic roton excitations in quadrupolar Bose–Einstein condensates

M Lahrz, M Lemeshko, L Mathey

Published Apr 14, 2015• 14 citations
arXivHTMLPDF

Abstract

We investigate the occurrence of rotons in a quadrupolar Bose–Einstein condensate confined to two dimensions. Depending on the particle density, the ratio of the contact and quadrupole–quadrupole interactions, and the alignment of the quadrupole moments with respect to the confinement plane, the dispersion relation features two or four point-like roton minima or one ring-shaped minimum. We map out the entire parameter space of the roton behavior and identify the instability regions. We propose to observe the exotic rotons by monitoring the characteristic density wave dynamics resulting from a short local perturbation, and discuss the possibilities to detect the predicted effects in state-of-the-art experiments with ultracold homonuclear molecules.

DOI
10.1088/1367-2630/17/4/045005

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We investigate the occurrence of rotons in a quadrupolar Bose–Einstein condensate confined to two dimensions. Depending on the particle density, the ratio of the contact and quadrupole–quadrupole interactions, and the alignment of the quadrupole moments with respect to the confinement plane, the dispersion relation features two or four point-like roton minima or one ring-shaped minimum. We map out the entire parameter space of the roton behavior and identify the instability regions. We propose to observe the exotic rotons by monitoring the characteristic density wave dynamics resulting from a short local perturbation, and discuss the possibilities to detect the predicted effects in state-of-the-art experiments with ultracold homonuclear molecules.
Roton excitations constitute a key feature of dipolar gases, connecting these gases with superfluid helium. We show that the density dependence of the roton minimum results in a spatial roton confinement, particularly relevant in pancake dipolar condensates with large aspect ratios. We show that roton confinement plays a crucial role in the dynamics after roton instability, and that arresting the instability may create a trapped roton gas revealed by confined density modulations. We discuss the local susceptibility against density perturbations, which we illustrate for the case of vortices. Roton confinement is expected to play a key role in experiments.
Dipolar Bose-Einstein condensates (dBECs) exhibit a plethora of physics phenomena, from supersolidity to the rotonlike minimum in the elementary excitation spectrum. In this work we first demonstrate the existence of axis-symmetric solitary waves in (quasi-)two-dimensional dBECs: these localized excitations are characterized by quantized vortex dipoles that continuously transit to vortex-free density depletions. We then show how the presence of the roton minimum fundamentally alters the fate of such solutions when approaching Landau’s critical speed: when propagating along the polarization direction where the roton minimum occurs, the solitary wave transits into roton excitations rather than into phonons as for standard contact-interaction BECs. This finding suggests that Feynman’s hypothesis, conjectured for 3D superfluid liquid helium regarding the creation of rotons as fading vortex excitations, is valid in the context of 2D dBECs.
The effect of dipolar orientation with respect to the condensate plane on the mean-field dynamics of dipolar Bose-Einstein condensates in a pancake-shaped confinement is discussed. The stability of a quasi-two-dimensional condensate, with respect to the tilting angle, is found to be different from a two-dimensional layer of dipoles, indicating the relevance of the transverse extension while characterizing two-dimensional dipolar systems. An anisotropic excitation spectrum exhibiting a highly tunable, rotonlike minimum can arise entirely from the dipole-dipole interactions, by tilting the dipoles. At the magic angle and in the absence of contact interactions, the long-wavelength excitations are not phononlike and always unstable. The post-roton-instability dynamics, in contrast to phonon instability, in a uniform condensate, is featured by a transient, defect-free, stripe pattern, which eventually undergoes local collapses, and driving the condensate back into the stable regime can make them sustained for longer. Hopping between stripes has been observed before it melts into a uniform state in the presence of dissipation. Finally, we discuss a class of solutions, in which a quasi-two-dimensional condensate is self-trapped in one direction, as well as a regime of interaction parameters, including attractive short-range interactions, at which a two-dimensional anisotropic soliton can be stabilized, and we show that a chromium condensate with a relatively small number of atoms is well suited for this.
In three dimensions, noninteracting bosons undergo Bose-Einstein condensation at a critical temperature, T(c), which is slightly shifted by ΔT(c), if the particles interact. We calculate the excitation spectrum of interacting Bose systems, (4)He and (87)Rb, and show that a roton minimum emerges in the spectrum above a threshold value of the gas parameter. We provide a general theoretical argument for why the roton minimum and the maximal upward critical temperature shift are related. We also suggest two experimental avenues to observe rotons in condensates. These results, based upon a path-integral Monte Carlo approach, provide a microscopic explanation of the shift in the critical temperature and also show that a roton minimum does emerge in the excitation spectrum of particles with a structureless, short-range, two-body interaction.
Ensembles with long-range interactions between particles are promising for revealing strong quantum collective effects and many-body phenomena. Here we study the ground-state phase diagram of a two-dimensional Bose system with quadrupolar interactions using a diffusion Monte Carlo technique. We predict a quantum phase transition from a gas to a solid phase. The Lindemann ratio and the condensate fraction at the transition point are $\ensuremath{\gamma}=0.269(4)$ and n0/n=0.031(4){n}_{0}/n=0.031(4)n0​/n=0.031(4), correspondingly. We observe the strong rotonization of the collective excitation branch in the vicinity of the phase transition point. Our results can be probed using state-of-the-art experimental systems of various nature, such as quasi-two-dimensional systems of quadrupolar excitons in transition metal dichalcogenide trilayers, quadrupolar molecules, and excitons or Rydberg atoms with quadrupole moments induced by strong magnetic fields.
Dipolar Bose-Einstein condensates (dBECs) exhibit a plethora of physics phenomena, from supersolidity to the rotonlike minimum in the elementary excitation spectrum. In this work we first demonstrate the existence of axis-symmetric solitary waves in (quasi-)two-dimensional dBECs: these localized excitations are characterized by quantized vortex dipoles that continuously transit to vortex-free density depletions. We then show how the presence of the roton minimum fundamentally alters the fate of such solutions when approaching Landau's critical speed: when propagating along the polarization direction where the roton minimum occurs, the solitary wave transits into roton excitations rather than into phonons as for standard contact-interaction BECs. This finding suggests that Feynman's hypothesis, conjectured for 3D superfluid liquid helium regarding the creation of rotons as fading vortex excitations, is valid in the context of 2D dBECs.