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arXiv:1411.4258 · Physical Review A

Spinor Bose-Einstein condensates of rotating polar molecules

Yuangang Deng, S. Yi

Published Sep 25, 2015• 4 citations
arXivHTMLPDF

Abstract

We propose a scheme to realize a pseudospin-$1/2$ model of the ${}^{1}\mathrm{\ensuremath{\Sigma}}(v=0)$ bialkali polar molecules with the spin states corresponding to two sublevels of the first excited rotational level. We show that the effective dipole-dipole interaction between two spin-$1/2$ molecules couples the rotational and orbital angular momenta and is highly tunable via a microwave field. We also investigate the ground-state properties of a spin-$1/2$ molecular condensate. A variety of nontrivial quantum phases, including the doubly quantized vortex states, are discovered. Our scheme can also be used to create spin-1 model of polar molecules. Thus we show that the ultracold gases of bialkali polar molecules provide a unique platform for studying the spinor condensates of rotating molecules.

DOI
10.1103/physreva.92.033624

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We propose a scheme to realize a pseudospin-1/21/21/2 model of the 1\ensuremathΣ(v=0){}^{1}\mathrm{\ensuremath{\Sigma}}(v=0)1\ensuremathΣ(v=0) bialkali polar molecules with the spin states corresponding to two sublevels of the first excited rotational level. We show that the effective dipole-dipole interaction between two spin-1/21/21/2 molecules couples the rotational and orbital angular momenta and is highly tunable via a microwave field. We also investigate the ground-state properties of a spin-1/21/21/2 molecular condensate. A variety of nontrivial quantum phases, including the doubly quantized vortex states, are discovered. Our scheme can also be used to create spin-1 model of polar molecules. Thus we show that the ultracold gases of bialkali polar molecules provide a unique platform for studying the spinor condensates of rotating molecules.
An experimental proposal for realizing spin-orbit (SO) coupling of pseudospin 1 in the ground manifold ${}^{1}\mathrm{\ensuremath{\Sigma}}(\ensuremath{\upsilon}=0)$ of (bosonic) bialkali polar molecules is presented. The three spin components are composed of the ground rotational state and two substates from the first excited rotational level. Using hyperfine resolved Raman processes through two select excited states resonantly coupled by a microwave, an effective coupling between the spin tensor and linear momentum is realized. The properties of Bose-Einstein condensates for such SO-coupled molecules exhibiting dipolar interactions are further explored. In addition to the SO-coupling-induced stripe structures, the singly and doubly quantized vortex phases are found to appear, implicating exciting opportunities for exploring novel quantum physics using SO-coupled rotating polar molecules with dipolar interactions.
We investigate the properties of the ground state and low-lying excitations of an oblate Bose-Einstein condensate composed of rigid rotor molecules in the presence of an external polarizing electric field. We build in a quantum model of molecular polarizability by including the full manifold of rotational states. The interplay between spatial and microscopic degrees of freedom via feedback between the molecular polarizability and inter-molecular dipole-dipole interactions leads to a rich quasi-particle spectrum. Under large applied fields, we reproduce the well-understood density-wave rotonization that appears in a fully polarized dipolar BEC, but under smaller applied fields, we predict the emergence of a spin wave instability and possible new stable ground state phases.
We review the topic of quantized vortices in multicomponent Bose–Einstein condensates of dilute atomic gases, with an emphasis on the two-component condensates. First, we review the fundamental structure, stability and dynamics of a single vortex state in a slowly rotating two-component condensates. To understand recent experimental results, we use the coupled Gross–Pitaevskii equations and the generalized nonlinear sigma model. An axisymmetric vortex state, which was observed by the JILA group, can be regarded as a topologically trivial skyrmion in the pseudospin representation. The internal, coherent coupling between the two components breaks the axisymmetry of the vortex state, resulting in a stable vortex molecule (a meron pair). We also mention unconventional vortex states and monopole excitations in a spin-1 Bose–Einstein condensate. Next, we discuss a rich variety of vortex states realized in rapidly rotating two-component Bose–Einstein condensates. We introduce a phase diagram with axes of rotation frequency and the intercomponent coupling strength. This phase diagram reveals unconventional vortex states such as a square lattice, a double-core lattice, vortex stripes and vortex sheets, all of which are in an experimentally accessible parameter regime. The coherent coupling leads to an effective attractive interaction between two components, providing not only a promising candidate to tune the intercomponent interaction to study the rich vortex phases but also a new regime to explore vortex states consisting of vortex molecules characterized by anisotropic vorticity. A recent experiment by the JILA group vindicated the formation of a square vortex lattice in this system.
