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arXiv:1411.7065 · Physical Review Letters

Quantum Manipulation of Two-Electron Spin States in Isolated Double Quantum Dots

Benoît Bertrand, Hanno Flentje, Shintaro Takada, Michihisa Yamamoto, Seigo Tarucha, Arne Ludwig, Andreas Dirk Wieck, Christopher Bäuerle, Tristan Meunier

Published Aug 28, 2015• 79 citations
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Abstract

We studied experimentally the dynamics of the exchange interaction between two antiparallel electron spins in an isolated double quantum dot where coupling to the electron reservoirs can be ignored. We demonstrate that the level of control of such a double dot is higher than in conventional double dots. In particular, it allows us to couple coherently two electron spins in an efficient manner following a scheme initially proposed by Loss and DiVincenzo [Phys. Rev. A 57, 120 (1998)]. The present study demonstrates that isolated quantum dots are a possible route to increase the number of coherently coupled quantum dots.

DOI
10.1103/physrevlett.115.096801

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We studied experimentally the dynamics of the exchange interaction between two antiparallel electron spins in an isolated double quantum dot where coupling to the electron reservoirs can be ignored. We demonstrate that the level of control of such a double dot is higher than in conventional double dots. In particular, it allows us to couple coherently two electron spins in an efficient manner following a scheme initially proposed by Loss and DiVincenzo [Phys. Rev. A 57, 120 (1998)]. The present study demonstrates that isolated quantum dots are a possible route to increase the number of coherently coupled quantum dots.
Recently, an implementation of a universal set of one- and two-quantum-bit gates for quantum computation using spin states of coupled single-electron quantum dots was proposed. It was demonstrated that it is possible to execute a coherent control of a quantum system based on two-electron spin states in a double quantum dot, allowing state preparation, coherent manipulation, and projective readout. This possibility is based on rapid electrical control of the spin exchange interaction. These results motivated us to develop a formal theoretical study of the corresponding model of two coupled spins placed in a magnetic field and subjected to a time-dependent mutual Heisenberg interaction. Using possible exact solutions of the corresponding quantum problem, we study entangling of different separable initial states in this model. It is demonstrated that the entanglement due to a time-dependent Heisenberg interaction is dominating in comparison with the entanglement due to the action of an external magnetic field.
We have analyzed theoretically quenched dynamics of correlated double quantum dot (DQD) due to the switching "on" and "off" coupling to reservoirs. The possibility for controllable manipulation of charge and spin states in the double quantum dot was revealed and discussed. The proposed experimental scheme allows to prepare in DQD maximally entangled pure triplet state and to drive it to another entangled singlet state by tuning both applied bias and gate voltage. It was also demonstrated that the symmetry properties of the total system (double quantum dot coupled to electron reservoirs) allow to resolve the initially prepared two-electron states by detecting non-stationary spin-polarized currents flowing in both reservoirs and controlling the residual charge.
Recent experiments have demonstrated quantum manipulation of two-electron spin states in double quantum dots using electrically controlled exchange interactions. Here we present a detailed theory for electron-spin dynamics in two-electron double-dot systems that was used to guide those experiments and analyze the results. Specifically, we analyze both spin- and charge-relaxation and dephasing mechanisms that are relevant to experiments and discuss practical approaches for quantum control of two-electron systems. We show that both charge and spin dephasing play important roles in the dynamics of the two-spin system, but neither represents a fundamental limit for electrical control of spin degrees of freedom in semiconductor quantum bits.
Quantum dots are microscopic structures that can trap single electrons for study and manipulation. Such devices are of interest as potential logic elements in a future quantum computer in which electron spins are used as quantum bits. The problem is that the spins on the nuclei of the device material itself can interfere with the electron spins. In his Perspective, [DiVincenzo][1] discusses results reported in the same issue by [ Petta et al. ][2] in which a double quantum dot structure was used to avoid the effect of the background spins. By swapping the quantum spin states back and forth between the dots, the researchers were able to greatly increase the quantum coherence time of the stored states. The results show that fully electric (as opposed to magnetic) control of the spin states offers the possibility of using such double dots in a quantum computer. [1]: http://www.sciencemag.org/cgi/content/full/309/5744/2173 [2]: http://www.sciencemag.org/cgi/content/short/309/5744/2180
A robust scheme for state preparation and state trapping for the spins of two electrons in a semiconductor double quantum dot is presented. The system is modeled by two spins coupled to two independent bosonic reservoirs. Decoherence effects due to this environment are minimized by application of optimized control fields which make the target state to the ground state of the isolated driven spin system. We show that stable spin entanglement with respect to pure dephasing is possible. Specifically, we demonstrate state trapping in a maximally entangled state (Bell state) in the presence of decoherence.
Semiconductor double‐quantum dots represent an ideal system for studying the novel spin physics of localized spins. On each quantum dot when the number of electrons is odd and the net spin is 1/2, a strong coupling of this localized spin to conducting electrons in the leads gives rise to Kondo correlation. On the other hand, in the coupled double‐quantum‐dot if the inter‐dot antiferromagnetic interaction is strong, the two spins can form a correlated spin‐singlet state, quenching the Kondo effect. This competition between Kondo and antiferromagnetic correlation is studied in a controlled manner by tuning the inter‐dot tunnel coupling. Increasing the inter‐dot tunneling, we observe a continuous transition from a single‐peaked to a double‐peaked Kondo resonance in the differential conductance. On the double‐peaked side, the differential conductance becomes suppressed at zero source‐drain bias. The observed strong suppression of the differential conductance at zero bias provides direct evidence signaling the formation of an entangled spin‐singlet state. This evidence for entanglement and the tunability of our devices bode well for quantum computation applications.