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arXiv:1411.1622 · Physical Review B

Gapless chiral spin liquid in a kagome Heisenberg model

Samuel Bieri, Laura Messio, B. Bernu, C. Lhuillier

Published Aug 14, 2015• 90 citations
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Abstract

Motivated by recent experiments on the Heisenberg $S=1/2$ quantum spin liquid candidate material kapellasite, we classify all possible chiral (time-reversal symmetry breaking) spin liquids with fermionic spinons on the kagome lattice. We obtain the phase diagram for the physically relevant extended Heisenberg model, comparing the energies of a wide range of microscopic variational wave functions. We propose that, at low temperature, kapellasite exhibits a gapless chiral spin liquid phase with spinon Fermi surfaces. This two-dimensional state inherits many properties of the nearby one-dimensional phase of decoupled antiferromagnetic spin chains, but also shows some remarkable differences. We discuss the spin structure factors and other physical properties.

DOI
10.1103/physrevb.92.060407

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Motivated by recent experiments on the Heisenberg S=1/2S=1/2S=1/2 quantum spin liquid candidate material kapellasite, we classify all possible chiral (time-reversal symmetry breaking) spin liquids with fermionic spinons on the kagome lattice. We obtain the phase diagram for the physically relevant extended Heisenberg model, comparing the energies of a wide range of microscopic variational wave functions. We propose that, at low temperature, kapellasite exhibits a gapless chiral spin liquid phase with spinon Fermi surfaces. This two-dimensional state inherits many properties of the nearby one-dimensional phase of decoupled antiferromagnetic spin chains, but also shows some remarkable differences. We discuss the spin structure factors and other physical properties.
Using a perturbative renormalization group approach, we show that the extended ( J_1-J_2-J_d J 1 − J 2 − J d ) Heisenberg model on the kagome lattice with a staggered chiral interaction ( J_\chi J χ ) can exhibit a gapless chiral quantum spin liquid phase. Within a coupled-chain construction, this phase can be understood as a chiral sliding Luttinger liquid with algebraic decay of spin correlations along the chain directions. We calculate the low-energy properties of this gapless chiral spin liquid using the effective field theory and show that they are compatible with the predictions from parton mean-field theories with symmetry-protected line Fermi surfaces. These results may be relevant to the state observed in the kapellasite material.
We present a general review of the projective symmetry group classification of fermionic quantum spin liquids for lattice models of spin S=1/2S=1/2S=1/2. We then introduce a systematic generalization of the approach for symmetric Z2{\mathbb{Z}}_{2}Z2​ quantum spin liquids to the one of chiral phases (i.e., singlet states that break time reversal and lattice reflection, but conserve their product). We apply this framework to classify and discuss possible chiral spin liquids on triangular and kagome lattices. We give a detailed prescription on how to construct quadratic spinon Hamiltonians and microscopic wave functions for each representation class on these lattices. Among the chiral Z2{\mathbb{Z}}_{2}Z2​ states, we study the subset of U(1) phases variationally in the antiferromagnetic ${J}_{1}\text{\ensuremath{-}}{J}_{2}\text{\ensuremath{-}}{J}_{d}$ Heisenberg model on the kagome lattice. We discuss static spin structure factors and symmetry constraints on the bulk spectra of these phases.
We calculate dynamical spin structure factors for gapped chiral spin liquid states in the spin-1/2 Heisenberg antiferromagnet on the kagome lattice using Schwinger-boson mean-field theory. In contrast to static (equal-time) structure factors, the dynamical structure factor shows clear signatures of time-reversal symmetry breaking for chiral spin liquid states. In particular, momentum inversion $\mathbit{k}\ensuremath{\rightarrow}\ensuremath{-}\mathbit{k}$ symmetry as well as the sixfold rotation symmetry around the $\mathrm{\ensuremath{\Gamma}}$ point are lost. We highlight other interesting features, such as a relatively flat onset of the two-spinon continuum for the cuboc1 state. Our work is based on the projective symmetry group classification of time-reversal symmetry breaking Schwinger-boson mean-field states by Messio, Lhuillier, and Misguich.
Abstract The nature of the ground state for the S = 1/2 Kagome Heisenberg antiferromagnet (KHAF) has been elusive. We revisit this challenging problem and provide numerical evidence that its ground state is a chiral spin liquid. Combining the density matrix renormalization group method with analytical analyses, we demonstrate that the previously observed chiral spin liquid phase in the KHAF with longer-range couplings is stable in a broader region of the phase diagram. We characterize the nature of the ground state by computing energy derivatives, revealing the ground-state degeneracy arising from the spontaneous breaking of the time-reversal symmetry, and targeting the semion sector. We further investigate the phase diagram in the vicinity of the KHAF and observe a 3×3\sqrt{3}\times \sqrt{3}3​×3​ 3 × 3 magnetically ordered phase and two valence-bond crystal phases.
Inspired by the recent discovery of a new instability towards a chiral phase of the classical Heisenberg model on the kagome lattice, we propose a specific chiral spin liquid that reconciles different, well-established results concerning both the classical and quantum models. This proposal is analyzed in an extended mean-field Schwinger boson framework encompassing time reversal symmetry breaking phases, which allows both a classical and a quantum phase description. At low temperatures, we find that quantum fluctuations favor this chiral phase, which is stable against small perturbations of second- and third-neighbor interactions. For spin-1/2, this phase may be, beyond the mean field, a chiral gapped spin liquid. Such a phase is consistent with the density matrix renormalization group results of Yan et al. [Science 332, 1173 (2011)]. Mysterious features of the low-lying excitations of exact diagonalization spectra also find an explanation in this framework. Moreover, thermal fluctuations compete with quantum ones and induce a transition from this flux phase to a planar zero flux phase at a nonzero value of the renormalized temperature (T/S2), reconciling these results with those obtained for the classical system.
The search for exotic quantum spin liquid states in simple yet realistic spin models remains a central challenge in the field of frustrated quantum magnetism. Here we consider the canonical nearest-neighbor kagome Heisenberg antiferromagnet restricted to a quasi-one-dimensional strip consisting entirely of corner-sharing triangles. Using large-scale density matrix renormalization group calculations, we identify in this model an extended gapless quantum phase characterized by central charge c=2c=2c=2 and power-law decaying spin and bond-energy correlations which oscillate at tunably incommensurate wave vectors. We argue that this intriguing spin liquid phase can be understood as a marginal instability of a two-band spinon Fermi surface coupled to an emergent U(1) gauge field, an interpretation which we substantiate via bosonization analysis and Monte Carlo calculations on model Gutzwiller variational wave functions. Our results represent one of the first numerical demonstrations of emergent fermionic spinons in a simple SU(2) invariant nearest-neighbor Heisenberg model beyond the strictly one-dimensional (Bethe chain) limit.