We present a technique for engineering quantum magnets via ultracold polar molecules in optical lattices and explore exotic interplay between its spin superfluidity and solidity. The molecular ground and first excited rotational states are resonantly coupled by a linearly polarized microwave field. The spin-up (spin-down) states are presented by molecular rotational states of electric dipole moment along (against) the coupling field. By controlling the angle between the lattice direction and the coupling field, the inter-site interaction can be tuned from antiferromagnetic to ferromagnetic. Furthermore, the dipole-dipole interaction induces an exotic interplay between spin superfluidity and solidity, and spin supersolid phases may appear in mediate regions.
We propose an experimental scheme to create spin-orbit coupling in spin-3 Cr atoms using Raman processes. By employing the linear Zeeman effect and optical Stark shift, two spin states within the ground electronic manifold are selected, which results in a pseudospin-1/2 model. We further study the ground state structures of a spin-orbit-coupled Cr condensate. We show that, in addition to the stripe structures induced by the spin-orbit coupling, the magnetic dipole-dipole interaction gives rise to the vortex phase, in which a spontaneous spin vortex is formed.
This thesis contains theoretical studies of weakly interacting, trapped Bose-Einstein condensed gases. The main emphasis is on the rotational properties of these systems. A typical Bose-Einstein condensate reacts to external rotation by forming singly quantized vortices. By the word ”typical” we refer to a condensate with repulsive interparticle interactions and with a frozen spin degree of freedom. However, there are some atomic species for which the low-energy interactions are attractive. Moreover, the tuning of different condensate properties is relatively easy. For example, there are ways to experimentally change the effective interaction from repulsive to attractive. For an attractively interacting condensate the vortex is not the only possible rotational state but the sample may also experience rotation through its center of mass. In the first part of the thesis, we analyze some properties of a rotating attractive Bose gas at the zero temperature limit. First, we note that in order to maintain energetical stability, the gas has to be rotated in an external trap which is steeper than a harmonic trap. We study the system in an anharmonic quadratic + quartic potential. The rotating ground state phase-space is determined with analytical and numerical methods. If the interactions are strong enough, the rotating ground state appears to be a state with the rotating center of mass. On the other hand, at the limit of weak interactions the system experiences rotation by forming a multiply quantized vortex. We also determine the spectrum of elementary excitations for these quantum many-particle states. We find that the broken symmetry of the center of mass rotating state induces an additional zero-energy (Goldstone) mode and that the small oscillations of the ground state exhibit the decoupling between the center of mass and relative motions. If the spin of the atoms is allowed to change freely, a rich variety of topological excitations in condensates can be studied. External rotation is one of the tools for examining the excitations in spinor condensates. In a spinless scalar condensate the appearance of a quantized vortex is manifested by the vortex line in which the condensate density vanishes. In the plane perpendicular to the vortex line, one speaks of the vortex core for the density minimum. We study the properties of slowly rotated F = 1 spinor condensates and show that for ferromagnetic interactions the ground state is a coreless vortex. While the individual spin components may carry ordinary vortices the overall density of the system is coreless. We also study a method to create a point-like monopole structure in a ferromagnetic condensate by suitably imprinting vortices and solitons for different spin components of the condensate.